Wavevector-dependent shear viscosity in Lennard-Jones liquids

Computer simulation data for the generalized wavevector-dependent shear viscosity η(q) are reported for the first time in a Lennard-Jones fluid. The transverse current autocorrelation functions are also presented. The results are carefully compared with simple viscoelectric theory. Although the latter is found to give a respectable description of the data, discrepancies are pointed out.

[1]  M. Schoen,et al.  The shear viscosity of a Lennard-Jones fluid calculated by equilibrium molecular dynamics , 1985 .

[2]  U. Balucani,et al.  Self-diffusion and relative diffusion processes in liquids: microdynamic and hydrodynamic points of view , 1985 .

[3]  D. Jou,et al.  The underlying thermodynamic aspects of generalized hydrodynamics , 1985 .

[4]  C. Murthy,et al.  CORRIGENDUM: Velocity correlations, cooperative effects and relative diffusion in simple liquids , 1983 .

[5]  B. Alder,et al.  Generalized transport coefficients for hard spheres , 1983 .

[6]  B. Alder,et al.  Neutron scattering function for hard spheres , 1983 .

[7]  D. Heyes Self-diffusion and shear viscosity of simple fluids. A molecular-dynamics study , 1983 .

[8]  R. Mountain Molecular-dynamics study of liquid rubidium , 1982 .

[9]  E. Leutheusser Dynamics of a classical hard-sphere gas. II. Numerical results , 1982 .

[10]  E. Leutheusser Dynamics of a classical hard-sphere gas I. Formal theory , 1982 .

[11]  P. Mason,et al.  Atomic dynamics and momentum transfer in dense liquids , 1981 .

[12]  L. Sjögren Kinetic theory of current fluctuations in simple classical liquids , 1980 .

[13]  L. Sjögren Numerical results on the density fluctuations in liquid rubidium , 1980 .

[14]  L. Sjogren,et al.  Kinetic theory of self-motion in monatomic liquids , 1979 .

[15]  S. Miller,et al.  Longitudinal modes, transverse modes and velocity correlations in liquids. I , 1978 .

[16]  W. Götze,et al.  Mode-coupling theory of simple classical liquids , 1978 .

[17]  L. Verlet,et al.  Computer "Experiments" on Classical Fluids. IV. Transport Properties and Time-Correlation Functions of the Lennard-Jones Liquid near Its Triple Point , 1973 .

[18]  R. Zwanzig,et al.  Generalized Hydrodynamics and Analysis of Current Correlation Functions , 1971 .

[19]  A. Akcasu,et al.  Fluctuation Analysis in Simple Fluids , 1970 .