Active Optically Controlled Broadband Terahertz Modulator Based on Fe3O4 Nanoparticles

We report an active broadband terahertz (THz) modulator based on an Fe3O4 nanoparticle/silicon (Si) structure, where the interface effects were measured in a homemade THz time-domain spectroscopy system. An approximately 100-nm Fe3O4 nanoparticle thin film on the high-resistance Si substrate was easily attained by spin-coating ferrofluids. In our experiment, a modulation depth as high as 92% was achieved at an external laser irradiance of 3.6 W/cm2. This result can be explained by the accumulation of carriers at the interface of the hybrid structure, which induces intense absorption of the THz transmission. In addition, the limit modulated frequency of the device is ∼12 kHz. The superior performance of this device for THz wave modulation in comparison to other nanomaterial-based THz modulators and the ease of fabrication both illustrate that this is a promising method in the modulation of THz transmission. Furthermore, this modulator could also potentially provide an essential component in a wide variety of technologies, such as THz communications, THz imaging, etc.

[1]  J C Cao Interband impact ionization and nonlinear absorption of terahertz radiation in semiconductor heterostructures. , 2003, Physical review letters.

[2]  Hui Yan,et al.  Electrical transport, magnetic properties of the half-metallic Fe3O4-based Schottky diode , 2009 .

[3]  Zhenxiang Cheng,et al.  Terahertz broadband modulation in a biased BiFeO3/Si heterojunction. , 2016, Optics express.

[4]  A. Davies,et al.  Terahertz spectroscopy of explosives and drugs , 2008 .

[5]  Kai Liu,et al.  Recent advances in terahertz technology for biomedical applications. , 2017, Quantitative imaging in medicine and surgery.

[6]  Electronic structure of half-metallic magnets , 2006, cond-mat/0611476.

[7]  Bo Zhang,et al.  Conjugated polymer-based broadband terahertz wave modulator. , 2014, Optics letters.

[8]  R. Morandotti,et al.  Terahertz magnetic modulator based on magnetically clustered nanoparticles , 2014, 1409.4963.

[9]  Bo Liu,et al.  Magnetically tunable terahertz magnetoplasmons in ferrofluid-filled photonic crystals , 2013 .

[10]  Jing-ling Shen,et al.  Conjugated polymer based active electric-controlled terahertz device , 2016, 2016 41st International Conference on Infrared, Millimeter, and Terahertz waves (IRMMW-THz).

[11]  B. Zhang,et al.  Photo-excited terahertz switch based on composite metamaterial structure , 2016 .

[12]  Zhenxiang Cheng,et al.  Thermodynamics of quasi-2D electron gas at BFO/Si interface probed with THz time-domain spectroscopy , 2017 .

[13]  Yufeng Hu,et al.  High-efficiency THz modulator based on phthalocyanine-compound organic films , 2015 .

[14]  Zhiyong Zhong,et al.  Enhanced Optical Modulation Depth of Terahertz Waves by Self‐Assembled Monolayer of Plasmonic Gold Nanoparticles , 2016 .

[15]  Bo Zhang,et al.  Monolayer graphene based organic optical terahertz modulator , 2017 .

[16]  H. V. Thakur,et al.  Photonic crystal fiber injected with Fe3O4 nanofluid for magnetic field detection , 2011 .

[17]  B. Zhang,et al.  High efficiency THz-wave modulators based on conjugated polymer-based organic films , 2016 .

[18]  Zhen Tian,et al.  Active graphene–silicon hybrid diode for terahertz waves , 2015, Nature Communications.

[19]  Hao Zhang,et al.  Temperature tunability of photonic crystal fiber filled with Fe3O4 nanoparticle fluid , 2011 .

[20]  Ghanshyam Singh,et al.  Terahertz planar antennas for future wireless communication: A technical review , 2013 .

[21]  Beatriz Pelaz,et al.  Enhanced All-Optical Modulation of Terahertz Waves on the Basis of Manganese Ferrite Nanoparticles , 2017 .

[22]  L. D. Negro,et al.  Optical gain in silicon nanocrystals , 2000, Nature.

[23]  Xin Liu,et al.  Active terahertz wave modulator based on molybdenum disulfide , 2017 .

[24]  Zhang Xi,et al.  Materials for terahertz science and technology , 2003 .

[25]  Makoto Nakajima,et al.  Efficient optical terahertz-transmission modulation in solution-processable organic semiconductor thin films on silicon substrate , 2016 .