Co-combustion of sewage sludge from different treatment processes and a lignite coal in a laboratory scale combustor

Abstract One sustainable use of sewage sludge (SS) is to use it as fuel in existing coal-fired plants. Towards this end, this study evaluated thermal characteristics and co-combustion efficiency of dried SS samples from six wastewater treatment plants with different sludge treatment units. Fuel quality of SS based on proximate and ultimate analyses and calorific value, and ash composition by XRF analysis were investigated. Then the SS samples were co-combusted in a laboratory batch reactor in mixtures with coal (3%, 5%, 10%, 20% and 30%). Results showed that samples had good calorific values (between 1931 and 3852 cal/g). Furthermore, the type of sludge stabilization processes had an important effect on thermal characteristics of samples and the point where the sludge addition started to intrude the combustion efficiency. Among all stabilization methods, lime stabilization was observed to affect the thermal characteristics the most. Sludge treated with anaerobic stabilization had lower calorific values than the ones stabilized aerobically. The results from co-combustion experiments showed that as the percentage of SS in the mixture increased from 5% to 30%, the combustion efficiency decreased gradually from 99.5% to 97.5%. Furthermore, according to XRF analysis result, fouling and slagging indices of samples were higher than the limit values.

[1]  M. Otero,et al.  Simultaneous thermogravimetric-mass spectrometric study on the co-combustion of coal and sewage sludges , 2006 .

[2]  Y. Liu,et al.  A new method for evaluating the sewage sludge pyrolysis kinetics. , 2010, Waste management.

[3]  A. Atimtay,et al.  Emission Characteristics of Co-combustion of Sewage Sludge with Olive Cake and Lignite Coal in a Circulating Fluidized Bed , 2004, Journal of environmental science and health. Part A, Toxic/hazardous substances & environmental engineering.

[4]  Janne Nerg,et al.  Performance analysis of power generating sludge combustion plant and comparison against other sludge treatment technologies , 2010 .

[5]  J. Kozinski,et al.  Properties of ash generated during sewage sludge combustion: A multifaceted analysis , 2016 .

[6]  Liao Yanfen,et al.  Thermogravimetric analysis of the co-combustion of coal and paper mill sludge , 2010 .

[7]  M. Folgueras,et al.  Thermogravimetric analysis of the co-combustion of coal and sewage sludge ☆ , 2003 .

[8]  J. Ferrasse,et al.  Co-gasification of wastewater sludge and different feedstock: Feasibility study , 2016 .

[9]  Mohd Roslee Othman,et al.  Thermogravimetric characteristics and pyrolysis kinetics of Giheung Respia sewage sludge , 2010 .

[10]  R. Font,et al.  Comparison between emissions from the pyrolysis and combustion of different wastes , 2013 .

[11]  Takayuki Takarada,et al.  Nitrogen transformations during fast pyrolysis of sewage sludge , 2013 .

[12]  L Zhang,et al.  INFLUENCE OF COAL PROPERTIES ON THE CO-COMBUSTION CHARACTERISTICS OF LOW-GRADE COAL AND CITY MUD , 2014 .

[13]  M. Baratieri,et al.  Clay-sewage sludge co-pyrolysis. A TG-MS and Py-GC study on potential advantages afforded by the presence of clay in the pyrolysis of wastewater sewage sludge. , 2011, Waste management.

[14]  Vladimir Strezov,et al.  Thermal characterisation of the products of wastewater sludge pyrolysis , 2009 .

[15]  P. Rangsunvigit,et al.  Pyrolytic characteristics of sewage sludge. , 2006, Chemosphere.

[16]  M. Folgueras,et al.  Influence of FeCl3 and lime added to sludge on sludge–coal pyrolysis , 2010 .

[17]  Oliver Krüger,et al.  Complete survey of German sewage sludge ash. , 2014, Environmental science & technology.

[18]  Joachim Werther,et al.  Gaseous emissions from co-combustion of sewage sludge and coal/wood in a fluidized bed , 2004 .

[19]  P. Gale,et al.  Land application of treated sewage sludge: quantifying pathogen risks from consumption of crops , 2005, Journal of applied microbiology.

[20]  Shengyong Lu,et al.  Emission characteristics of dioxins, furans and polycyclic aromatic hydrocarbons during fluidized-bed combustion of sewage sludge. , 2009, Journal of environmental sciences.

[21]  Meng Niu,et al.  Combustion Characteristics of Sewage Sludge in a Fluidized Bed , 2012 .

