Measuring non-volatile particles properties in the exhaust of an aircraft engine

The steady growth of air traffic and its foreseen expansion during future years have raised concerns about its potential impact on climate and ground-level air quality. So far, the smoke number has been used to evaluate the non-volatile particulate matter amount emitted by aircraft engines, but it is a poor proxy for modern engine emissions. Therefore, new sampling and measurement techniques have recently been tested on aircraft engine emissions, especially as a new ICAO particle emission standard is currently being developed. Number and mass of emitted particles are generally used, but are not sufficient to fully characterize soot emissions and further address atmospheric impact issues. Chemical composition is crucial to evaluate their atmospheric reactivity. This paper presents a complete set of techniques that have been used to characterize soot emissions from an aircraft engine in a comprehensive manner. It reports results from a campaign on a PowerJet SaM146 engine, performed within the framework of the MERMOSE (Mesure et Etude de la Reactivite des emissions de MOteurS aEronautiques) project. It emphasizes the influence of the engine regime, ranging from 30% to 100% of the takeoff thrust, on the various particle properties investigated, including the size, number, morphology and chemical composition.

[1]  John S. Kinsey,et al.  Physical characterization of the fine particle emissions from commercial aircraft engines during the Aircraft Particle Emissions eXperiment (APEX) 1–3 , 2010 .

[2]  The Effect of Altitude Conditions on the Particle Emissions of a J85-GE-5L Turbojet Engine , 1995 .

[4]  Reinhard Niessner,et al.  Raman microspectroscopy of soot and related carbonaceous materials: Spectral analysis and structural information , 2005 .

[5]  A. Ishitani,et al.  Raman spectra of graphite edge planes , 1988 .

[6]  Zhenhong Yu,et al.  Identification of lubrication oil in the particulate matter emissions from engine exhaust of in-service commercial aircraft. , 2012, Environmental science & technology.

[7]  P. Salatino,et al.  Evolution of Reactivity of Highly Porous Chars from Raman Microscopy , 2000 .

[8]  G. G. Stokes "J." , 1890, The New Yale Book of Quotations.

[9]  P ? ? ? ? ? ? ? % ? ? ? ? , 1991 .

[10]  David S. Lee,et al.  Transport impacts on atmosphere and climate: Aviation , 2009, Atmospheric Environment.

[11]  Bernd Kärcher,et al.  Carbonaceous aerosol in jet engine exhaust: emission characteristics and implications for heterogeneous chemical reactions , 1999 .

[12]  R.T. Brown,et al.  Topics in applied physics , 1980, Proceedings of the IEEE.

[13]  J. Rouzaud,et al.  Raman microspectroscopy characterization of carbon blacks: Spectral analysis and structural information , 2015 .

[14]  J. Heintzenberg,et al.  NIR FT Raman spectroscopic study of flame soot , 1999 .