CFD Simulation of Mass Transfer Efficiency and Pressure Drop in a Structured Packed Distillation Column

The pressure drop and mass transfer efficiency for two-phase flow in a structured packed column were simulated using a commercial CFD package, CFX version 10. The distillation of the methanol/isopropanol system was carried out in a 0.073 m diameter column, with an element composed of a ceramic structured packing and 0.053 m in height. The Height Equivalent to Theoretical Plate (HETP) value varied from 0.106–0.146 m. Pressure drop experiments were measured with an air/water system. The pressure drops at the flooding and loading points were ca. 173 and 580 Pa/m of packing, respectively. HETPs and pressure drops calculated from the Computational Fluid Dynamics (CFD) model were compared to their experimental counterparts. The average relative error between CFD predictions and the experimental data for the prediction of dry pressure drop, irrigated pressure drop and mass transfer efficiency are 20.3 %, 23 % and 9.15 %, respectively. In all cases, the CFD predictions show a good agreement with the experimental data, indicating that CFD is a reliable, cost saving and suitable technique for the design and optimization of separation processes.

[1]  T. Chung Computational Fluid Dynamics: FOUR. AUTOMATIC GRID GENERATION, ADAPTIVE METHODS, AND COMPUTING TECHNIQUES , 2002 .

[2]  Lothar Spiegel,et al.  Distillation Columns with Structured Packings in the Next Decade , 2003 .

[3]  Hiroshi Takeuchi,et al.  MASS TRANSFER COEFFICIENTS BETWEEN GAS AND LIQUID PHASES IN PACKED COLUMNS , 1968 .

[4]  Djamel Lakehal,et al.  On the modelling of multiphase turbulent flows for environmental and hydrodynamic applications , 2002 .

[5]  Ireneusz Zbicinski,et al.  Liquid Flow on Structured Packing: CFD Simulation and Experimental Study , 2003 .

[6]  Liquid-phase mass transfer within KATAPAK-S® structures studied using computational fluid dynamics simulations , 2001 .

[7]  Rajamani Krishna,et al.  Radial and axial dispersion of the liquid phase within a KATAPAK-S® structure : experiments vs. CFD simulations , 2001 .

[8]  Faïçal Larachi,et al.  Pressure drop through structured packings: Breakdown into the contributing mechanisms by CFD modeling , 2003 .

[9]  Bernard P. A. Grandjean,et al.  Tailoring the pressure drop of structured packings through CFD simulations , 2003 .

[10]  Rajamani Krishna,et al.  Gas and liquid phase mass transfer within KATAPAK-S® structures studied using CFD simulations , 2002 .

[11]  J. A. Rocha,et al.  Design Method for Distillation Columns Filled with Metallic, Ceramic, or Plastic Structured Packings , 1997 .

[12]  James R. Fair,et al.  Distillation Columns Containing Structured Packings: A Comprehensive Model for Their Performance. 2. Mass-Transfer Model , 1996 .