Sampling-time effects for persistence and survival in step structural fluctuations.

The effects of sampling rate and total measurement time have been determined for single-point measurements of step fluctuations within the context of first-passage properties. Time dependent scanning tunneling microscopy has been used to evaluate step fluctuations on Ag(111) films grown on mica as a function of temperature (300-410 K) , on screw dislocations on the facets of Pb crystallites at 320 K , and on Al-terminated Si(111) over the temperature range 770-970 K . Although the fundamental time constant for step fluctuations on Ag and Al/Si varies by orders of magnitude over the temperature ranges of measurement, no dependence of the persistence amplitude on temperature is observed. Instead, the persistence probability is found to scale directly with t/delta t where delta t is the time interval used for sampling. Survival probabilities show a more complex scaling dependence, which includes both the sampling interval and the total measurement time t(m) . Scaling with t/delta t occurs only when delta t/ t(m) is a constant. We show that this observation is equivalent to theoretical predictions that the survival probability will scale as delta t/ L(z) , where L is the effective length of a step. This implies that the survival probability for large systems, when measured with fixed values of t(m) or delta t , should also show little or no temperature dependence.

[1]  E. Williams Nanoscale Structures: Lability, Length Scales, and Fluctuations , 2004 .

[2]  T. Einstein,et al.  Distinguishing step relaxation mechanisms via pair correlation functions , 2004, cond-mat/0408463.

[3]  O. Bondarchuk,et al.  Correlation time for step structural fluctuations , 2004, cond-mat/0408181.

[4]  E. Williams,et al.  Triggered fast relaxation of metastable Pb crystallites , 2004 .

[5]  S. Majumdar,et al.  Persistence in nonequilibrium surface growth. , 2004, Physical review. E, Statistical, nonlinear, and soft matter physics.

[6]  S. Ciliberto,et al.  Power and heat fluctuation theorems for electric circuits. , 2003, Physical review letters.

[7]  S. Majumdar,et al.  Survival in equilibrium step fluctuations. , 2003, Physical review. E, Statistical, nonlinear, and soft matter physics.

[8]  O. Bondarchuk,et al.  Infinite family of persistence exponents for interface fluctuations. , 2003, Physical review letters.

[9]  O. Bondarchuk,et al.  Persistence exponents for step edge diffusion , 2003 .

[10]  T. Einstein Crossover between terrace-diffusion and diffusion step-to-step on vicinal surfaces: scaling function and analytic approximations , 2002 .

[11]  T. Einstein,et al.  Dynamics of step fluctuations on a chemically heterogeneous surface of Al/Si(111)-(√3×√3) , 2002 .

[12]  E. Williams,et al.  Experimental persistence probability for fluctuating steps. , 2002, Physical review letters.

[13]  R. Zia,et al.  Watching a drunkard for 10 nights: A study of distributions of variances , 2002, cond-mat/0209044.

[14]  S. Majumdar,et al.  Persistence of a continuous stochastic process with discrete-time sampling: non-Markov processes. , 2001, Physical review. E, Statistical, nonlinear, and soft matter physics.

[15]  T. Einstein,et al.  Step wandering on Al/Si(1 1 1)-(√3×√3) surface at high temperatures , 2001 .

[16]  S. Redner A guide to first-passage processes , 2001 .

[17]  M. Giesen Step and island dynamics at solid/vacuum and solid/liquid interfaces , 2001 .

[18]  Sidney Redner,et al.  A guide to first-passage processes , 2001 .

[19]  E. Williams,et al.  Continuous and discontinuous transitions on 3D equilibrium crystal shapes : a new look at Pb and Au , 2001 .

[20]  B. Hammer,et al.  Kinetics of fast island decay on Ag(111) , 2001 .

[21]  S. Majumdar,et al.  Persistence of a continuous stochastic process with discrete-time sampling. , 2000, Physical review. E, Statistical, nonlinear, and soft matter physics.

[22]  Z. Toroczkai,et al.  Nanoscale Fluctuations at Solid Surfaces , 1999 .

[23]  Ellen D. Williams,et al.  Steps on surfaces: experiment and theory , 1999 .

[24]  P. Wynblatt,et al.  Step energetics of Pb(111) vicinal surfaces from facet shape , 1999 .

[25]  Thomas Ihle,et al.  EQUILIBRIUM STEP DYNAMICS ON VICINAL SURFACES REVISITED , 1998 .

[26]  T. Einstein,et al.  Unified view of step-edge kinetics and fluctuations , 1998 .

[27]  S. Majumdar,et al.  Persistence exponents for fluctuating interfaces , 1997, cond-mat/9704238.

[28]  Kuipers,et al.  Step and kink dynamics on Au(110) and Pb(111) studied with a high-speed STM. , 1995, Physical review. B, Condensed matter.

[29]  Rosenfeld,et al.  Brownian motion of vacancy islands on Ag(111). , 1995, Physical review letters.

[30]  Evans,et al.  Diffusion of large two-dimensional Ag clusters on Ag(100). , 1994, Physical review letters.

[31]  J. L. Goldberg,et al.  The equilibration of terrace width distributions on stepped surfaces , 1992 .