Stabilization of unstable states, relaxation, and critical slowing down in a bistable system

The unstable branch of stationary states in an illuminated thermochemical bistable system is stabilized with an external feedback loop which does not otherwise alter the autonomous system. The technique allows the measurement of the entire set of stationary states available to the system. Trajectories of transition between branches of stationary states (relaxation) are investigated theoretically and experimentally. Critical slowing down in the speed of the trajectories is predicted and measured as the points of marginal stability are approached. Trajectories are observed to spread as they depart from the unstable stationary state and then to coalesce as they approach a stable stationary state. These results are obtained due to experimental spread in initial conditions and not from noise along the relaxation trajectory.