Electrodynamic mechanism and array stability in optical binding

Addressing optically induced interactions between nanoparticles, new results from quantum electrodynamical studies are employed to produce surfaces representing the variation of potential energy with the various geometric degrees of freedom - the positions and orientations of each particle relative to each other, and to the throughput radiation. The results take the form of energy landscapes exhibiting highly detailed topographic features. The analysis of these features facilitates the determination of possible stability points associated with optical binding, and the identification of other, anisotropic features revealing the operation of local forces and torques. Extending previous theory, the present study gives results for both polarized and non-polarized light, also providing a critical analysis of the significance of multipole interactions. It is shown that the pair potential provides a prototypical template for the optical assembly of larger numbers of particles, and a discussion is given of the possibilities to optically fabricate structures using polarized or non-polarized laser beams. The results are applicable to optically trapped molecules, nanoparticles, microparticles, colloids, etc.

[1]  D. S. Bradshaw,et al.  Laser-induced forces between carbon nanotubes. , 2005, Optics letters.

[2]  D. S. Bradshaw,et al.  Interactions between spherical nanoparticles optically trapped in Laguerre-Gaussian modes. , 2005, Optics letters.

[3]  D. S. Bradshaw,et al.  Erratum: Optically induced forces and torques: Interactions between nanoparticles in a laser beam [Phys. Rev. A 72 , 033816 (2005)] , 2006 .

[4]  K Dholakia,et al.  Optically bound microscopic particles in one dimension. , 2004, Physical review. E, Statistical, nonlinear, and soft matter physics.

[5]  M Mazilu,et al.  Measurement of the restoring forces acting on two optically bound particles from normal mode correlations. , 2007, Physical review letters.

[6]  D. Blom,et al.  Laser-induced nanoparticle ordering , 2002 .

[7]  T. Thirunamachandran,et al.  Molecular Quantum Electrodynamics , 1984 .

[8]  Johann Rohner,et al.  Building optical matter with binding and trapping forces , 2004, SPIE Optics + Photonics.

[9]  D. S. Bradshaw,et al.  Resonance energy transfer: The unified theory revisited , 2003 .

[10]  A. Ashkin Acceleration and trapping of particles by radiation pressure , 1970 .

[11]  D. Andrews,et al.  Optically induced potential energy landscapes , 2007 .

[12]  D. S. Bradshaw,et al.  Optically induced forces and torques: Interactions between nanoparticles in a laser beam , 2005 .

[13]  D. Andrews Two-group Raman optical activity revisited , 1994 .

[14]  K. Dholakia,et al.  One-dimensional optically bound arrays of microscopic particles. , 2002, Physical review letters.

[15]  D. S. Bradshaw,et al.  Optically induced inter-particle forces: from the bonding of dimers to optical electrostriction in molecular solids , 2006 .

[16]  A. Salam Intermolecular interactions in a radiation field via the method of induced moments , 2006 .

[17]  Wolfgang Singer,et al.  Self-organized array of regularly spaced microbeads in a fiber-optical trap , 2003 .

[18]  J. Golovchenko,et al.  Optical Matter: Crystallization and Binding in Intense Optical Fields , 1990, Science.

[19]  G. Scholes,et al.  Damping and higher multipole effects in the quantum electrodynamical model for electronic energy transfer in the condensed phase , 1997 .

[20]  S. Chu,et al.  Observation of a single-beam gradient force optical trap for dielectric particles. , 1986, Optics letters.

[21]  D. Andrews,et al.  Optical Harmonics in Molecular Systems: Quantum Electrodynamical Theory , 2002 .

[22]  D. Andrews,et al.  Phased and Boltzmann-weighted rotational averages , 1984 .