State-of-the-art assessment of natural gas liquids recovery processes: Techno-economic evaluation, policy implications, open issues, and the way forward

Abstract Although many improved conceptual designs of natural gas liquids (NGLs) recovery processes have been introduced to enhance the economics and efficiency, real-world applications remain elusive because of the communication gap between researchers and practitioners. To bridge this gap, a state-of-the-art assessment of the NGLs recovery processes is presented along with an overall outline considering the feed conditions, product recovery, purity, specific energy consumption (SEC), process economics, and analysis software using the equation of state model. Lower NGL components in the feed have a higher SEC and lower operating costs than a rich feed. It was also found that the conceptual processes are more energy intensive and complex than commercial processes. The major challenges associated with NGL recovery were assessed, including a high energy consumption, varying feed composition, flexibility in the product recovery, and design considerations for offshore NGL processing. Future directions are proposed, including the application of hybrid separation processes and a process intensification to enhance the compactness, particularly for offshore applications, process optimization, and heat integration. Further, an economic policy study is conducted that provides insight into market dynamics. The development of new natural gas (NG) reserves will boost the NGL market and NG business.

[1]  Ana Paula Meneguelo,et al.  Assessment of a process flow diagram for NGL recovery using different condensation mechanisms , 2019, Comput. Chem. Eng..

[2]  Ehsan Barekat-Rezaei,et al.  Thermo–Economical Evaluation of Producing Liquefied Natural Gas and Natural Gas Liquids from Flare Gases , 2018, Energies.

[3]  Eric P. Johnson Process Technologies and Projects for BioLPG , 2019, Energies.

[4]  Kamarul Asri Ibrahim,et al.  Energy Efficient Distillation Columns Design for Retrofit NGLs Fractionation Process , 2015 .

[5]  Qiang Xu,et al.  Optimal design and operation for simultaneous shale gas NGL recovery and LNG re-gasification under uncertainties , 2014 .

[6]  T. Gundersen,et al.  Use of exergy efficiency for the optimization of LNG processes with NGL extraction , 2020, Energy.

[7]  Iftekhar A. Karimi,et al.  Heating Value Reduction of LNG (Liquefied Natural Gas) by Recovering Heavy Hydrocarbons: Technoeconomic Analyses Using Simulation-Based Optimization , 2018 .

[8]  Mehdi Mehrpooya,et al.  Exergy analysis of C2+ recovery plants refrigeration cycles , 2008 .

[9]  Jin-Kuk Kim,et al.  Development of energy-efficient processes for natural gas liquids recovery , 2017 .

[10]  Jiaqiang Jing,et al.  Thermodynamic and economic analysis of ethane recovery processes based on rich gas , 2019, Applied Thermal Engineering.

[11]  Majid Amidpour,et al.  Simulation and optimization of refrigeration cycle in NGL recovery plants with exergy-pinch analysis , 2012 .

[12]  Meng Shi,et al.  Extraction of ethane from natural gas by adsorption on modified ETS-10 , 2011 .

[13]  Muhammad Tahir,et al.  Recent Developments in Natural Gas Flaring Reduction and Reformation to Energy-Efficient Fuels: A Review , 2021 .

[14]  M.F.M. Fahmy,et al.  Optimization and comparative analysis of LNG regasification processes , 2015 .

[15]  Ahmed A. Bhran,et al.  Maximization of natural gas liquids production from an existing gas plant , 2016 .

[16]  Majid Amidpour,et al.  Development and optimization of an integrated process configuration for natural gas liquefaction (LNG) and natural gas liquids (NGL) recovery with a nitrogen rejection unit (NRU) , 2016 .

[18]  Moonyong Lee,et al.  Plant-wide control for the economic operation of modified single mixed refrigerant process for an offshore natural gas liquefaction plant , 2014 .

[19]  Enrico Drioli,et al.  Membrane Gas Separation: A Review/State of the Art , 2009 .

[20]  Inwon Lee,et al.  Alternatives of integrated processes for coproduction of LNG and NGLs recovery , 2016 .

[21]  Jin-Kuk Kim,et al.  Application of exergy analysis for improving energy efficiency of natural gas liquids recovery processes , 2015 .

[22]  Nguyen Van Duc Long,et al.  A novel NGL (natural gas liquid) recovery process based on self-heat recuperation , 2013 .