[22]  O. M. Martinez,et al.  Kinetic study and characterization of sewage sludge for its incineration , 2008 .

[23]  Sang-Woo Park,et al.  Effects of carbonization and solvent-extraction on change in fuel characteristics of sewage sludge. , 2011, Bioresource technology.

[24]  Ken-Lin Chang,et al.  Thermogravimetric characteristics of textile dyeing sludge, coal and their blend in N2/O2 and CO2/O2 atmospheres , 2017 .

[25]  S. Keel,et al.  Thermogravimetric study for the co-combustion of coal and dried sewage sludge , 2017, Korean Journal of Chemical Engineering.

[26]  Xiaoqian Ma,et al.  Isoconversional kinetic analysis of co-combustion of sewage sludge with straw and coal , 2009 .

[27]  Sonja Schreurs,et al.  Study of bio-oils and solids from flash pyrolysis of sewage sludges , 2009 .

[28]  Zhiyong Wang,et al.  Additive adsorption behavior of sludge and its influence on the slurrying ability of coal–sludge–slurry and petroleum coke–sludge–slurry , 2018 .

[29]  Susanna Nilsson,et al.  Gasification reactivity of char from dried sewage sludge in a fluidized bed , 2012 .

[30]  D. Bright,et al.  Contaminant risks from biosolids land application: contemporary organic contaminant levels in digested sewage sludge from five treatment plants in Greater Vancouver, British Columbia. , 2003, Environmental pollution.

[31]  B. Lecknera,et al.  Gaseous emissions from co-combustion of sewage sludge and coal / wood in a fluidized bed , 2003 .

[32]  Jae kwan Kim,et al.  Investigation on the combustion possibility of dry sewage sludge as a pulverized fuel of thermal power plant , 2010 .

[33]  J. A. Menéndez,et al.  Bio-syngas production with low concentrations of CO2 and CH4 from microwave-induced pyrolysis of wet and dried sewage sludge. , 2008, Chemosphere.

[34]  G. O. Thomas,et al.  Behavior of sewage sludge-derived PAHs on pasture. , 2001, Environmental science & technology.

[35]  Monica Puccini,et al.  Cogasification of sewage sludge in an updraft gasifier , 2012 .

[36]  M. B. Murillo,et al.  Study of catalytic post-treatment of the vapours from sewage sludge pyrolysis by means of γ-Al2O3 , 2013 .

[37]  J. Werther,et al.  Sewage sludge combustion , 1999 .

[38]  Uwe Schnell,et al.  Behaviour of Gaseous Chlorine and Alkali Metals During Biomass Thermal Utilisation , 2005 .

[39]  Kunio Yoshikawa,et al.  Characteristics of tar, NOx precursors and their absorption performance with different scrubbing solvents during the pyrolysis of sewage sludge , 2011 .

[40]  Geir Skjevrak,et al.  Sintering characteristics of sewage sludge ashes at elevated temperatures , 2012 .

[41]  Cheng Zhang,et al.  Co-firing sludge in a pulverized coal-fired utility boiler: Combustion characteristics and economic impacts , 2017 .

[42]  Johannes W Judex,et al.  Gasification of dried sewage sludge: status of the demonstration and the pilot plant. , 2012, Waste management.

[43]  L. F. Calvo,et al.  TG-MS as a technique for a better monitoring of the pyrolysis, gasification and combustion of two kinds of sewage sludge , 2004 .

[44]  M. Otero,et al.  Thermogravimetric analysis of biowastes during combustion. , 2010, Waste management.

[45]  Baoqing Li,et al.  Formation of NOx precursors during the pyrolysis of coal and biomass. Part V. Pyrolysis of a sewage sludge , 2002 .

[46]  Y. Xing,et al.  Combustion behaviors and kinetics of sewage sludge blended with pulverized coal: With and without catalysts. , 2018, Waste management.

[47]  J. S. Dennis,et al.  The devolatilisation of particles of a complex fuel (dried sewage sludge) in a fluidised bed , 2007 .

[48]  Sang-Woo Park,et al.  Characteristics of carbonized sludge for co-combustion in pulverized coal power plants. , 2011, Waste management.

[49]  Hitoshi Hirose,et al.  Combustion characteristics of sewage sludge in an incineration plant for energy recovery , 2009 .

[50]  J. S. Dennis,et al.  Thermogravimetric measurements of the kinetics of pyrolysis of dried sewage sludge , 2006 .

