Laser-induced jet formation and droplet ejection from thin metal films

An experimental study of femtosecond laser-induced jet formation and droplet ejection from thin metal films is presented. These processes are compared to liquid jet formation during laser-induced forward transfer of viscous liquids. As a result of this comparison, a mechanism explaining the main features of laser processing of thin metal films is proposed. According to this mechanism, laser-induced generation of a molten bump and its collapse are similar to the collapse of cavitation bubbles on a liquid–air interface. Material criteria required for realization of the jetting process are discussed and supported by experimental observations.

[1]  Gerard M. O'Connor,et al.  Nanocrystalline structure of nanobump generated by localized photoexcitation of metal film , 2010 .

[2]  D. Georgiev,et al.  Field-emission properties of sharp high-aspect-ratio gold cones formed via single pulse laser irradiation , 2010 .

[3]  Juergen Koch,et al.  Time-resolved imaging of hydrogel printing via laser-induced forward transfer , 2011 .

[4]  T. Okada,et al.  Nano-Sized Hollow Bump Array Generated by Single Femtosecond Laser Pulse , 2003 .

[5]  A. I. Kuznetsov,et al.  Laser-induced backward transfer of gold nanodroplets. , 2009, Optics express.

[6]  Boris N. Chichkov,et al.  Formation of microbumps and nanojets on gold targets by femtosecond laser pulses , 2004 .

[7]  Alberto Piqué,et al.  Plume and jetting regimes in a laser based forward transfer process as observed by time-resolved optical microscopy , 2002 .

[8]  Yoshiki Nakata,et al.  Effect of pulse width and fluence of femtosecond laser on the size of nanobump array , 2007 .

[9]  Jacobs,et al.  Surface tension of liquid metals: Results from measurements on ground and in space. , 1995, Physical review letters.

[10]  Yoshiki Nakata,et al.  Mesoscopic nanomaterials generated by interfering femtosecond laser processing , 2010 .

[11]  T. Glynn,et al.  The mechanism of nanobump formation in femtosecond pulse laser nanostructuring of thin metal films , 2008 .

[12]  A. I. Kuznetsov,et al.  Laser fabrication of 2D and 3D metal nanoparticle structures and arrays. , 2010, Optics express.

[13]  S. Sauerland,et al.  Surface Tension of Levitated Liquid Noble Metals , 1994 .

[14]  Claudia Unger,et al.  Dispensing pico to nanolitre of a natural hydrogel by laser-assisted bioprinting , 2011, Biomedical engineering online.

[15]  Droplet formation on metallic surfaces during low-fluence laser irradiation , 1996 .

[16]  Leonid V. Zhigilei,et al.  Combined atomistic-continuum modeling of short-pulse laser melting and disintegration of metal films , 2003 .

[17]  Boris N. Chichkov,et al.  Direct-write subwavelength structuring with femtosecond laser pulses , 2005 .

[18]  J. M. Fernández-Pradas,et al.  Time-resolved imaging of the laser forward transfer of liquids , 2009 .

[19]  Nadezhda M. Bulgakova,et al.  Thermoelastic modeling of microbump and nanojet formation on nanosize gold films under femtosecond laser irradiation , 2006 .

[20]  Craig B. Arnold,et al.  Time-resolved study of polyimide absorption layers for blister-actuated laser-induced forward transfer , 2010 .

[21]  R. Reitz,et al.  DROP AND SPRAY FORMATION FROM A LIQUID JET , 1998 .

[22]  D. Ofte The viscosities of liquid uranium, gold and lead , 1967 .

[23]  J. P. Moening Formation of Nano-Sharp Tips and Microbumps on Silicon and Metal Films by Localized Single-Pulse Laser Irradiation , 2010 .

[24]  Zhibin Lin,et al.  Atomistic Modeling of Short Pulse Laser Ablation of Metals: Connections between Melting, Spallation, and Phase Explosion† , 2009 .

[25]  Boris N. Chichkov,et al.  Laser fabrication of large-scale nanoparticle arrays for sensing applications. , 2011, ACS nano.

[26]  L. Chai,et al.  Microdroplet deposition of copper film by femtosecond laser-induced forward transfer , 2006 .

[27]  Boris N. Chichkov,et al.  Nanostructuring of thin gold films by femtosecond lasers , 2009 .

[28]  Yukio Tomita,et al.  Interaction of cavitation bubbles with a free surface , 2001 .

[29]  M. Stuke,et al.  Sub-picosecond UV laser ablation of metals , 1995 .

[30]  D. Georgiev,et al.  Formation of high-aspect-ratio protrusions on gold films by localized pulsed laser irradiation , 2009 .

[31]  Aiko Narazaki,et al.  Nano- and Microdot Array Formation of FeSi2 by Nanosecond Excimer Laser-Induced Forward Transfer , 2008 .

[32]  Ioanna Zergioti,et al.  Nanodroplets deposited in microarrays by femtosecond Ti:sapphire laser-induced forward transfer , 2006 .

[33]  C. Lupis,et al.  The surface tension of liquid silver alloys: Part I. Silver-gold alloys , 1971 .

[34]  B. Chichkov,et al.  Laser-induced transfer of metallic nanodroplets for plasmonics and metamaterial applications , 2009 .

[35]  Yong Huang,et al.  Droplet formation in matrix-assisted pulsed-laser evaporation direct writing of glycerol-water solution , 2009 .

[36]  Boris N. Chichkov,et al.  Nanotexturing of gold films by femtosecond laser-induced melt dynamics , 2005 .

[37]  Computer simulations of laser-induced ejection of droplets , 1998 .

[38]  S. R. Otto,et al.  Bubble interactions near a free surface , 2004 .

[39]  Vicentiu Grosu,et al.  Microdroplet deposition by laser-induced forward transfer , 2005 .

[40]  D. Georgiev,et al.  Focused ion beam and electron microscopy characterization of nanosharp tips and microbumps on silicon and metal thin films formed via localized single-pulse laser irradiation , 2011 .

[41]  P. Leiderer,et al.  Nanostructuring of thin films by ns pulsed laser interference , 2010 .