Optical angular manipulation of liquid crystal droplets in laser tweezers

The high sensitivity of liquid crystals to external fields, especially electromagnetic fields, confer to them fascinating properties. In the case of light fields, their large optical nonlinearities over a broad spectrum have great application potential for all-optical devices. The linear optical properties of liquid crystals, such as their high refractive index, birefringence and transparency, are also of great practical interest in optofluidics, which combines the use of optical tools in microfluidic environments. A representative example is the laser micromanipulation of liquid crystalline systems using optical tweezing techniques. Liquid crystal droplets represent a class of systems that can be easily prepared and manipulated by light, with or without a nonlinear light-matter coupling. Here we review different aspects of quasi-statics and dynamical optical angular manipulation of liquid crystal droplets trapped in laser tweezers. In particular, we discuss to the influence of the phase (nematic, cholesteric or smectic), the bulk ordering symmetry, the droplet size, the polarization state and power of the trapping light, together with the prominent role of light–matter angular momentum exchanges and optical orientational nonlinearities.

[1]  Saulius Juodkazis,et al.  Control of the molecular alignment inside liquid-crystal droplets by use of laser tweezers. , 2005, Small.

[2]  Simon Hanna,et al.  Optical angular momentum transfer by Laguerre-Gaussian beams. , 2009, Journal of the Optical Society of America. A, Optics, image science, and vision.

[3]  H. Rubinsztein-Dunlop,et al.  Optical alignment and spinning of laser-trapped microscopic particles , 1998, Nature.

[4]  Paras N Prasad,et al.  Laser trapping in anisotropic fluids and polarization-controlled particle dynamics , 2006, Proceedings of the National Academy of Sciences.

[5]  Saulius Juodkazis,et al.  Statics and dynamics of radial nematic liquid-crystal droplets manipulated by laser tweezers. , 2008, Physical review. E, Statistical, nonlinear, and soft matter physics.

[6]  Mason,et al.  Emulsification in Viscoelastic Media. , 1996, Physical review letters.

[7]  I Musevic,et al.  Laser trapping of small colloidal particles in a nematic liquid crystal: clouds and ghosts. , 2004, Physical review letters.

[8]  Christelle Monat,et al.  Integrated optofluidics: A new river of light , 2007 .

[9]  D. O. Krimer,et al.  Light-induced instabilities driven by competing helical patterns in long-pitch cholesterics , 2005, The European physical journal. E, Soft matter.

[10]  Nobuyuki Tamaoki,et al.  Design of chiral dimesogens containing cholesteryl groups; formation of new molecular organizations and their application to molecular photonics. , 2004, Chemical Society reviews.

[11]  Kishan Dholakia,et al.  Optically Anisotropic Colloids of Controllable Shape , 2005 .

[12]  Paras N. Prasad,et al.  Optical Trapping, Manipulation, and 3D Imaging of Disclinations in Liquid Crystals and Measurement of their Line Tension , 2005 .

[13]  Miles J. Padgett,et al.  Lights, action: Optical tweezers , 2002 .

[14]  Simon Hanna,et al.  Rotation of absorbing spheres in Laguerre-Gaussian beams. , 2009, Journal of the Optical Society of America. A, Optics, image science, and vision.

[15]  Mark Dickinson,et al.  Laser manipulation in liquid crystals: an approach to microfluidics and micromachines , 2006, Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences.

[16]  P. Gupta,et al.  Rotation of transparent, nonbirefringent objects by transfer of the spin angular momentum of light. , 2005, Optics Letters.

[17]  Kuan Fang Ren,et al.  Radiation pressure forces exerted on a particle arbitrarily located in a Gaussian beam by using the generalized Lorenz-Mie theory, and associated resonance effects , 1994 .

[18]  Pavel Zemánek,et al.  Light at work: The use of optical forces for particle manipulation, sorting, and analysis , 2008, Electrophoresis.

[19]  P. Crooker,et al.  Chiral nematic droplets with parallel surface anchoring , 1997 .

[20]  Amanda J. Wright,et al.  Mechanisms of optical angular momentum transfer to nematic liquid crystalline droplets. , 2004 .

[21]  H. Rubinsztein-Dunlop,et al.  Optical application and measurement of torque on microparticles of isotropic nonabsorbing material , 2003, physics/0309122.

[22]  L. Marrucci,et al.  Light-induced rotation of dye-doped liquid crystal droplets. , 2006, Physical review. E, Statistical, nonlinear, and soft matter physics.

