Control of interannual and longer‐term variability of stratospheric water vapor

[1] We use trajectory calculations based on 40-year European Reanalysis (ERA-40) data to predict the water mixing ratio of air entering the stratosphere in the tropics ([H2O]e) and thereby to examine interannual and longer-term changes. [H2O]e is determined from the saturation mixing ratio of the coldest point during ascent from the troposphere to the stratosphere (the Lagrangian cold point). These model predictions for the time variation of [H2O]e agree very well with a broad range of measurements (Stratospheric Aerosol and Gas Experiment (SAGE) II, Halogen Occultation Experiment (HALOE), Microwave Limb Sounder (MLS), and Atmospheric Trace Molecule Spectroscopy (ATMOS)). During periods when measurements are consistent among various sensors and ERA-40 temperatures show good agreement with radiosondes (1995–2002), the correlation between model predictions and HALOE water vapor anomalies in the tropical lower stratosphere is r = 0.81, as high as that between HALOE and SAGE II (r = 0.8). The model predictions suggest that the stratospheric quasi-biennial oscillation, El Nino–Southern Oscillation, and possibly volcanic eruptions all play a significant role in modulating [H2O]e, leading to interannual anomalies of order 0.5 ppmv with timescales of several months to years. Although the Lagrangian calculations show substantial interannual variability of transport pathways into the stratosphere, the results show that the interannual anomalies of [H2O]e are dominated by anomalies of the zonal mean temperature rather than by transport changes or localized temperature anomalies. This reinforces the paradox of apparently increasing stratospheric water vapor concentrations alongside, if anything, slightly decreasing temperatures at the tropical tropopause. The combination of measurement uncertainties and relatively strong interannual variability with periods of several months to years, on the one hand, limits our ability to detect, attribute, and verify long-term trends and, on the other hand, raises the question as to whether the previously published estimates of long-term trends are too large.

[1]  S. Fueglistaler,et al.  Stratospheric water vapor predicted from the Lagrangian temperature history of air entering the stratosphere in the tropics , 2005 .

[2]  D. Weisenstein,et al.  Influence of tropospheric SO2 emissions on particle formation and the stratospheric humidity , 2005 .

[3]  S. Fueglistaler,et al.  Control of Stratospheric Water Vapor , 2004 .

[4]  P. Haynes,et al.  A trajectory‐based study of the tropical tropopause region , 2004 .

[5]  Fei Wu,et al.  Interannual changes of stratospheric water vapor and correlations with tropical tropopause temperatures , 2004 .

[6]  J. Zawodny,et al.  A revised water vapor product for the Stratospheric Aerosol and Gas Experiment (SAGE) II version 6.2 data set , 2004 .

[7]  William G. Read,et al.  A new 147–56 hPa water vapor product from the UARS Microwave Limb Sounder , 2004 .

[8]  H. Wernli,et al.  Tropical troposphere‐to‐stratosphere transport inferred from trajectory calculations , 2004 .

[9]  A. Simmons Representation of the stratosphere in ECMWF operations and ERA-40 , 2004 .

[10]  B. Soden,et al.  WATER VAPOR FEEDBACK AND GLOBAL WARMING 1 , 2003 .

[11]  H. Hatsushika,et al.  Stratospheric drain over Indonesia and dehydration within the tropical tropopause layer diagnosed by air parcel trajectories , 2003 .

[12]  Adam A. Scaife,et al.  Can changes in ENSO activity help to explain increasing stratospheric water vapor? , 2003 .

[13]  S. Klein,et al.  Temporal Homogenization of Monthly Radiosonde Temperature Data. Part II: Trends, Sensitivities, and MSU Comparison. , 2003 .

[14]  D. Waugh,et al.  AGE OF STRATOSPHERIC AIR: THEORY, OBSERVATIONS, AND MODELS , 2002 .

[15]  K. Rosenlof Transport Changes Inferred from HALOE Water and Methane Measurements , 2002 .

