Removal of ammonia and particulate matter using a modified turbulent wet scrubbing system

Abstract Conventional scrubbers are typically modified to serve the needs of modern industries that discharge effluents that cause synergetic, adverse effects on the environment. We designed and developed a modified turbulent wet scrubber (MTWS) to remove air pollutants as they emerge from a coal furnace. Experiments were conducted to estimate the pressure drop and the efficiencies of ammonia gas and particulate removal via the MTWS. The optimum water levels and gas flow rates for effective scrubbing of ammonia gas at different concentrations and particulate matter at different feed rates were estimated. For ammonia gas at a concentration of 45 ppm, a gas flow rate of 3.5 m 3 /s and a water level of 58 cm in MTWS and position B (central position of the nozzle) in the water level of the nozzle yielded efficient ammonia gas removal for the given time. Similarly, for a fly ash feeding rate of 140 mg/min, the same gas flow rate and water level in the MTWS yielded high efficiencies even for particles at the submicron level.

[1]  M. Duduković,et al.  Ammonia/flyash interactions and their impact on flue gas treatment technologies , 1994 .

[2]  P. Keshavarz,et al.  Prediction of the spray scrubbers’ performance in the gaseous and particulate scrubbing processes , 2008 .

[3]  Friedrich Löffler,et al.  Investigations on fine particle separation using an electrostatic nozzle scrubber , 1992 .

[4]  L. Claxton,et al.  Genotoxicity of industrial wastes and effluents. , 1992, Mutation research.

[5]  Jaya Narayan Sahu,et al.  Catalytic Hydrolysis of Urea with Fly Ash for Generation of Ammonia in a Batch Reactor for Flue Gas Conditioning and NOx Reduction , 2009 .

[6]  Xavier Font,et al.  Ammonia emissions from the composting of different organic wastes. Dependency on process temperature. , 2006, Chemosphere.

[7]  Bhim Charan Meikap,et al.  Fly-ash removal efficiency in a modified multi-stage bubble column scrubber , 2004 .

[8]  Gautam Kundu,et al.  Modeling of a novel multi-stage bubble column scrubber for flue gas desulfurization☆ , 2002 .

[9]  Gautam Kundu,et al.  Scrubbing of fly‐ash laden SO2 in modified multistage bubble column scrubber , 2002 .

[10]  B. C. Meikap,et al.  Performance characteristics of the particulates scrubbing in a counter-current spray-column , 2008 .

[11]  Oxana Botalova,et al.  Identification and chemical characterization of specific organic constituents of petrochemical effluents. , 2009, Water research.

[12]  R. F. Henry,et al.  Particulate removal from high-temperature, high-pressure combustion gases , 1985 .

[13]  J. Meisinger,et al.  Validation of Ogawa passive samplers for the determination of gaseous ammonia concentrations in agricultural settings , 2003 .

[14]  Sutton,et al.  Ammonia Abatement Strategies in Livestock Production: A Case Study of a Poultry Installation , 2006 .

[15]  Hyung-Keun Lee,et al.  Removal of NO from flue gas by aqueous chlorine-dioxide scrubbing solution in a lab-scale bubbling reactor. , 2008, Journal of hazardous materials.

[16]  B. C. Meikap,et al.  Removal of SO2 from Industrial Effluents by a Novel Twin Fluid Air-Assist Atomized Spray Scrubber , 2008 .

[17]  C. Tseng,et al.  Biotreatment of H2S- and NH3-containing waste gases by co-immobilized cells biofilter. , 2000, Chemosphere.

[18]  J. Lou,et al.  Removal of ammonia solutions used in catalytic wet oxidation processes. , 2003, Chemosphere.

[19]  C. E. Lapple,et al.  PERFORMANCE OF WET DUST SCRUBBERS , 1955 .

[20]  K. W. Lee,et al.  Filtration of Fine Particles by Multiple Liquid Droplet and Gas Bubble Systems , 1998 .

[21]  S. Calvert Venturi and other atomizing scrubbers efficiency and pressure drop , 1970 .

[22]  Kiejin Lee,et al.  Particle Removal Efficiency of Gravitational Wet Scrubber Considering Diffusion, Interception, and Impaction , 2001 .

[23]  Y. Liang,et al.  Long-term results of ammonia removal and transformation by biofiltration. , 2000, Journal of hazardous materials.

[24]  Hyung-Keun Lee,et al.  Simultaneous removal of SO2 and NO by wet scrubbing using aqueous chlorine dioxide solution. , 2006, Journal of hazardous materials.

[25]  Byeong-Kyu Lee,et al.  Development and application of a novel swirl cyclone scrubber—(1) Experimental , 2008 .

[26]  M. N. Biswas,et al.  Fly ash scrubbing in a novel dual flow scrubber. , 2007, Waste management.

[27]  Prediction of the particle capture efficiency based on the combined mechanisms (turbulent diffusion, inertial impaction, interception, and gravitation) by a 3-D simulation of a wet scrubber , 1992 .

[28]  Albert J. Heber,et al.  Sampling and Measurement of Ammonia at Animal Facilities , 2008 .

[29]  Huey-Jen Jenny Su,et al.  Exposure assessment to airborne endotoxin, dust, ammonia, hydrogen sulfide and carbon dioxide in open style swine houses. , 2001 .

[30]  K. Hein,et al.  Mercury emission control in coal-fired plants: The role of wet scrubbers , 2007 .

[31]  I. Moon,et al.  Experimental aspects of combined NOx and SO2 removal from flue-gas mixture in an integrated wet scrubber-electrochemical cell system. , 2009, Chemosphere.

[32]  P. Keshavarz,et al.  Simulation of a spray scrubber performance with Eulerian/Lagrangian approach in the aerosol removing process. , 2006, Journal of hazardous materials.

[33]  T. Curtin,et al.  The selective oxidation of ammonia using copper-based catalysts: The effects of water , 2009 .

[34]  M. Peters,et al.  Simulation of particulate removal in gas‐solid fluidized beds , 1982 .