Display Omitted We report a novel simple sub-15nm L/S patterning process using PS-b-PMMA for DSA lithography.The HP 15nm L/S DSA patterning was demonstrated on 300mm wafer.3D BCP internal defect could be minimized by an optimization of material and anneal conditions.The 15nm PS line patterns were transferred into SOG/SOC stacked substrate. In order to evaluate process performances of directed self-assembly (DSA) lithography for semiconductor device manufacturing, we developed a novel simple sub-15nm line-and-space (L/S) patterning process using polystyrene-block-poly(methyl methacrylate) (PS-b-PMMA) lamellar block copolymer (BCP). The new process with grapho- and chemo-hybrid coordinated line epitaxy, using trimming resist and shallow etching spin-on-glass (SOG) as pinning guide, requires neither special pinning guide materials to control surface free energy on guideline patterns nor any resist strip process after guideline pattern fabrication. In this process, insolubility and thermal resistance of pinning guide are provided by shallow SOG etching deposition residue consisting of SOG-occurring Si and CF4 gas-occurring CF compound. By optimization of guide resist critical dimension (CD) and resist film thickness, the half-pitch (HP) 15nm L/S patterns after dry development were fabricated with the maximum dose margin of approximately 15%. The HP 15nm L/S DSA patterning after SOG full etching was demonstrated on 300mm wafer with 85 chips. The presence of characteristic 3-dimensional (3D) BCP internal defects related to PS short defects was suggested by observation at SOG half-depth etching condition, and defects could be minimized by optimization of neutral layer (NL) material and sufficient phase-separation annealing. The 15nm PS line patterns were transferred to SOG and spin-on-carbon (SOC) stacked substrate.
[1]
K. Daoulas,et al.
Computing free energies of interfaces in self-assembling systems.
,
2009,
Physical chemistry chemical physics : PCCP.
[2]
Hirokazu Kato,et al.
Sub-30nm via interconnects fabricated using directed self-assembly
,
2013
.
[3]
Takayuki Toshima,et al.
Contact hole shrink process using graphoepitaxial directed self-assembly lithography
,
2013
.
[4]
Joy Y. Cheng,et al.
Simple and versatile methods to integrate directed self-assembly with optical lithography using a polarity-switched photoresist.
,
2010,
ACS nano.
[5]
Jian Yin,et al.
The SMARTTM Process for Directed Block Co-Polymer Self-Assembly
,
2013
.
[6]
Juan J. de Pablo,et al.
Chemical Patterns for Directed Self-Assembly of Lamellae-Forming Block Copolymers with Density Multiplication of Features
,
2013
.
[7]
Moon Jeong Park,et al.
Phase Behavior of Symmetric Sulfonated Block Copolymers
,
2008
.
[8]
Hirokazu Kato,et al.
Electrical Via Chain Yield for DSA Contact Hole Shrink Process
,
2013
.