Spatial and temporal variations of the concentrations of PM 10 , PM 2.5 and PM 1 in China

Abstract. Concentrations of PM10, PM2.5 and PM1 were monitored at 24 CAWNET (China Atmosphere Watch Network) stations from 2006 to 2014. The highest particulate matter (PM) concentrations were observed at the stations of Xian, Zhengzhou and Gucheng, on the Guanzhong Plain and the Huabei Plain (HBP). The second highest PM concentrations were observed in northeast China, followed by southern China. According to the latest air quality standards of China, 14 stations reached the PM10 standard, and only 7 stations, mainly rural and remote stations, reached the PM2.5 standard. The ratios of PM2.5 to PM10 showed a clear increasing trend from northern to southern China, because of the substantial contribution of coarse mineral aerosol in northern China. The ratios of PM1 to PM2.5 were higher than 80 % at most stations. PM concentrations tended to be highest in winter and lowest in summer at most stations, and mineral dust influenced the results in spring. A decreasing interannual trend was observed on the HBP and in southern China for the period 2006 to 2014, but an increasing trend occurred at some stations in northeast China. Bimodal and unimodal diurnal variation patterns were identified at urban stations. Both emissions and meteorological variations dominate the long-term PM concentration trend, while meteorological factors play a leading role in the short term.

[1]  R. Burnett,et al.  The Relationship Among TSP, PM10, PM2.5, and Inorganic Constituents of Atmospheric Participate Matter at Multiple Canadian Locations , 1997 .

[2]  William C. Malm,et al.  Spatial and monthly trends in speciated fine particle concentration in the United States , 2004 .

[3]  Shixiang Gao,et al.  Measurements of PM10 and PM2.5 in urban area of Nanjing, China and the assessment of pulmonary deposition of particle mass. , 2002, Chemosphere.

[4]  Hans Grimm,et al.  Aerosol Measurement: The Use of Optical Light Scattering for the Determination of Particulate Size Distribution, and Particulate Mass, Including the Semi-Volatile Fraction , 2009, Journal of the Air & Waste Management Association.

[5]  L. Weiliang,et al.  Characteristics of the spatial distribution and yearly variation of aerosol optical depth over China in last 30 years , 2001 .

[6]  J. Schauer,et al.  Seasonal trends in PM2.5 source contributions in Beijing, China , 2005 .

[7]  D. S. Bisht,et al.  Variations in Mass of the PM10, PM2.5 and PM1 during the Monsoon and the Winter at New Delhi , 2012 .

[8]  Kebin He,et al.  The water-soluble ionic composition of PM2.5 in Shanghai and Beijing, China , 2002 .

[9]  Kebin He,et al.  The characteristics of PM2.5 in Beijing, China , 2001 .

[10]  W. Wilson,et al.  Ambient Concentrations and Elemental Compositions of PM10 and PM2.5 in Four Chinese Cities , 1999 .

[11]  Xu Tang,et al.  Regional characteristics of dust storms in China , 2004 .

[12]  Qing Mu,et al.  Simulation of the interannual variations of aerosols in China: role of variations in meteorological parameters , 2014 .

[13]  Robert Gehrig,et al.  Characterising seasonal variations and spatial distribution of ambient PM10 and PM2.5 concentrations based on long-term Swiss monitoring data , 2003 .

[14]  Constantinos Sioutas,et al.  Potential Role of Ultrafine Particles in Associations between Airborne Particle Mass and Cardiovascular Health , 2005, Environmental health perspectives.

[15]  R. Sarda-Estève,et al.  Semi‐volatile aerosols in Beijing (R.P. China): Characterization and influence on various PM2.5 measurements , 2007 .

[16]  G. Carmichael,et al.  Asian emissions in 2006 for the NASA INTEX-B mission , 2009 .

[17]  Jiming Hao,et al.  Environmental effects of the recent emission changes in China: implications for particulate matter pollution and soil acidification , 2013 .

[18]  L. Sheng,et al.  Aerosol background at two remote CAWNET sites in western China. , 2009, The Science of the total environment.

