Surface Acoustic Wave Driven Light Shutters Using Polymer‐Dispersed Liquid Crystals

displays, [ 3 ] microlenses, [ 4 , 5 ] lasers, [ 6 , 7 ] and data storage, [ 8 ] due to their excellent electro-optical properties. PDLC fi lms can be prepared between two conductive, transparent substrates using methods such as encapsulation, thermally induced phase separation, solvent-induced phase separation, and polymerizationinduced phase separation. [ 9 ] Within a PDLC fi lm, liquid crystals (LCs) are generally trapped in a transparent polymer medium, thus forming micrometer-scale LC droplets. The random dispersion of LC droplets in the polymer matrix causes a strong scattering of light due to the signifi cant refractive index mismatch between the two materials; therefore, a PDLC fi lm is naturally opaque. Based on laser interference holography, various periodic structures such as gratings [ 10–12 ] and photonic crystals, [ 13 , 14 ] can be also introduced inside the fi lm, coined as holographic PDLCs (HPDLCs). [ 15 ] The application of an electric fi eld can re-orientate the LC molecules inside a droplet, thus modulating the refractive index difference between the polymer matrix and the LC. A complete refractive index match between the two materials can be achieved by tuning the LCs to a specifi c orientation. In such a way, the PDLC fi lm can be switched from opaque to transparent. The switching properties of PDLCs are infl uenced by many variables including the size and shape of the LC droplets, [ 16 , 17 ] and molecular interactions between the LCs and polymer matrix. [ 18 , 19 ]

[1]  P. Filippi,et al.  First French Conference on Acoustics , 1991 .

[2]  Y. Fainman,et al.  Form-birefringent metal and its plasmonic anisotropy , 2010, CLEO/QELS: 2010 Laser Science to Photonic Applications.

[3]  R A Schmidt,et al.  Full-field acoustomammography using an acousto-optic sensor. , 2009, Medical physics.

[4]  Shin-Tson Wu,et al.  Tunable-focus microlens arrays using nanosized polymer-dispersed liquid crystal droplets , 2005 .

[5]  A. Wixforth,et al.  Planar chip device for PCR and hybridization with surface acoustic wave pump. , 2005, Lab on a chip.

[6]  Giuseppe Chidichimo,et al.  Self-adjusting smart windows based on polymer-dispersed liquid crystals , 2009 .

[7]  T. Huang,et al.  Electrically switchable phase-type fractal zone plates and fractal photon sieves. , 2009, Optics express.

[8]  Xiao Wei Sun,et al.  A polarization insensitive 2×2 optical switch fabricated by liquid crystal–polymer composite , 2005 .

[9]  Paul S Drzaic Liquid crystal dispersions , 1995 .

[10]  Xiang Zhang,et al.  Surface plasmon interference nanolithography. , 2005, Nano letters.

[11]  H. Cao,et al.  Effects of the structures of epoxy monomers on the electro-optical properties of heat-cured polymer-dispersed liquid crystal films , 2010 .

[12]  T. Huang,et al.  A frequency-addressed plasmonic switch based on dual-frequency liquid crystals , 2010 .

[13]  Yuebing Zheng,et al.  Light‐Driven Plasmonic Switches Based on Au Nanodisk Arrays and Photoresponsive Liquid Crystals , 2008 .

[14]  Paul S. Drzaic Droplet size and shape effects in nematic droplet/polymer films , 1990, Other Conferences.

[15]  J. W. Doane,et al.  Field controlled light scattering from nematic microdroplets , 1986 .

[16]  Achim Wixforth,et al.  Microfluidic mixing via acoustically driven chaotic advection. , 2008, Physical review letters.

[17]  Paul Mulvaney,et al.  Direct observation of chemical reactions on single gold nanocrystals using surface plasmon spectroscopy. , 2008, Nature nanotechnology.

[18]  Jinjie Shi,et al.  Optically switchable gratings based on azo-dye-doped, polymer-dispersed liquid crystals. , 2009, Optics letters.

[19]  Jaswinder S. Sandhu,et al.  Liquid crystal-based acoustic imaging , 2000, Electronic Imaging.

[20]  Dwight W. Berreman,et al.  Liquid‐crystal twist cell dynamics with backflow , 1975 .

[21]  David W. Gerdt,et al.  Ultrasonic liquid crystal-based underwater acoustic imaging , 1999, Electronic Imaging.

[22]  X. W. Sun,et al.  Gain narrowing and random lasing from dye-doped polymer-dispersed liquid crystals with nanoscale liquid crystal droplets , 2006 .

