Establishment of a Confined Swirling Natural Gas/Air Flame as a Standard Flame: Temperature and Species Distributions from Laser Raman Measurements

A prototype of an industrial burner for confined swirling natural gas diffusion flames with thermal powers in the range of 100 to 300 kW is presented. Within the TECFLAM research cooperation, a well-defined "standard flame" was investigated in this burner with complementary measuring techniques to yield a comprehensive characterization of the combustion process. The aims of the investigations were a better understanding of the complex physical and chemical processes, their interactions in turbulent swirling flames, and the establishment of a database that can be used as a test case for numerical simulations. The results from single-pulse Raman measurements of the temperature, mixture fraction, and major species concentrations are presented. The global flame behavior is illustrated by the spatial distributions of the mean values and fluctuations of the temperature and mixture fraction. The different flame regions and their characteristic features are discussed. The main objective is the investigation of finite-rate chemistry effects, which can be deduced from the correlations between the various simultaneously measured quantities (scatterplots). Within the shear layers and the region of flame reactions, large deviations from chemical equilibrium are observed, which can be attributed to local flame extinction and ignition delay. Further discussion points are the stabilization mechanism of the flame and the influence of turbulent mixing on the thermochemical state. Finally, the effect of increased swirl on the flame behavior is illustrated and discussed.

[1]  Volker Beushausen,et al.  Spatially resolved Raman scattering for multi-species and temperature analysis in technically applied combustion systems: Spray flame and four-cylinder in-line engine , 1994 .

[2]  Rainer Koch,et al.  Validation of Numerical Methods at a Confined Turbulent Natural Gas Diffusion Flame Considering Detailed Radiative Transfer , 1998 .

[3]  F. Takahashi,et al.  Structure of Turbulent Hydrogen Jet Diffusion Flames With or Without Swirl , 1996 .

[4]  Wolfgang Leuckel,et al.  Turbulent swirling flames: Experimental investigation of the flow field and formation of nitrogen oxide , 2000 .

[5]  Normand M. Laurendeau,et al.  Comparison of laser-induced and planar laser-induced fluorescence measurements of nitric oxide in a high-pressure, swirl-stabilized, spray flame , 2000 .

[6]  P. Andresen,et al.  Quantitative one-dimensional single-pulse multi-species concentration and temperature measurement in the lift-off region of a turbulent H2/air diffusion flame , 1995 .

[7]  M. Long,et al.  Three-scalar imaging in turbulent non-premixed flames of methane , 1998 .

[8]  W. Meier,et al.  Laser Raman scattering in fuel-rich flames: background levels at different excitation wavelengths , 2002 .

[9]  James F. Driscoll,et al.  Effect of Heat Release and Swirl on the Recirculation within Swirl-Stabilized Flames , 1985 .

[10]  Winfried Stricker,et al.  Investigations in the TECFLAM swirling diffusion flame: Laser Raman measurements and CFD calculations , 2000 .

[11]  Study of swirling recirculating hydrogen diffusion flame using UV Raman spectroscopy , 1996 .

[12]  R. Pitz,et al.  Raman scattering measurements in flames using a tunable KrF excimer laser. , 1992, Applied optics.

[13]  Ruey-Hung Chen Some Characteristics of NOx Emission of Turbulent Nonpremixed Hydrogen-Air Flames Stabilized by Swirl-Generated Flow Recirculation , 1995 .

[14]  Robert W. Bilger,et al.  The structure of turbulent nonpremixed flames , 1989 .

[15]  R. Barlow,et al.  Some raman/rayleigh/lif measurements in turbulent propane flames , 1991 .

[16]  M. Mansour,et al.  Measurements of Scalar Dissipation in Turbulent Hydrogen Diffusion Flames and Some Implications on Combustion Modeling , 1997 .

[17]  Winfried Stricker,et al.  Application of spontaneous Raman and Rayleigh scattering and 2D LIF for the characterization of a turbulent CH4/H2/N2 jet diffusion flame , 1998 .

[18]  János M. Beér,et al.  Combustion in swirling flows: A review , 1974 .

[19]  One-dimensional raman scattering for determination of multipoint joint scalar probability density functions in turbulent diffusion flames , 1998 .

[20]  W. Meier,et al.  Characterization of Turbulent hytVAir Jet Diffusion Flames by Single-Pulse Spontaneous Raman Scattering , 1996 .

[21]  A. Leipertz,et al.  One-Dimensional, Time-Resolved Raman Measurements in a Sooting Flame made with 355-nm Excitation. , 1998, Applied optics.

[22]  W. Meier,et al.  A flat flame burner as calibration source for combustion research: Temperatures and species concentrations of premixed H2/air flames , 1994 .

[23]  Finite rate chemistry and NO molefraction in non-premixed turbulent flames , 1998 .

[24]  T. O’Doherty,et al.  Vortex breakdown: a review , 2001 .

[25]  Wolfgang Leuckel,et al.  Swirl-induced intermittency: A novel effect modifying the turbulence structure of swirling free jets , 1996 .

[26]  H. Eickhoff,et al.  Experimental and numerical study concerning stabilization of strongly swirling premixed and nonpremixed flames , 1992 .

[27]  S. Turns,et al.  Measurement and prediction of NOx emissions from unconfined propane flames from turbulent-jet, bluff-body, swirl and precessing jet burners , 2000 .

[28]  S. Pope,et al.  Raman measurements and joint PDF modeling of a nonpremixed bluff-body-stabilized methane flame , 1994 .

[29]  Y. Chao,et al.  Effects of fuel-air mixing on flame structures and NOx emissions in swirling methane jet flames , 1998 .

[30]  R. Pitz,et al.  Intermittency and Conditional Averaging in a Turbulent Nonpremixed Flame by Raman Scattering , 1984 .

[31]  David L. Warren,et al.  Turbulent velocity and temperature measurements from a gas-fueled technology combustor with a practical fuel injector , 1995 .

[32]  R. Barlow,et al.  The structure of turbulent nonpremixed flames revealed by Raman-Rayleigh-LIF measurements , 1996 .

[33]  Jürgen Wolfrum,et al.  Simultaneous single-shot laser-based imaging of formaldehyde, OH, and temperature in turbulent flames , 2000 .

[34]  F. Beretta,et al.  Ultraviolet and visible fluorescence in the fuel pyrolysis regions of gaseous diffusion flames , 1985 .

[35]  David G. Lilley,et al.  Swirl Flows in Combustion: A Review , 1977 .

[36]  C. Schulz,et al.  Laser-diagnostic multi-species imaging in strongly swirling natural gas flames , 2000 .

[37]  A. Eckbreth Laser Diagnostics for Combustion Temperature and Species , 1988 .