Polar twilight UV-visible radiation field: Perturbations due to multiple scattering, ozone depletion, stratospheric clouds, and surface albedo

The polar twilight atmosphere is different from that at mid-latitude in several ways which lead to significant changes in the wavelength-dependent radiation field. Ozone depletion in the stratosphere leads to increased scattering below 340 nm. Polar stratospheric clouds produce changes in the radiation field which depend on cloud height and thickness. A surface albedo near unity produces a large increase in scattering. Multiple scattering becomes a larger percentage of the radiation field as solar zenith angle increases. These perturbations on the radiation field lead to enhanced ozone destruction in the stratosphere, increased surface irradiance, and a significant wavelength-dependent increase in nadir radiance.

[1]  M. Molina,et al.  Production of Cl2O2 from the self-reaction of the ClO radical , 1987 .

[2]  M. Patrick McCormick,et al.  Polar stratospheric clouds and the Antarctic ozone hole , 1988 .

[3]  M. Ko,et al.  Chlorine chemistry in the Antarctic stratosphere: Impact of OClO and Cl2 O2 and implications for observations , 1986 .

[4]  R. Meier,et al.  Effects of anisotropic multiple scattering on solar radiation in the troposphere and stratosphere. , 1979, Applied optics.

[5]  Improved model of Mie scattering contribution to tropospheric and stratospheric photodissociation fluxes. , 1980, Applied optics.

[6]  D. Toohey,et al.  Kinetics of O3 destruction by ClO and BrO within the Antarctic vortex: An analysis based on in situ ER‐2 data , 1989 .

[7]  R. Gelinas,et al.  Effect of molecular multiple scattering and surface albedo on atmospheric photodissociation rates , 1976 .

[8]  Y. Yung A numerical method for calculating the mean intensity in an inhomogeneous Rayleigh scattering atmosphere , 1976 .

[9]  M. Nicolet,et al.  Radiation field in the troposphere and stratosphere from 240-1000 NM. I - General analysis. II - Numerical analysis , 1982 .

[10]  D. Anderson The troposphere-stratosphere radiation field at twilight: A spherical model , 1983 .

[11]  M. Nicolet,et al.  On the molecular scattering in the terrestrial atmosphere : An empirical formula for its calculation in the homosphere , 1984 .

[12]  Charles W. Hord,et al.  Multidimensional radiative transfer: Applications to planetary coronae , 1977 .