Making carbon sequestration a paying proposition

Atmospheric carbon dioxide (CO2) has increased from a preindustrial concentration of about 280 ppm to about 367 ppm at present. The increase has closely followed the increase in CO2 emissions from the use of fossil fuels. Global warming caused by increasing amounts of greenhouse gases in the atmosphere is the major environmental challenge for the 21st century. Reducing worldwide emissions of CO2 requires multiple mitigation pathways, including reductions in energy consumption, more efficient use of available energy, the application of renewable energy sources, and sequestration. Sequestration is a major tool for managing carbon emissions. In a majority of cases CO2 is viewed as waste to be disposed; however, with advanced technology, carbon sequestration can become a value-added proposition. There are a number of potential opportunities that render sequestration economically viable. In this study, we review these most economically promising opportunities and pathways of carbon sequestration, including reforestation, best agricultural production, housing and furniture, enhanced oil recovery, coalbed methane (CBM), and CO2 hydrates. Many of these terrestrial and geological sequestration opportunities are expected to provide a direct economic benefit over that obtained by merely reducing the atmospheric CO2 loading. Sequestration opportunities in 11 states of the Southeast and South Central United States are discussed. Among the most promising methods for the region include reforestation and CBM. The annual forest carbon sink in this region is estimated to be 76 Tg C/year, which would amount to an expenditure of $11.1–13.9 billion/year. Best management practices could enhance carbon sequestration by 53.9 Tg C/year, accounting for 9.3% of current total annual regional greenhouse gas emission in the next 20 years. Annual carbon storage in housing, furniture, and other wood products in 1998 was estimated to be 13.9 Tg C in the region. Other sequestration options, including the direct injection of CO2 in deep saline aquifers, mineralization, and biomineralization, are not expected to lead to direct economic gain. More detailed studies are needed for assessing the ultimate changes to the environment and the associated indirect cost savings for carbon sequestration.

[1]  Catherine A Peters,et al.  Safe storage of CO2 in deep saline aquifers. , 2002, Environmental science & technology.

[2]  S. Kempe Carbon in the rock cycle , 1979 .

[3]  R. Birdsey,et al.  Costs of creating carbon sinks in the U.S. , 1993 .

[4]  O. Hoegh‐Guldberg,et al.  Ecological responses to recent climate change , 2002, Nature.

[5]  Jürgen Mienert,et al.  Gas hydrates: relevance to world margin stability and climate change , 1998 .

[6]  B. Haq Methane in the Deep Blue Sea , 1999, Science.

[7]  Sohei Shimada,et al.  Displacement behavior of CH4 adsorbed on coals by injecting pure CO2, N2, and CO2–N2 mixture , 2005 .

[8]  Duane H. Smith,et al.  Assessing the Thermodynamic Feasibility of the Conversion of Methane Hydrate into Carbon Dioxide Hydrate in Porous Media , 2001 .

[9]  V. Ramanathan The Greenhouse Theory of Climate Change: A Test by an Inadvertent Global Experiment , 1988, Science.

[10]  Olivier Braissant,et al.  Biomineralization in plants as a long-term carbon sink , 2004, Naturwissenschaften.

[11]  A. A. Reznik,et al.  An analysis of the effect of CO2 injection on the recovery of in situ methane from bituminous coal: an experimental simulation , 1984 .

[12]  É. Verrecchia,et al.  Biologically induced mineralization in the tree Milicia excelsa (Moraceae): its causes and consequences to the environment , 2004 .

[13]  R. Vogel,et al.  Global warming and the hydrologic cycle , 1996 .

[14]  R. Lal Carbon sequestration in soil. , 2008 .

[15]  Mark Peters,et al.  Economics of Sequestering Carbon in the U.S. Agricultural Sector , 2004 .

[16]  O. Davidson,et al.  Climate change 2001 : mitigation , 2001 .

[17]  Pathegama Gamage Ranjith,et al.  The effect of CO2 on the geomechanical and permeability behaviour of brown coal: Implications for coal seam CO2 sequestration , 2006 .

[18]  J. Houghton,et al.  Climate change 2001 : the scientific basis , 2001 .

[19]  H. Isenberg,et al.  The Mechanisms of Mineralization in the Invertebrates and Plants , 1976 .

[20]  G. Edwards,et al.  C3, C4: Mechanisms and Cellular and Environmental Regulation of Photosynthesis , 1983 .

[21]  Keith Paustian,et al.  Management Controls on Soil Carbon , 2019, Soil Organic Matter in Temperate Agroecosystems.

[22]  H. Herzog Peer Reviewed: What Future for Carbon Capture and Sequestration? , 2001 .

[23]  M. Lacuesta,et al.  A study of photorespiratory ammonia production in the C4 plant Amaranthus edulis, using mutants with altered photosynthetic capacities , 1997 .

