Optimal representation of source‐sink fluxes for mesoscale carbon dioxide inversion with synthetic data

[1] The inversion of CO2 surface fluxes from atmospheric concentration measurements involves discretizing the flux domain in time and space. The resolution choice is usually guided by technical considerations despite its impact on the solution to the inversion problem. In our previous studies, a Bayesian formalism has recently been introduced to describe the discretization of the parameter space over a large dictionary of adaptive multiscale grids. In this paper, we exploit this new framework to construct optimal space-time representations of carbon fluxes for mesoscale inversions. Inversions are performed using synthetic continuous hourly CO2 concentration data in the context of the Ring 2 experiment in support of the North American Carbon Program Mid Continent Intensive (MCI). Compared with the regular grid at finest scale, optimal representations can have similar inversion performance with far fewer grid cells. These optimal representations are obtained by maximizing the number of degrees of freedom for the signal (DFS) that measures the information gain from observations to resolve the unknown fluxes. Consequently information from observations can be better propagated within the domain through these optimal representations. For the Ring 2 network of eight towers, in most cases, the DFS value is relatively small compared to the number of observations d (DFS/d < 20%). In this multiscale setting, scale-dependent aggregation errors are identified and explicitly formulated for more reliable inversions. It is recommended that the aggregation errors should be taken into account, especially when the correlations in the errors of a priori fluxes are physically unrealistic. The optimal multiscale grids allow to adaptively mitigate the aggregation errors.

[1]  M. Ghil,et al.  A stochastic-dynamic model for the spatial structure of forecast error statistics , 1983 .

[2]  I. Fung,et al.  Observational Contrains on the Global Atmospheric Co2 Budget , 1990, Science.

[3]  Gloor,et al.  A Large Terrestrial Carbon Sink in North America Implied by Atmospheric and Oceanic Carbon Dioxide Data and Models , 2022 .

[4]  Corinne Le Quéré,et al.  Regional changes in carbon dioxide fluxes of land and oceans since 1980. , 2000, Science.

[5]  Clive D Rodgers,et al.  Inverse Methods for Atmospheric Sounding: Theory and Practice , 2000 .

[6]  Thomas Kaminski,et al.  On aggregation errors in atmospheric transport inversions , 2001 .

[7]  T Kaminski,et al.  Inverse modeling of atmospheric carbon dioxide fluxes. , 2001, Science.

[8]  R L Tao,et al.  The Broad Reach of Helminthology , 2001, Science.

[9]  Ian G. Enting,et al.  Inverse problems in atmospheric constituent transport , 2002 .

[10]  John C. Lin,et al.  A near-field tool for simulating the upstream influence of atmospheric observations: The Stochastic Time-Inverted Lagrangian Transport (STILT) model , 2003 .

[11]  Sander Houweling,et al.  CO 2 flux history 1982–2001 inferred from atmospheric data using a global inversion of atmospheric transport , 2003 .

[12]  Ian G. Enting,et al.  Data and modelling requirements for CO2 inversions using high-frequency data , 2003 .

[13]  John C. Lin,et al.  Toward constraining regional‐scale fluxes of CO2 with atmospheric observations over a continent: 2. Analysis of COBRA data using a receptor‐oriented framework , 2003 .

[14]  P. Tans,et al.  A geostatistical approach to surface flux estimation of atmospheric trace gases , 2004 .

[15]  Petra Seibert,et al.  Source-receptor matrix calculation with a Lagrangian particle dispersion model in backward mode , 2004 .

[16]  Philippe Bousquet,et al.  Daily CO2 flux estimates over Europe from continuous atmospheric measurements: 1, inverse methodology , 2005 .

[17]  Jordan G. Powers,et al.  A Description of the Advanced Research WRF Version 2 , 2005 .

[18]  Christoph Gerbig,et al.  What can tracer observations in the continental boundary layer tell us about surface-atmosphere fluxes? , 2005 .

[19]  Markus Reichstein,et al.  On the assignment of prior errors in Bayesian inversions of CO2 surface fluxes , 2006 .

[20]  Philippe Bousquet,et al.  Mesoscale inversion: first results from the CERES campaign with synthetic data , 2007 .

[21]  J. Randerson,et al.  An atmospheric perspective on North American carbon dioxide exchange: CarbonTracker , 2007, Proceedings of the National Academy of Sciences.

[22]  François-Marie Bréon,et al.  Contribution of the Orbiting Carbon Observatory to the estimation of CO2 sources and sinks: Theoretical study in a variational data assimilation framework , 2007 .

[23]  A. J. Dolman,et al.  Modelling representation errors of atmospheric CO2 mixing ratios at a regional scale , 2008 .

[24]  G. Powers,et al.  A Description of the Advanced Research WRF Version 3 , 2008 .

[25]  Philippe Bousquet,et al.  What can we learn from European continuous atmospheric CO 2 measurements to quantify regional fluxes – Part 1: Potential of the 2001 network , 2008 .

[26]  Olivier Pannekoucke,et al.  Structure of the transport uncertainty in mesoscale inversions of CO 2 sources and sinks using ensemble model simulations , 2008 .

[27]  Philippe Bousquet,et al.  What can we learn from European continuous atmospheric CO 2 measurements to quantify regional fluxes – Part 2: Sensitivity of flux accuracy to inverse setup , 2008 .

[28]  Wouter Peters,et al.  Modelling representation errors of atmospheric CO2 concentrations at a regional scale , 2008 .

[29]  E. Lokupitiya,et al.  Incorporation of crop phenology in Simple Biosphere Model (SiBcrop) to improve land-atmosphere carbon exchanges from croplands , 2009 .

[30]  Marc Bocquet Toward Optimal Choices of Control Space Representation for Geophysical Data Assimilation , 2009 .

[31]  Beniamino Gioli,et al.  Bridging the gap between atmospheric concentrations and local ecosystem measurements , 2009 .

[32]  Vineet Yadav,et al.  Regional-scale geostatistical inverse modeling of North American CO 2 fluxes: a synthetic data study , 2009 .

[33]  Nicholas C. Parazoo,et al.  A regional high-resolution carbon flux inversion of North America for 2004 , 2010 .

[34]  Lin Wu,et al.  Optimal representation of source‐sink fluxes for mesoscale carbon dioxide inversion with synthetic data , 2011 .

[35]  Colm Sweeney,et al.  Constraining the CO 2 budget of the corn belt: exploring uncertainties from the assumptions in a mesoscale inverse system , 2011 .

[36]  Marc Bocquet,et al.  Bayesian design of control space for optimal assimilation of observations. Part II: Asymptotic solutions , 2011 .

[37]  Marc Bocquet,et al.  Constraining surface emissions of air pollutants using inverse modelling: method intercomparison and a new two-step two-scale regularization approach , 2011 .

[38]  Lin Wu,et al.  Bayesian design of control space for optimal assimilation of observations. Part I: Consistent multiscale formalism , 2011 .

[39]  A X EL O SSES,et al.  Constraining surface emissions of air pollutants using inverse modelling : method intercomparison and a new two-step two-scale regularization approach , 2011 .

[40]  Shamil Maksyutov,et al.  Atmospheric CO2 inversion validation using vertical profile measurements: Analysis of four independent inversion models , 2011 .