Groundwater flow and radionuclide transport calculations for a performance assessment of a low-level waste site

Abstract Predictions of subsurface radionuclide transport are used to support the groundwater pathway analysis for the performance assessment of the low-level, solid radioactive waste site at Los Alamos National Laboratory. Detailed process-based models rather than higher-level performance-assessment models are used to perform the transport calculations. The deterministic analyses predict the fate of the waste from its source, through the vadose zone, into the saturated zone and, finally, the potential dose to humans at the accessible environment. The calculations are run with the finite-element code FEHM, which simulates fluid flow, heat transport, and reactive, contaminant transport through porous and fractured media. The modeling approach for this study couples realistic source-term models with an unsaturated-zone flow and transport model, which is then linked to the saturated-zone flow and transport model. The three-dimensional unsaturated-zone flow and transport model describes the complex hydrology associated with the mesa-top and volcanic geology of the site. The continued migration of nuclides into the main aquifer is calculated using a three-dimensional, steady-flow, saturated-zone model that maintains the spatial and temporal distribution of nuclide flux from the vadose zone. Preliminary results for the aquifer-related dose assessments show that doses are well below relevant performance objectives for low-level waste sites. A general screening technique that compares the nuclide's half-life to its unsaturated-zone travel time is described. This technique helps to decrease the number of transport calculations required at a site. In this case, over half the nuclides were eliminated from further consideration through this screening.

[1]  W. J. Herrera,et al.  Distribution of radionuclides and water in Bandelier Tuff beneath a former Los Alamos liquid waste disposal site after 33 years , 1984 .

[2]  E. Vold,et al.  Phase two of the source release modeling for the Los Alamos Area G Disposal Facility Performance Assessment , 1997 .

[3]  C. Welty,et al.  A Critical Review of Data on Field-Scale Dispersion in Aquifers , 1992 .

[4]  N. A. Eisenberg,et al.  Development of a Performance Assessment Capability in the Waste Management Programs of the U.S. Nuclear Regulatory Commission , 1999, Risk analysis : an official publication of the Society for Risk Analysis.

[5]  I. Triay,et al.  Batch sorption results for neptunium transport through Yucca Mountain tuffs. Yucca Mountain Site Characterization Program milestone 3349 , 1996 .

[6]  B. G. J. Thompson The role of performance assessment in the regulation of underground disposal of radioactive wastes: an international perspective. , 1999 .

[7]  Claude Degueldre,et al.  Groundwater colloid properties: a global approach , 2000 .

[8]  R. V. Fisher Models for pyroclastic surges and pyroclastic flows , 1979 .

[9]  W. E. Soll,et al.  The influence of coatings and fills on flow in fractured, unsaturated tuff porous media systems , 1998 .

[10]  Van Genuchten,et al.  A closed-form equation for predicting the hydraulic conductivity of unsaturated soils , 1980 .

[11]  M. A. Rogers,et al.  History and environmental setting of LASL near-surface land disposal facilities for radioactive wastes (Areas A, B, C, D, E, F, G, and T). Appendixes. [Appendices only] , 1977 .

[12]  F. Goff,et al.  Stratigraphic relations and lithologic variations in the Jemez volcanic field , 1986 .

[13]  M. A. Rogers,et al.  History and environmental setting of LASL near-surface land disposal facilities for radioactive wastes (Areas A, B, C, D, E, F, G, and T). A source document , 1977 .

[14]  W. D. Purtymun,et al.  Geologic and hydrologic records of observation wells, test holes, test wells, supply wells, springs, and surface water stations in the Los Alamos area , 1995 .

[15]  Jiamin Wan,et al.  Colloid transport in unsaturated porous media , 1994 .

[16]  R. Carsel,et al.  Developing joint probability distributions of soil water retention characteristics , 1988 .

[17]  S. P. Neuman Universal scaling of hydraulic conductivities and dispersivities in geologic media , 1990 .

[18]  H. A. Dockery,et al.  Total-system performance assessment for Yucca Mountain - SNL second iteration (TSPA-1993); Volume 2 , 1994 .

[19]  E. A. Klavetter,et al.  A continuum model for water movement in an unsaturated fractured rock mass , 1988 .

[20]  James L. Conca,et al.  Diffusion And Flow In Gravel, Soil, And Whole Rock , 1992 .

[21]  D. K. Smith,et al.  Migration of plutonium in ground water at the Nevada Test Site , 1999, Nature.

[22]  B. Robinson,et al.  Summary of the Models and Methods for the FEHM Application-A Finite-Element Heat- and Mass-Transfer Code , 1997 .

[23]  R. A. Bailey,et al.  The Bandelier Tuff: A study of ash-flow eruption cycles from zoned Magma Chambers , 1966 .