[23]  Holger Stark,et al.  Novel Colloidal Interactions in Anisotropic Fluids , 1997, Science.

[24]  Nelson V. Tabiryan,et al.  Transfer of momentum and torque from a light beam to a liquid , 1997 .

[25]  A. Ashkin Acceleration and trapping of particles by radiation pressure , 1970 .

[26]  J. Cooper,et al.  Multipoint holographic optical velocimetry in microfluidic systems. , 2006 .

[27]  D. Grier A revolution in optical manipulation , 2003, Nature.

[28]  David McGloin,et al.  Optical tweezers: 20 years on , 2006, Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences.

[29]  H. Rubinsztein-Dunlop,et al.  Numerical modelling of optical trapping , 2001 .

[30]  Saulius Juodkazis,et al.  Laser manipulation based on a light-induced molecular reordering. , 2006, Optics express.

[31]  Jonathan Leach,et al.  Multipoint holographic optical velocimetry in microfluidic systems , 2006, SPIE Optics + Photonics.

[32]  Saulius Juodkazis,et al.  Viscosity measurement using a rotating laser-trapped microsphere of liquid crystal , 2006 .

[33]  Electromagnetic torque and force in axially symmetric liquid-crystal droplets. , 2008, Optics letters.

[34]  I. Khoo Nonlinear optics of liquid crystalline materials , 2009 .

[35]  Saulius Juodkazis,et al.  High-efficiency optical transfer of torque to a nematic liquid crystal droplet , 2003 .

[36]  Simon Hanna,et al.  Optical trapping of spheroidal particles in Gaussian beams. , 2007, Journal of the Optical Society of America. A, Optics, image science, and vision.

[37]  H. Misawa,et al.  Laser manipulation of a smectic liquid-crystal droplet , 2006, The European physical journal. E, Soft matter.

[38]  Paras N Prasad,et al.  Optical trapping of director structures and defects in liquid crystals using laser tweezers. , 2007, Optics express.

[39]  I. Jánossy,et al.  Influence of anthraquinone dyes on optical reorientation of nematic liquid crystals. , 1992, Optics letters.

[40]  Hajime Tanaka,et al.  Optical manipulation of defects in a lyotropic lamellar phase. , 2003, Physical review letters.

[41]  Saulius Juodkazis,et al.  Characterization of bipolar and radial nematic liquid crystal droplets using laser-tweezers , 2005 .

[42]  Saulius Juodkazis,et al.  Fast optical switching by a laser-manipulated microdroplet of liquid crystal , 1999 .

[43]  Hiroshi Yokoyama,et al.  Direct observation of anisotropic interparticle forces in nematic colloids with optical tweezers. , 2004, Physical review letters.

[44]  Bifurcation analysis of optically induced dynamics in nematic liquid crystals: elliptical polarization at normal incidence , 2005 .

[45]  Hiroshi Masuhara,et al.  Manipulation of liquid crystal textures with a focused near infrared laser beam , 1997 .

[46]  Nelson V. Tabiryan,et al.  Orientational Optical Nonlinearity of Liquid Crystals , 1986 .

[47]  Brian S. Wherrett,et al.  Anomalous optical Freedericksz transition in an absorbing liquid crystal , 1990 .

[48]  A. Pattanaporkratana,et al.  Manipulation of Disk-Shaped Islands on Freely Suspended Smectic Films and Bubbles Using Optical Tweezers , 2004 .

[49]  J. P. Barton,et al.  Theoretical determination of net radiation force and torque for a spherical particle illuminated by a focused laser beam , 1989 .

[50]  Enrico Santamato,et al.  Optical angular momentum transfer to transparent isotropic particles using laser beam carrying zero average angular momentum. , 2002, Optics express.

[51]  E. Brasselet,et al.  Light-induced chaotic rotations in nematic liquid crystals. , 2006, Physical review. E, Statistical, nonlinear, and soft matter physics.

[52]  Saulius Juodkazis,et al.  Rheology Measurement at Liquid-Crystal Water Interface Using Laser Tweezers , 2006 .

[53]  M. Dickinson,et al.  Continuously rotating chiral liquid crystal droplets in a linearly polarized laser trap. , 2008, Optics express.

[54]  E. Santamato,et al.  On-off intermittency in chaotic rotation induced in liquid crystals by competition between spin and orbital angular momentum of light. , 2003, Physical review. E, Statistical, nonlinear, and soft matter physics.