Critical levels and loads and the regulation of industrial emissions in northwest British Columbia, Canada

Abstract Northwest British Columbia, Canada, a sparsely populated and largely pristine region, is targeted for rapid industrial growth owing to the modernization of an aluminum smelter and multiple proposed liquefied natural gas (LNG) facilities. Consequently, air quality in this region is expected to undergo considerable changes within the next decade. In concert, the increase in LNG capacity driven by gas production from shale resources across North America has prompted environmental concerns and highlighted the need for science-based management decisions regarding the permitting of air emissions. In this study, an effects-based approach widely-used to support transboundary emissions policy negotiations was used to assess industrial air emissions in the Kitimat and Prince Rupert airsheds under permitted and future potential industrial emissions. Critical levels for vegetation of SO 2 and NO 2 and critical loads of acidity and nutrient nitrogen for terrestrial and aquatic ecosystems were estimated for both regions and compared with modelled concentration and deposition estimates to identify the potential extent and magnitude of ecosystem impacts. The critical level for SO 2 was predicted to be exceeded in an area ranging from 81 to 251 km 2 in the Kitimat airshed owing to emissions from an existing smelter, compared with 2 in Prince Rupert under the lowest to highest emissions scenarios. In contrast, the NO 2 critical level was not exceeded in Kitimat, and ranged from 4.5 to 6 km 2 in Prince Rupert owing to proposed LNG related emissions. Predicted areal exceedance of the critical load of acidity for soil ranged from 1 to 28 km 2 in Kitimat and 4–10 km 2 in Prince Rupert, while the areal exceedance of empirical critical load for nutrient N was predicted to be greater in the Prince Rupert airshed (20–94 km 2 ) than in the Kitimat airshed (1–31 km 2 ). The number of lakes that exceeded the critical load of acidity did not vary greatly across emissions scenarios in the Kitimat (21–23 out of 80 sampled lakes) and Prince Rupert (0 out of 35 sampled lakes) airsheds. While critical loads have been widely used to underpin international emissions reductions of transboundary pollutants, it is clear that they can also play an important role in managing regional air emissions. In the current study, exceedance of critical levels and loads suggests that industrial emissions from the nascent LNG export sector may require careful regulation to avoid environmental impacts. Emissions management from LNG export facilities in other regions should consider critical levels and loads analyses to ensure industrial development is synergistic with ecosystem protection. While recognizing uncertainties in dispersion modelling, critical load estimates, and subsequent effects, the critical levels and loads approach is being used to inform regulatory decisions in British Columbia to prevent impacts that have been well documented in other regions.

[1]  R. Cameron,et al.  CYANOLICHENS: THEIR RESPONSE TO POLLUTION AND POSSIBLE MANAGEMENT STRATEGIES FOR THEIR CONSERVATION IN NORTHEASTERN NORTH AMERICA , 2004 .

[2]  L. H. Weinstein,et al.  Fluorides in the Environment: Effects on Plants and Animals , 2003 .

[3]  J. Lynch,et al.  FOCUS: A pilot study for national-scale critical loads development in the United States , 2014 .

[4]  M. Small,et al.  A regional pH-alkalinity relationship , 1986 .

[5]  William H. McDowell,et al.  Nitrogen Saturation in Temperate Forest Ecosystems , 1998 .

[6]  Oa Us Epa 2012 National Ambient Air Quality Standards (NAAQS) for Particulate Matter (PM) , 2016 .

[7]  S. Piketh,et al.  Atmospheric dry and wet deposition of sulphur and nitrogen species and assessment of critical loads of acidic deposition exceedance in South Africa , 2011 .

[8]  J. Aherne,et al.  Impacts of nitrogen and sulphur deposition on forest ecosystem services in Canada , 2013 .

[9]  J. Aherne,et al.  Critical Load Assessments and Dynamic Model Applications for Lakes in North America , 2015 .

[10]  G. Hornberger,et al.  Time scales of catchment acidification. A quantitative model for estimating freshwater acidification. , 1985, Environmental science & technology.

[11]  C. Curtis,et al.  Critical loads of sulphur and nitrogen for freshwaters in Great Britain and assessment of deposition reduction requirements with the First-order Acidity Balance (FAB) model , 2000 .

[12]  Fluoride emissions and forest survival, growth and regeneration , 1984 .

[13]  L. Nanus,et al.  Mapping critical loads of nitrogen deposition for aquatic ecosystems in the Rocky Mountains, USA. , 2012, Environmental pollution.

[14]  P. Dillon,et al.  Critical loads of acidity for surface waters in south-central Ontario, Canada: regional application of the Steady-State Water Chemistry (SSWC) model , 2002 .

[15]  M. Posch,et al.  Critical loads of acidity for surface waters , 1995 .

[16]  A. P. Wolfe,et al.  Critical Nitrogen Deposition Loads in High-elevation Lakes of the Western US Inferred from Paleolimnological Records , 2011 .

[17]  M. Turetsky,et al.  Response of Sphagnum fuscum to Nitrogen Deposition: A Case Study of Ombrogenous Peatlands in Alberta, Canada , 2003 .

[18]  J. Cape Direct damage to vegetation caused by acid rain and polluted cloud: definition of critical levels for forest trees. , 1993, Environmental pollution.

[19]  J. Aherne,et al.  Estimating base cation weathering rates in Canadian forest soils using a simple texture-based model , 2010 .

[20]  José G. Siri,et al.  Changes in European greenhouse gas and air pollutant emissions 1960–2010: decomposition of determining factors , 2014, Climatic Change.