[23]  Mehdi Mehrpooya,et al.  Optimum design of integrated liquid recovery plants by variable population size genetic algorithm , 2010 .

[24]  Jin-Kuk Kim,et al.  Systematic retrofit design with Response Surface Method and process integration techniques: A case study for the retrofit of a hydrocarbon fractionation plant , 2014 .

[25]  Rachid Chebbi,et al.  Optimizing ethane recovery in turboexpander processes , 2015 .

[26]  Majid Amidpour,et al.  Exergoeconomic analysis of integrated natural gas liquids (NGL) and liquefied natural gas (LNG) processes , 2017 .

[27]  Mahmoud Omid,et al.  Optimum Thermal Concentration of Solar Thermoelectric Generators (STEG) in Realistic Meteorological Condition , 2018, Energies.

[28]  Yajun Li,et al.  Cost-effective optimization design of light hydrocarbon recovery process based on exergy analysis , 2019 .

[29]  Mehdi Mehrpooya,et al.  A novel process configuration for co-production of NGL and LNG with low energy requirement , 2013 .

[30]  Mehdi Mehrpooya,et al.  A novel process configuration for hydrocarbon recovery process with auto–refrigeration system , 2017 .

[31]  W. Luyben NGL Demethanizer Control , 2013 .

[32]  Jiaqiang Jing,et al.  Optimization and Exergy Analysis of Natural Gas Liquid Recovery Processes for the Maximization of Plant Profits , 2018, Chemical Engineering & Technology.

[33]  Minbo Yang,et al.  A systematic simulation-based process intensification method for shale gas processing and NGLs recovery process systems under uncertain feedstock compositions , 2017, Comput. Chem. Eng..

[34]  Jian Zhang,et al.  A novel conceptual design by integrating NGL recovery and LNG regasification processes for maximum energy savings , 2013 .

[35]  Alireza Bahadori,et al.  Risk-based optimization for representative natural gas liquid (NGL) recovery processes by considering uncertainty from the plant inlet , 2015 .

[36]  K. Peinemann,et al.  Membranes for separation of higher hydrocarbons from methane , 1996 .

[37]  Saad A. Al-Sobhi,et al.  Potential energy savings and greenhouse gases (GHGs) emissions reduction strategy for natural gas liquid (NGL) recovery: Process simulation and economic evaluation , 2018, Journal of Cleaner Production.

[38]  Jim Lee,et al.  A Comparative Study of Natural Gas Liquids Recovery Methods , 2012 .

[39]  Alireza Bahadori,et al.  Techno-economic evaluation of a novel NGL recovery scheme with nine patented schemes for offshore applications , 2015 .

[40]  Miguel Menéndez,et al.  Separation of hydrocarbons from natural gas using silicalite membranes , 2001 .

[41]  Mamdouh Gadalla,et al.  Integrated Process Development for an Optimum Gas Processing Plant , 2017 .

[42]  Membranes for Gas Separation Current Development and Challenges , 2015 .

[43]  Davide Fissore,et al.  Simulation and energy consumption analysis of a propane plus recovery plant from natural gas , 2011 .

[44]  Kun Huang,et al.  Techno-Economic Comparison and Analysis of a Novel NGL Recovery Scheme with Three Patented Schemes , 2017 .

[45]  Majid Amidpour,et al.  Implementing absorption refrigeration cycle in lieu of DMR and C3MR cycles in the integrated NGL, LNG and NRU unit , 2017 .

[46]  Jin-Kuk Kim,et al.  Process Design of Natural Gas Liquid Recovery Processes , 2013 .

[47]  Jose A. Romagnoli,et al.  Operation optimization of a cryogenic NGL recovery unit using deep learning based surrogate modeling , 2020, Comput. Chem. Eng..

[48]  Kyu Suk Hwang,et al.  Design process of LNG heavy hydrocarbons fractionation: Low LNG temperature recovery , 2014 .

[49]  M. El‐Halwagi,et al.  Optimal Selection of Shale Gas Processing and NGL Recovery Plant from Multiperiod Simulation , 2020 .

[50]  Shahram Tahmasebi,et al.  Investigation of various feed conditions on NGL recovery plant energy and exergy performance: A case study , 2015 .

[51]  Mehdi Mehrpooya,et al.  Energy and advanced exergy analysis of an existing hydrocarbon recovery process , 2016 .