[16]  Minghua Zhang,et al.  Simulations of the Interannual Variability of Stratospheric Water Vapor , 2002 .

[17]  P. Forster,et al.  Assessing the climate impact of trends in stratospheric water vapor , 2002 .

[18]  S. Sherwood A Microphysical Connection Among Biomass Burning, Cumulus Clouds, and Stratospheric Moisture , 2002, Science.

[19]  J. Russell,et al.  El niño as a natural experiment for studying the tropical tropopause region , 2001 .

[20]  A. Gettelman,et al.  Horizontal transport and the dehydration of the stratosphere , 2001 .

[21]  Kevin Hamilton,et al.  The quasi‐biennial oscillation , 2001 .

[22]  D. Seidel,et al.  Climatological characteristics of the tropical tropopause as revealed by radiosondes , 2001 .

[23]  S. Solomon,et al.  Response of the stratospheric temperatures and ozone to past and future increases in stratospheric humidity , 2001 .

[24]  M. McCormick,et al.  Stratospheric water vapor increases over the past half‐century , 2001 .

[25]  Minghua Zhang,et al.  Cooling trend of the tropical cold point tropopause temperatures and its implications , 2001 .

[26]  S. Oltmans,et al.  The increase in stratospheric water vapor from balloonborne, frostpoint hygrometer measurements at Washington, D.C., and Boulder, Colorado , 2000 .

[27]  G. Toon,et al.  Features and trends in Atmospheric Trace Molecule Spectroscopy (ATMOS) version 3 stratospheric water vapor and methane measurements , 2000 .

[28]  S. Sherwood,et al.  On the control of stratospheric humidity , 2000 .

[29]  James M. Russell,et al.  SPARC assessment of upper tropospheric and stratospheric water vapour , 2000 .

[30]  L. Bengtsson,et al.  Potential role of the quasi-biennial oscillation in the stratosphere-troposphere exchange as found in water vapor in general circulation model experiments , 1999 .

[31]  Richard Swinbank,et al.  Global QBO Circulation Derived from UKMO Stratospheric Analyses , 1999 .

[32]  D. McKenna,et al.  Balloon‐borne in situ measurements of stratospheric H2O, CH4 and H2 at midlatitudes , 1999 .

[33]  E. J. Dlugokencky,et al.  Continuing decline in the growth rate of the atmospheric methane burden , 1998, Nature.

[34]  J. Russell,et al.  Trends in stratospheric humidity and the sensitivity of ozone to these trends , 1998 .

[35]  James M. Russell,et al.  Seasonal Cycles and QBO Variations in Stratospheric CH4 and H2O Observed in UARS HALOE Data , 1998 .

[36]  S. Pawson,et al.  The Descent Rates of the Shear Zones of the Equatorial QBO , 1996 .

[37]  J. Holton,et al.  Stratosphere‐troposphere exchange , 1995 .

[38]  D. Wuebbles,et al.  The chemical and radiative effects of the Mount Pinatubo eruption , 1994 .

[39]  James M. Russell,et al.  The Halogen Occultation Experiment , 1993 .

[40]  E. Danielsen In situ evidence of rapid, vertical, irreversible transport of lower tropospheric air into the lower tropical stratosphere by convective cloud turrets and by larger-scale upwelling in tropical cyclones , 1993 .

[41]  D. Etheridge,et al.  Changes in tropospheric methane between 1841 and 1978 from a high accumulation‐rate Antarctic ice core , 1992 .

[42]  Arlin J. Krueger,et al.  Global tracking of the SO2 clouds from the June , 1992 .

[43]  J. Holton On the Global Exchange of Mass between the Stratosphere and Troposphere , 1990 .

[44]  R. Garcia,et al.  The role of molecular hydrogen and methane oxidation in the water vapour budget of the stratosphere , 1988 .

[45]  R. Newell,et al.  A Stratospheric Fountain , 1981 .