[51]  J. A. Menéndez,et al.  Microwave pyrolysis of sewage sludge: analysis of the gas fraction , 2004 .

[52]  J. Ferrasse,et al.  Mineralogy and leachability of gasified sewage sludge solid residues. , 2011, Journal of hazardous materials.

[53]  Jian-hua Yan,et al.  Co-combustion of Bituminous Coal and Pickling Sludge in a Drop-Tube Furnace: Thermodynamic Study and Experimental Data on the Distribution of Cr, Ni, Mn, As, Cu, Sb, Pb, Cd, Zn, and Sn , 2017 .

[54]  R. Junga,et al.  Experimental tests of co-combustion of laying hens manure with coal by using thermogravimetric analysis , 2017 .

[55]  Ryszard Wasielewski,et al.  Co-combustion of dried sewage sludge and coal in a pulverized coal boiler , 2008 .

[56]  L. F. Calvo,et al.  Analysis of the co-combustion of sewage sludge and coal by TG-MS , 2002 .

[57]  Combustion kinetics of sewage sludge and combustible wastes , 2009 .

[58]  M. Otero,et al.  Non-isothermal thermogravimetric analysis of the combustion of two different carbonaceous materials , 2008 .

[59]  D. Vamvuka,et al.  Combustion behaviour of biomass fuels and their blends with lignite , 2011 .

[60]  Hai‐feng Liu,et al.  Behavior of Phosphorus during Co-gasification of Sewage Sludge and Coal , 2012 .

[61]  Liang Wang,et al.  Effects of Sewage Sludge and Marble Sludge Addition on Slag Characteristics during Wood Waste Pellets Combustion , 2011 .

[62]  Alexandros Kelessidis,et al.  Comparative study of the methods used for treatment and final disposal of sewage sludge in European countries. , 2012, Waste management.

[63]  Kunio Yoshikawa,et al.  Pyrolysis gasification of dried sewage sludge in a combined screw and rotary kiln gasifier , 2011 .

[64]  J. Jiang,et al.  Analysis of the combustion of sewage sludge-derived fuel by a thermogravimetric method in China. , 2010, Waste management.

[65]  Y. Yue,et al.  Investigation of sulfur forms and transformation during the co-combustion of sewage sludge and coal using X-ray photoelectron spectroscopy. , 2009, Journal of hazardous materials.

[66]  N Lapa,et al.  The behaviour of ashes and heavy metals during the co-combustion of sewage sludges in a fluidised bed. , 2003, Waste management.

[67]  M. Otero,et al.  Effects of sewage sludge blending on the coal combustion: a thermogravimetric assessment. , 2007, Chemosphere.

[68]  Enrico Biagini,et al.  Devolatilization rate of biomasses and coal–biomass blends: an experimental investigation , 2002 .

[69]  Małgorzata Wzorek,et al.  Characterisation of the properties of alternative fuels containing sewage sludge , 2012 .

[70]  M. V. Gil,et al.  Co-combustion of different sewage sludge and coal: a non-isothermal thermogravimetric kinetic analysis. , 2008, Bioresource technology.

[71]  Stanisław Ledakowicz,et al.  The kinetics of gasification of char derived from sewage sludge , 2011 .

[72]  Xiaoqian Ma,et al.  Co-combustion kinetics of sewage sludge with coal and coal gangue under different atmospheres , 2010 .

[73]  Marek Pronobis,et al.  Evaluation of the influence of biomass co-combustion on boiler furnace slagging by means of fusibility correlations , 2005 .

[74]  J. Vaxelaire,et al.  Product distribution and kinetic scheme for the fixed bed thermal decomposition of sewage sludge , 2009 .

[75]  Se-Joon Park,et al.  Effects of Hydrothermally Pretreated Sewage Sludge on the Stability and Dispersibilty of Slurry Fuel Using Pulverized Coal , 2011 .

[76]  Helena Lopes,et al.  Evaluation of slagging and fouling tendency during biomass co-firing with coal in a fluidized bed , 2012 .

[77]  Michał Kozioł,et al.  Co-combustion of sludge with coal , 2003 .

[78]  J. A. Menéndez,et al.  On the pyrolysis of sewage sludge: the influence of pyrolysis conditions on solid, liquid and gas fractions , 2002 .

[79]  Monika Kosowska-Golachowska,et al.  Experimental research of sewage sludge with coal and biomass co-combustion, in pellet form. , 2016, Waste management.