[52]  Mehdi Mehrpooya,et al.  Introducing a new parameter for evaluating the degree of integration in cryogenic liquid recovery processes , 2011 .

[53]  Stanley H. Huang,et al.  Experimental studies of hydrocarbon separation on zeolites, activated carbons and MOFs for applications in natural gas processing , 2017 .

[54]  Yajun Li,et al.  System optimization of turbo-expander process for natural gas liquid recovery , 2017 .

[55]  Muhammad Abdul Qyyum,et al.  Nitrogen self-recuperation expansion-based process for offshore coproduction of liquefied natural gas, liquefied petroleum gas, and pentane plus , 2019, Applied Energy.

[56]  Liang Yu,et al.  Ultra-thin MFI membranes for removal of C3+ hydrocarbons from methane , 2018 .

[57]  Ting Gao,et al.  Improved processes of light hydrocarbon separation from LNG with its cryogenic energy utilized , 2011 .

[58]  Mehdi Mehrpooya,et al.  Evaluation of novel process configurations for coproduction of LNG and NGL using advanced exergoeconomic analysis , 2017 .

[59]  Ghaleb A. Husseini,et al.  Optimum ethane recovery in conventional turboexpander process , 2010 .

[61]  Mohd Shariq Khan,et al.  Energy saving opportunities in integrated NGL/LNG schemes exploiting: Thermal-coupling common-utilities and process knowledge , 2014 .

[62]  Mehdi Mehrpooya,et al.  A comprehensive approach toward utilizing mixed refrigerant and absorption refrigeration systems in an integrated cryogenic refrigeration process , 2018 .

[63]  Dong-Yeon Lee,et al.  By-product hydrogen from steam cracking of natural gas liquids (NGLs): Potential for large-scale hydrogen fuel production, life-cycle air emissions reduction, and economic benefit , 2018, International Journal of Hydrogen Energy.

[64]  S. Semenova Polymer membranes for hydrocarbon separation and removal , 2004 .

[65]  S. Deng,et al.  Adsorption of ethane, ethylene, propane, and propylene on a magnesium-based metal-organic framework. , 2011, Langmuir : the ACS journal of surfaces and colloids.

[66]  M. Mehrpooya,et al.  Novel LNG-Based Integrated Process Configuration Alternatives for Coproduction of LNG and NGL , 2014 .

[67]  M. Mehrpooya,et al.  A novel energy efficient LNG/NGL recovery process using absorption and mixed refrigerant refrigeration cycles – Economic and exergy analyses , 2018 .

[68]  Mehdi Mehrpooya,et al.  Introducing a novel integrated NGL recovery process configuration (with a self-refrigeration system (open–closed cycle)) with minimum energy requirement , 2010 .

[69]  Yonglin Ju,et al.  Design and Optimization of a Novel Mixed Refrigerant Cycle Integrated with NGL Recovery Process for Small-Scale LNG Plant , 2014 .

[70]  Z. Xin,et al.  Structure effect of benzofuranone on the anti‐oxidation kinetics in polypropylene , 2012 .

[71]  Seyyed Hossein Hosseini,et al.  An increased production capacity by a retrofitted industrial deethanizer column , 2016 .

[72]  Yu Qian,et al.  A Novel Process for Natural Gas Liquids Recovery from Oil Field Associated Gas with Liquefied Natural Gas Cryogenic Energy Utilization , 2011 .

[73]  Nguyen Van Duc Long,et al.  Novel retrofit designs using a modified coordinate descent methodology for improving energy efficiency of natural gas liquid fractionation process , 2016 .

[75]  Nguyen Van Duc Long,et al.  Techno-economic analysis of potential natural gas liquid (NGL) recovery processes under variations of feed compositions , 2013 .

[76]  W. Luyben Effect of Natural Gas Composition on the Design of Natural Gas Liquid Demethanizers , 2013 .

[77]  Youngsub Lim,et al.  Economic evaluation of NGL recovery process schemes for lean feed compositions , 2018 .

[78]  Dietrich M Gross,et al.  Experimental investigation of an adsorptive thermal energy storage , 2007 .

[79]  Mehdi Mehrpooya,et al.  An Optimization of Capital and Operating Alternatives in a NGL Recovery Unit , 2006 .