Global increase in atmospheric methane concentrations between 1978 and 1980

The concentration of methane has been measured in tropospheric air samples collected in remote locations between 55°N and 53°S during six collection periods between November 1977 and November 1980. The observed concentrations of CH4 have increased in each of six latitude locations by an average of 0.052±0.005 ppmv between January 1978 and January 1980. This (1.4±0.2)×1014 gram increase in the total atmospheric burden of CH4 corresponds to 35±12% of the yearly flux of (4.0±1.3)×1014 grams needed to maintain the CH4 concentration in steady-state at its recent level of about 1.6 ppmv. The 1978-1980 excess of about 0.7×1014 grams per year of sources over sinks for CH4 could arise from either an increase in biogenic releases or from a decrease in the average OH radical concentration in the lower troposphere, or from both.

[1]  D. E. Wagoner Presence of Male Determining Factors found on Three Autosomes in the House Fly, Musca domestica , 1969, Nature.

[2]  Ralph J. Cicerone,et al.  Sources of atmospheric methane: Measurements in rice paddies and a discussion , 1981 .

[3]  L. Heidt,et al.  Corrections of CH4 concentrations measured prior to 1974 , 1980 .

[4]  R. E. Larson,et al.  Trace gas concentrations, intertropical convergence, atmospheric fronts, and ocean currents in the tropical Pacific , 1979 .

[5]  W. Chameides,et al.  The two-dimensional diagnostic model for tropospheric OH - An uncertainty analysis , 1981 .

[6]  M. Khalil,et al.  Increase in the concentration of atmospheric methane , 1981 .

[7]  D. Ehhalt The CH 4 concentration over the ocean and its possible variation with latitude , 1978 .

[8]  F. Rowland,et al.  Tropospheric concentrations of methylchloroform, CH(3)CCl(3), in January 1978 and estimates of the atmospheric residence times for hydrohalocarbons. , 1981, Proceedings of the National Academy of Sciences of the United States of America.

[9]  S. Wofsy,et al.  Tropospheric chemistry: A global perspective , 1981 .

[10]  P. Fraser,et al.  Trends of atmospheric methane in the southern hemisphere , 1981 .

[11]  D. Blake,et al.  Methane: Interhemispheric concentration gradient and atmospheric residence time. , 1982, Proceedings of the National Academy of Sciences of the United States of America.

[12]  D. Ehhalt The atmospheric cycle of methane , 1974 .

[13]  M. Migeotte Spectroscopic Evidence of Methane in the Earth's Atmosphere , 1948 .

[14]  H. Schiff The Stratosphere 1981: Theory and Measurements World Meterological Organization Global Ozone Research and Monitoring Project Report Number 11 Causes and Effects of Stratospheric Ozone Reduction: An Update National Academy of Sciences , 1982 .

[15]  J. Hansen,et al.  Greenhouse effect of trace gases, 1970‐1980 , 1981 .

[16]  Ralph J. Cicerone,et al.  Possible variations in atmospheric methane , 1977 .

[17]  V. Linnenbom,et al.  C 1 -C 4 hydrocarbons in the North and South Pacific , 1974 .

[18]  J. Hansen,et al.  Greenhouse Effects due to Man-Made Perturbations of Trace Gases , 1976, Science.

[19]  S. Wofsy,et al.  Natural Sources of Atmospheric CO , 1971, Nature.

[20]  M. Khalil,et al.  Atmospheric methane /CH4/ - Trends and seasonal cycles , 1981 .

[21]  C. R. Burnett,et al.  Spectroscopic measurements of the vertical column, abundance of hydroxyl (OH) in the earth's atmosphere , 1981 .