Generic incubation law for laser damage and ablation thresholds

In multi-pulse laser damage and ablation experiments, the laser-induced damage threshold (LIDT) usually changes with the number of pulses in the train, a phenomenon known as incubation. We introduce a general incubation model based on two physical mechanisms—pulse induced change of (i) absorption and (ii) critical energy that must be deposited to cause ablation. The model is applicable to a broad class of materials and we apply it to fit data for dielectrics and metals. It also explains observed changes of the LIDT as a function of the laser repetition rate. We discuss under which conditions the crater-size method to determine LIDTs can be applied in multi-pulse experiments.

[1]  Jörg Krüger,et al.  Ultrashort pulse laser ablation of polycarbonate and polymethylmethacrylate , 2000 .

[2]  Jianhua Liu,et al.  Scaling laws of femtosecond laser pulse induced breakdown in oxide films , 2005 .

[3]  J. K. Chen,et al.  Numerical investigation of ultrashort laser damage in semiconductors , 2005 .

[4]  Jörg Krüger,et al.  Femtosecond pulse laser processing of TiN on silicon , 2000 .

[5]  Brent C. Stuart,et al.  Optical ablation by high-power short-pulse lasers , 1996 .

[6]  Boris N. Chichkov,et al.  Ablation of metals by ultrashort laser pulses , 1997 .

[7]  Ian D. Hutcheon,et al.  Morphology and microstructure in fused silica induced by high fluence ultraviolet 3ω (355 nm) laser pulses , 2006 .

[8]  T. Glynn,et al.  The effect of damage accumulation behaviour on ablation thresholds and damage morphology in ultrafast laser micro-machining of common metals in air , 2004 .

[9]  Carmen S. Menoni,et al.  Confocal photothermal microscopy of thin films based on etalon and thermal lensing effects , 2013, Laser Damage.

[10]  R. Samad,et al.  D-Scan measurement of ablation threshold incubation effects for ultrashort laser pulses. , 2012, Optics express.

[11]  Zhi‐zhan Xu,et al.  Origin of laser-induced near-subwavelength ripples: interference between surface plasmons and incident laser. , 2009, ACS nano.

[12]  A. Tünnermann,et al.  Femtosecond, picosecond and nanosecond laser ablation of solids , 1996 .

[13]  Igor Goenaga,et al.  On the incubation effect on two thermoplastics when irradiated with ultrashort laser pulses: Broadening effects when machining microchannels , 2006 .

[14]  J. Liu Simple technique for measurements of pulsed Gaussian-beam spot sizes. , 1982, Optics letters.

[15]  Perry,et al.  Nanosecond-to-femtosecond laser-induced breakdown in dielectrics. , 1996, Physical review. B, Condensed matter.

[16]  A. Rosenfeld,et al.  Area dependence of femtosecond laser-induced periodic surface structures for varying band gap materials after double pulse excitation , 2013 .

[17]  Luke A. Emmert,et al.  Modeling the effect of native and laser-induced states on the dielectric breakdown of wide band gap optical materials by multiple subpicosecond laser pulses , 2010 .

[18]  Razvan Stoian,et al.  Surface damage threshold and structuring of dielectrics using femtosecond laser pulses: the role of incubation , 1999 .

[19]  H. Urbassek,et al.  Influence of defects on extreme ultraviolet laser ablation of LiF , 2013 .

[20]  Luke A. Emmert,et al.  Femtosecond Laser-Induced Damage in Dielectric Materials , 2014 .

[21]  Michael F. Becker,et al.  Laser-induced damage on single-crystal metal surfaces , 1988 .

[22]  Hans Joachim Eichler,et al.  Femtosecond-laser induced ablation of silicate glasses and the intrinsic dissociation energy , 2014 .

[23]  P. M. Lugarà,et al.  Role of heat accumulation on the incubation effect in multi-shot laser ablation of stainless steel at high repetition rates. , 2014, Optics express.

[24]  Carmen S. Menoni,et al.  Transient phenomena in the dielectric breakdown of HfO2 optical films probed by ultrafast laser pulse pairs , 2010 .

[25]  B. Jaeggi,et al.  Factors controlling the incubation in the application of ps laser pulses on copper and iron surfaces , 2013, Photonics West - Lasers and Applications in Science and Engineering.

[26]  Herve Bercegol,et al.  What is laser conditioning: a review focused on dielectric multilayers , 1999, Laser Damage.

[27]  B. Luther-Davies,et al.  Ablation of solids by femtosecond lasers: ablation mechanism and ablation thresholds for metals and dielectrics , 2002 .

[28]  S G Demos,et al.  Wavelength dependence of laser-induced damage: determining the damage initiation mechanisms. , 2003, Physical review letters.

[29]  Kai Starke,et al.  On the damage behavior of dielectric films when illuminated with multiple femtosecond laser pulses , 2005 .

[30]  Peter Balling,et al.  Ultra-short pulse laser ablation of metals: threshold fluence, incubation coefficient and ablation rates , 2010 .

[31]  Mindaugas Gedvilas,et al.  Accumulation effects in laser ablation of metals with high-repetition-rate lasers , 2008, High-Power Laser Ablation.

[32]  F. Génin,et al.  Role of light intensification by cracks in optical breakdown on surfaces. , 2001, Journal of the Optical Society of America. A, Optics, image science, and vision.

[33]  Florenta Costache,et al.  Near-damage threshold femtosecond laser irradiation of dielectric surfaces: desorbed ion kinetics and defect dynamics , 2008 .

[34]  Semyon Papernov,et al.  Defect-Induced Damage , 2014 .