Modeling the grating-formation process in thick bacteriorhodopsin films.

We model the grating-formation process in bacteriorhodopsin films for the interference of two plane waves. We simulate the temporal dependence of grating recording and readout, and we examine the behavior of the diffraction efficiency with respect to exposure, write and read wavelengths, and film parameters such as initial optical density and lifetime of the upper state. Gratings written in thick bacteriorhodopsin films are generally nonuniform and nonsinusoidal owing to the absorption and saturation properties of the material. The simulations also show that one can often obtain optimization of hologram recording and readout by writing and reading at wavelengths far off the peak of the ground-state absorbance spectrum, especially for films with high values of the peak optical density.

[1]  J D Downie,et al.  Measurements of holographic properties of bacteriorhodopsin films. , 1996, Applied optics.

[2]  Norbert Hampp,et al.  Bacteriorhodopsin-films for dynamic time average interferometry , 1993 .

[3]  W. Tomlinson,et al.  Volume holograms in photochromic materials. , 1975, Applied optics.

[4]  Norbert Hampp,et al.  Biological photochrome bacteriorhodopsin and its genetic variant Asp96 ? Asn as media for optical pattern recognition. , 1992, Applied optics.

[5]  N. Hampp,et al.  Bacteriorhodopsin wildtype and variant aspartate-96 --> aspargine as reversible holographic media. , 1990, Biophysical journal.

[6]  Dorian Kermisch,et al.  Nonuniform Sinusoidally Modulated Dielectric Gratings , 1969 .

[7]  Phenomenological theory of photochromic media: optical data storage and processing with bacteriorhodopsin films , 1997 .

[8]  Norbert Hampp,et al.  Diffraction efficiency of bacteriorhodopsin films for holography containing bacteriorhodopsin wildtype BRWT and its variants BRD85E and BRD96N , 1992 .

[9]  R. Birge Photophysics and molecular electronic applications of the rhodopsins. , 1990, Annual review of physical chemistry.

[10]  Q W Song,et al.  Chemically enhanced bacteriorhodopsin thin-film spatial light modulator. , 1993, Optics letters.

[11]  D. Kermisch Efficiency of Photochromic Gratings , 1971 .

[12]  Dieter Oesterhelt,et al.  Kinetic optimization of bacteriorhodopsin by aspartic acid 96 as an internal proton donor , 1990 .

[13]  H. Kogelnik Coupled wave theory for thick hologram gratings , 1969 .

[14]  N. Hampp,et al.  Bacteriorhodopsin films as spatial light modulators for nonlinear-optical filtering. , 1991, Optics letters.

[15]  Norbert Hampp,et al.  Optical Applications of Bacteriorhodopsin and its mutated variants , 1991 .

[16]  J D Downie Real-time holographic image correction using bacteriorhodopsin. , 1994, Applied optics.

[17]  Y. Ninomiya Recording characteristics of volume holograms , 1973 .