[19]  Judith C. Chow,et al.  Winter and Summer PM 2.5 Chemical Compositions in , 2012 .

[20]  Jianping Guo,et al.  A study of the meteorological causes of a prolonged and severe haze episode in January 2013 over central-eastern China , 2014 .

[21]  G. Oberdörster,et al.  Nanotoxicology: An Emerging Discipline Evolving from Studies of Ultrafine Particles , 2005, Environmental health perspectives.

[22]  D. Dockery,et al.  Health Effects of Fine Particulate Air Pollution: Lines that Connect , 2006, Journal of the Air & Waste Management Association.

[23]  Sunling Gong,et al.  Surface observation of sand and dust storm in East Asia and its application in CUACE/Dust , 2007 .

[24]  L. Ruby Leung,et al.  Modeling the transport and radiative forcing of Taklimakan dust over the Tibetan Plateau: A case study in the summer of 2006 , 2013 .

[25]  Thomas A. Cahill,et al.  Composition of PM2.5 and PM10 Aerosols in the IMPROVE Network , 1997 .

[26]  Jiming Hao,et al.  Emission trends and mitigation options for air pollutants in East Asia , 2014 .

[27]  W. Meng,et al.  Scattering properties of the atmospheric aerosol in Beijing, China , 2011 .

[28]  J. Watson Visibility: Science and Regulation , 2002, Journal of the Air & Waste Management Association.

[29]  P. Fischer,et al.  Short-term effects of PM2.5, PM10 and PM2.5-10 on daily mortality in The Netherlands. , 2013, The Science of the total environment.

[30]  B. Gomišček,et al.  Spatial and temporal variations of PM1, PM2.5, PM10 and particle number concentration during the AUPHEP—project , 2004 .

[31]  Delbert J. Eatough,et al.  Semicontinuous PM2.5 and PM10 Mass and Composition Measurements in Lindon, Utah, during Winter 2007 , 2010, Journal of the Air & Waste Management Association.

[32]  Y. Q. Wang,et al.  Spatial distribution and interannual variation of surface PM 10 concentrations over eighty-six Chinese cities , 2010 .

[33]  G. Janssens‑Maenhout,et al.  “ HTAP _ v 2 : a mosaic of regional and global emission gridmaps for 2008 and 2010 to study hemispheric transport of air pollution , 2015 .

[34]  W. Meng,et al.  Seasonal and diurnal variations of ambient PM2.5 concentration in urban and rural environments in Beijing , 2009 .

[35]  Jiamo Fu,et al.  Chemical Composition and Sources of PM10 and PM2.5 Aerosols in Guangzhou, China , 2006, Environmental monitoring and assessment.

[36]  Y. Q. Wang,et al.  Atmospheric aerosol compositions in China: Spatial/temporal variability, chemical signature, regional haze distribution and comparisons with global aerosols , 2011 .

[37]  B. Brunekreef,et al.  Spatial variation of PM2.5, PM10, PM2.5 absorbance and PMcoarse concentrations between and within 20 European study areas and the relationship with NO2 : results of the ESCAPE project , 2012 .

[38]  Zijiang Zhou,et al.  Typical severe dust storms in northern China during 1954 —2002 , 2003 .

[39]  X. Y. Zhang,et al.  Sources of Asian dust and role of climate change versus desertification in Asian dust emission: ASIAN DUST SOURCES , 2003 .

[40]  V. Ramanathan,et al.  Aerosols, Climate, and the Hydrological Cycle , 2001, Science.

[41]  Tony Fletcher,et al.  PM10 and PM2.5 concentrations in Central and Eastern Europe: results from the Cesar study , 2001 .

[42]  O. Boucher,et al.  Estimates of the direct and indirect radiative forcing due to tropospheric aerosols: A review , 2000 .

[43]  Jietai Mao,et al.  Characteristics of distribution and seasonal variation of aerosol optical depth in eastern China with MODIS products , 2003, Science Bulletin.