[21]  L. Sheppard,et al.  Fine Structure of Acid Mist Treated Sitka Spruce Needles: Open-top Chamber and Field Experiments , 1996 .

[22]  Maximilian Posch,et al.  Steady-State Models for Calculating Critical Loads of Acidity for Surface Waters , 2001 .

[23]  J. Aherne,et al.  Past, present, and future exceedance of critical loads of acidity for surface waters in Finland. , 2012, Environmental science & technology.

[24]  J. Aherne,et al.  Staggering reductions in atmospheric nitrogen dioxide across Canada in response to legislated transportation emissions reductions , 2016 .

[25]  J. Aherne,et al.  Vegetation community change points suggest that critical loads of nutrient nitrogen may be too high , 2016 .

[26]  B. Gimeno,et al.  Empirical and simulated critical loads for nitrogen deposition in California mixed conifer forests. , 2008, Environmental pollution.

[27]  B. Emmett Nitrogen Saturation of Terrestrial Ecosystems: Some Recent Findings and Their Implications for Our Conceptual Framework , 2007 .

[28]  H. Sverdrup,et al.  Weathering of primary silicate minerals in the natural soil environment in relation to a chemical weathering model , 1988, Water, Air, and Soil Pollution.

[29]  L. Geiser,et al.  Lichen-based critical loads for atmospheric nitrogen deposition in Western Oregon and Washington Forests, USA. , 2010, Environmental pollution.

[30]  P. Dillon,et al.  A comparison of weathering rates for acid-sensitive catchments in Nova Scotia, Canada and their impact on critical load calculations , 2006 .

[31]  M. Whitmore,et al.  Responses of Herbaceous and Woody Plants to the Dry Deposition of SO2 and NO2 , 1987 .

[32]  P. Dillon,et al.  Critical Loads of Acidity for Surface Waters in South-Central Ontario, Canada: Regional Application of the First-Order Acidity Balance (FAB) Model , 2004 .

[33]  J. Aherne,et al.  The hydrochemistry of high-elevation lakes in the Georgia Basin, British Columbia , 2010 .

[34]  J. Aherne,et al.  Steady-state critical loads of acidity for forest soils in the Georgia Basin, British Columbia , 2010 .

[35]  Paul R. Wyrwoll,et al.  national ambient air quality standards (NAAQS) , 2012 .

[36]  H. Laudon,et al.  A Novel Environmental Quality Criterion for Acidification in Swedish Lakes – An Application of Studies on the Relationship Between Biota and Water Chemistry , 2007 .

[37]  Daniel Kurz,et al.  A2M - A program to compute all possible mineral modes from geochemical analyses , 2007, Comput. Geosci..

[38]  P. Arp,et al.  Determination and Mapping Critical Loads of Acidity and Exceedances for Upland Forest Soils in Eastern Canada , 2006 .

[39]  M. Lindholm,et al.  Nutrient enrichment effects of atmospheric N deposition on biology in oligotrophic surface waters - a review (ICP Waters report 101/2010) , 2010 .

[40]  G. Heuvelink,et al.  A generic framework for spatial prediction of soil variables based on regression-kriging , 2004 .

[41]  Back to the basics - estimating the sensitivity of freshwater to acidification using traditional approaches. , 2010, Journal of environmental management.

[42]  C. Guerreiro Air quality in Europe : 2013 report , 2013 .

[43]  C. Curtis,et al.  Critical loads of acidity for Irish lakes , 2003, Aquatic Sciences.

[44]  Budiman Minasny,et al.  On digital soil mapping , 2003 .

[45]  Harald Sverdrup,et al.  Calculating critical loads of acid deposition with PROFILE — A steady-state soil chemistry model , 1992 .

[46]  J. Lodge Air quality guidelines for Europe: WHO regional publications, European series, No. 23, World Health Organization, 1211 Geneva 27, Switzerland; WHO publications center USA, 49 Sheridan Avenue, Albany, NY 12210, 1987, xiii + 426 pp. price: Sw. fr. 60 , 1988 .

[47]  G. Likens,et al.  The biogeochemistry of calcium at Hubbard Brook , 1998 .

[48]  C. Gagnon,et al.  Soil weathering rates in 21 catchments of the Canadian Shield , 2011 .

[49]  M. Fenn,et al.  Interactive Effects of Air Pollution and Climate Change on Forest Ecosystems in the United States: Current Understanding and Future Scenarios , 2013 .

[50]  Assessing the Potential Extent of Damage to Inland Lakes in Eastern Canada due to Acidic Deposition. I. Development and Evaluation of a Simple "Site" Model , 1990 .

[51]  P. Arp,et al.  Modelling and mapping critical loads and exceedances for the Georgia Basin, British Columbia, using a zero base-cation depletion criterion , 2010 .

[52]  J. Clague Delaciation of the Prince Rupert – Kitimat area, British Columbia , 1985 .

[53]  Andrew Buffin,et al.  Improving cumulative effects assessment in Alberta: Regional strategic assessment , 2011 .

[54]  Kenneth R. Foster,et al.  Development and Application of Critical, Target and Monitoring Loads for the Management of Acid Deposition in Alberta, Canada , 2001 .

[55]  J. Lynch,et al.  Effects of nitrogen deposition and empirical nitrogen critical loads for ecoregions of the United States , 2011 .

[56]  W. K. Hicks,et al.  Factors Affecting Nitrogen Deposition Impacts on Biodiversity: An Overview , 2014 .