[23]  Daniel Ahmed,et al.  Acoustic tweezers: patterning cells and microparticles using standing surface acoustic waves (SSAW). , 2009, Lab on a chip.

[24]  Wu,et al.  Birefringence dispersions of liquid crystals. , 1986, Physical review. A, General physics.

[25]  C. D. Sheraw,et al.  Organic thin-film transistor-driven polymer-dispersed liquid crystal displays on flexible polymeric substrates , 2002 .

[26]  Achim Wixforth,et al.  Surface acoustic wave mediated coupling of free-space radiation into surface plasmon polaritons on plain metal films , 2010 .

[27]  Xiao Wei Sun,et al.  Effect of surfactant on the electro-optical properties of holographic polymer dispersed liquid crystal Bragg gratings , 2005 .

[28]  M. Ozaki,et al.  Reorientation of Cholesteric Liquid Crystal Molecules Using Acoustic Streaming , 2007 .

[29]  Masanori Ozaki,et al.  Lasing in Cholesteric Liquid Crystal Oriented by Acoustic Streaming , 2008 .

[30]  Jonathan V Selinger,et al.  Dynamics of the acousto‐optic effect in a nematic liquid crystal , 2005 .

[31]  Jonathan V Selinger,et al.  Acoustic realignment of nematic liquid crystals. , 2002, Physical review. E, Statistical, nonlinear, and soft matter physics.

[32]  W. Helfrich Orienting Action of Sound on Nematic Liquid Crystals , 1972 .

[33]  A. Wixforth,et al.  Flow patterns and transport in Rayleigh surface acoustic wave streaming: combined finite element method and raytracing numerics versus experiments , 2008, IEEE Transactions on Ultrasonics, Ferroelectrics and Frequency Control.

[34]  Yi Xiong,et al.  Tuning the far-field superlens: from UV to visible. , 2007, Optics express.

[35]  Xiao Wei Sun,et al.  Electrically switchable computer-generated hologram recorded in polymer-dispersed liquid crystals , 2007 .

[36]  C. Z. Van Doorn,et al.  Dynamic behavior of twisted nematic liquid‐crystal layers in switched fields , 1975 .

[37]  Jonathan V Selinger,et al.  Theory of the acoustic realignment of nematic liquid crystals. , 2004, Physical review. E, Statistical, nonlinear, and soft matter physics.

[38]  Lalgudi V. Natarajan,et al.  Holographic Formation of Electro‐Optical Polymer–Liquid Crystal Photonic Crystals , 2002 .

[39]  J. Dion,et al.  A new hypothesis on ultrasonic interaction with nematic liquid crystal , 1977 .

[40]  Daniel Ahmed,et al.  Focusing microparticles in a microfluidic channel with standing surface acoustic waves (SSAW). , 2008, Lab on a chip.

[41]  J. West,et al.  Light scattering from polymer‐dispersed liquid crystal films: Droplet size effects , 1991 .

[42]  Zhongze Gu,et al.  Phototunable Microlens Array Based on Polymer Dispersed Liquid Crystals , 2009 .

[43]  Bin Zhang,et al.  Improvement of the diffraction properties in holographic polymer dispersed liquid crystal bragg gratings , 2003 .

[44]  Lalgudi V. Natarajan,et al.  Bragg gratings in an acrylate polymer consisting of periodic polymer-dispersed liquid-crystal planes , 1993 .

[45]  L. V. Natarajan,et al.  Holographic Polymer-Dispersed Liquid Crystals (H-PDLCs)1 , 2000 .

[46]  X. W. Sun,et al.  Effect of liquid crystal concentration on the lasing properties of dye-doped holographic polymer-dispersed liquid crystal transmission gratings , 2007 .

[47]  T. Fujisawa,et al.  Reversible optical control of transmittance in polymer/liquid crystal composite films by photoinduced phase transition , 1999 .

[48]  X. W. Sun,et al.  Electrically Tunable Three-Dimensional Holographic Photonic Crystal Made of Polymer-Dispersed Liquid Crystals Using a Single Prism , 2007 .

[49]  J. William Doane,et al.  Response times and voltages for PDLC light shutters , 1989 .

[50]  Leslie Y Yeo,et al.  Microparticle collection and concentration via a miniature surface acoustic wave device. , 2007, Lab on a chip.

[51]  K. Miyano,et al.  Excitation of stripe domain patterns by propagating acoustic waves in an oriented nematic film , 1977 .