We report results from tests of {sup 83}Kr{sup m} as a calibration source in liquid argon and liquid neon. {sup 83}Kr{sup m} atoms are produced in the decay of {sup 83}Rb, and a clear {sup 83}Kr{sup m} scintillation peak at 41.5 keV appears in both liquids when filling our detector through zeolite coated with {sup 83}Rb. Based on this scintillation peak, we observe 6.0 photoelectrons/keV in liquid argon with a resolution of 8.2% (sigma/E) and 3.0 photoelectrons/keV in liquid neon with a resolution of 19% (sigma/E). The observed peak intensity subsequently decays with the {sup 83}Kr{sup m} half-life after stopping the fill, and we find evidence that the spatial location of {sup 83}Kr{sup m} atoms in the chamber can be resolved. {sup 83}Kr{sup m} will be a useful calibration source for liquid argon, neon dark matter, and solar neutrino detectors.