[24]  E. M. Winter,et al.  Disposal of carbon dioxide in aquifers in the U.S. , 1995 .

[25]  A. A. Reznik,et al.  A Laboratory Investigation Of Enhanced Recovery Of Methane From Coal By Carbon Dioxide Injection , 1980 .

[26]  Carl J. Bernacchi,et al.  The conversion of the corn/soybean ecosystem to no‐till agriculture may result in a carbon sink , 2005 .

[27]  Atul K. Jain,et al.  Energy implications of future stabilization of atmospheric CO2 content , 1998, Nature.

[28]  Nebojsa Nakicenovic,et al.  Summary for policymakers of impacts, adaptations and mitigation of climate change, IPCC Working Group II , 1995 .

[29]  W. A. Cunningham,et al.  Utilization of Texas serpentine. , 1950 .

[30]  Rattan Lal,et al.  Cropland to Sequester Carbon and Mitigate the Greenhouse Effect , 1998 .

[31]  M. Burger,et al.  Nitrogen oxide and methane emissions under varying tillage and fertilizer management. , 2005, Journal of environmental quality.

[32]  Donald L. DeAngelis,et al.  The global carbon cycle. , 1990 .

[33]  G. Robertson,et al.  Greenhouse gases in intensive agriculture: contributions of individual gases to the radiative forcing of the atmosphere , 2000, Science.

[34]  H. Delcourt,et al.  Carbon Budget of the Southeastern U.S. Biota: Analysis of Historical Change in Trend from Source to Sink , 1980, Science.

[35]  W. Gunter,et al.  Large CO2 Sinks: Their role in the mitigation of greenhouse gases from an international, national (Canadian) and provincial (Alberta) perspective , 1998 .

[36]  S. Arnórsson Environmental impact of geothermal energy utilization , 2004, Geological Society, London, Special Publications.

[37]  J. Downing,et al.  Workshop Summary Statement: Terrestrial Bioshperic Carbon Fluxes Quantification of Sinks and Sources of CO2 , 1993 .

[38]  Dever,et al.  Oxygen Requirement and Inhibition of C4 Photosynthesis. An analysis of c4 plants deficient in the c3 and c4 cycles An Analysis of C4 Plants Deficient in the C3 and C4 Cycles , 1998, Plant physiology.

[39]  Vello Kuuskraa,et al.  CO2 sequestration in deep coal seams , 1999 .

[40]  C. M. White,et al.  Separation and Capture of CO2 from Large Stationary Sources and Sequestration in Geological Formations—Coalbeds and Deep Saline Aquifers , 2003, Journal of the Air & Waste Management Association.

[41]  The effect of CO 2 on the geomechanical and permeability behaviour of brown coal : Implications for coal seam CO 2 sequestration , 2006 .

[42]  H. Herzog THE COST OF CARBON CAPTURE , 2000 .

[43]  Bernhard Schlamadinger,et al.  Forest Harvests and Wood Products: Sources and Sinks of Atmospheric Carbon Dioxide , 1998, Forest Science.

[44]  Rattan Lal,et al.  Managing U.S. cropland to sequester carbon in soil , 1999 .

[45]  K. Paustian,et al.  Soil Organic Matter in Temperate Agroecosystems , 1997 .

[46]  Estimation of diffusive resistance of bundle sheath cells to CO2 from modeling of C4 photosynthesis , 1996, Photosynthesis Research.

[47]  W. Gunter,et al.  Deep coalbed methane in Alberta, Canada: A fuel resource with the potential of zero greenhouse gas emissions , 1997 .

[48]  K. Kvenvolden,et al.  A primer on the geological occurrence of gas hydrate , 1998, Geological Society, London, Special Publications.

[49]  F. Han,et al.  Terrestrial carbon sequestration in southeast and south-central United States , 2006 .

[50]  Sam Holloway,et al.  An overview of the underground disposal of carbon dioxide , 1997 .

[51]  H. Herzog,et al.  What future for carbon capture and sequestration? , 2001, Environmental science & technology.

[52]  C. V. Cole,et al.  Global estimates of potential mitigation of greenhouse gas emissions by agriculture , 1997, Nutrient Cycling in Agroecosystems.

[53]  K. E. Skog,et al.  Carbon cycling through wood products : The role of wood and paper products in carbon sequestration , 1998 .

[54]  Maria Mastalerz,et al.  Carbon dioxide and methane sorption in high volatile bituminous coals from Indiana, USA , 2004 .

[55]  John R. Butnor,et al.  Meeting global policy commitments: carbon sequestration and southern pine forests , 2001 .

[56]  Tore A. Torp,et al.  An innovative European integrated project: Castor-CO2 from capture to storage , 2005 .