Integration of plasmonic antenna on quantum cascade laser facets for chip-scale molecular sensing

Many important bio-molecules, such as proteins and pharmaceuticals, have their natural resonances in the mid-infrared (2 – 30µm) region of the optical spectrum. The primary challenge of sensing these molecules is to increase the interaction between them and light with such long wavelengths. This can be overcome by exploiting optical nano-antennas which can squeeze the optical mode into a volume much smaller than the operating wavelength. We present a novel antenna design based on hybrid materials composed of a coupled Au-SiO2-Au nanorod integrated on the facet of a quantum cascade laser (QCL) operating in the mid-infrared region of the optical spectrum. FDTD simulations showed that for sandwiched dielectric thicknesses within the range of 20 to 30 nm, peak optical intensity at the top of the antenna ends is 4000 times greater than the incident field intensity. The device was fabricated using focused ion beam milling. Apertureless mid-infrared near field optical microscopy (NSOM) showed that the device can generate a spatially confined spot within a nanometric size about 12 times smaller than the operating wavelength. Such high intensity, hot spot locations can be exploited to enhance the photon interaction for bio-molecules for sensing applications.

[1]  Q. Gong,et al.  Resonances of sandwiched optical antenna , 2008 .

[2]  Nanfang Yu,et al.  Plasmonic Laser Antennas and Related Devices , 2008, IEEE Journal of Selected Topics in Quantum Electronics.

[3]  Garnett W. Bryant,et al.  Optical properties of coupled metallic nanorods for field-enhanced spectroscopy , 2005 .

[4]  E. Palik Handbook of Optical Constants of Solids , 1997 .

[5]  Federico Capasso,et al.  Plasmonic laser antenna , 2006 .

[6]  A. Bonakdar,et al.  Quantum-cascade laser integrated with a metal-dielectric-metal-based plasmonic antenna. , 2010, Optics letters.

[7]  C. Mirkin,et al.  Protein Nanoarrays Generated By Dip-Pen Nanolithography , 2002, Science.

[8]  Javier Alda,et al.  Optical antennas for nano-photonic applications , 2005 .

[9]  Xu,et al.  "Dip-Pen" nanolithography , 1999, Science.

[10]  M. Garcia-Parajo,et al.  Optical antennas focus in on biology , 2008 .

[11]  Qian-jin Wang,et al.  Enhanced optical transmission through metal-dielectric multilayer gratings , 2010 .

[12]  Hooman Mohseni,et al.  Quantum cascade laser integrated with metal-dielectric-metal plasmonic antenna , 2010, Optical Engineering + Applications.

[13]  Nanfang Yu,et al.  Plasmonic Quantum Cascade Laser Antenna , 2007, 2007 Conference on Lasers and Electro-Optics (CLEO).

[14]  Liang Wang,et al.  Design, fabrication, and characterization of nanometer-scale ridged aperture optical antennae , 2006, SPIE LASE.

[15]  James A. Bain,et al.  Imaging of optical field confinement in ridge waveguides fabricated on very-small-aperture laser , 2003 .

[16]  Fritz Keilmann,et al.  Enhanced dielectric contrast in scattering-type scanning near-field optical microscopy , 2000 .

[17]  Manijeh Razeghi,et al.  Quantum cascade lasers that emit more light than heat , 2010 .

[18]  Harald Giessen,et al.  Plasmon Hybridization in Stacked Cut‐Wire Metamaterials , 2007 .

[19]  Scott W. Corzine,et al.  High-temperature continuous wave operation of strain-balanced quantum cascade lasers grown by metal organic vapor-phase epitaxy , 2006 .

[20]  J. Faist,et al.  The Quantum Cascade Laser , 1994 .

[21]  Jacob B. Khurgin,et al.  Highly power-efficient quantum cascade lasers , 2010 .

[22]  P. Nordlander,et al.  A Hybridization Model for the Plasmon Response of Complex Nanostructures , 2003, Science.