Laser remote sensing of atmospheric ammonia using a CO2 lidar system.

A CO2 differential-absorption lidar system has been used for the remote sensing of ammonia in the atmosphere. For CO2 lidar returns backscattered from topographic targets at ranges up to 2.7 km, the path-averaged sensitivity of the DIAL system was 5 ppb of NH3 . Concentrations of atmospheric ammonia were found to vary during the day from undetectable levels (<5 ppb) to as high as 20 ppb, depending on temperature and humidity conditions.

[1]  R. Byer,et al.  Remote SO2 measurements at 4 Mum with a continuously tunable source. , 1978, Optics letters.

[2]  Dennis K. Killinger,et al.  Remote probing of the atmosphere using a CO 2 DIAL system , 1981 .

[3]  N. Lau,et al.  On the discrepancy between background atmospheric ammonia gas measurements and the existence of acid sulfates as a dominant atmospheric aerosol , 1977 .

[4]  J C Petheram Differential backscatter from the atmospheric aerosol: the implications for IR differential absorption lidar. , 1981, Applied optics.

[5]  N Menyuk,et al.  Remote sensing of NO using a differential absorption lidar. , 1980, Applied optics.

[6]  L. J. Cox Optical Properties of the Atmosphere , 1979 .

[7]  B Nilsson,et al.  Meteorological influence on aerosol extinction in the 0.2-40-microm wavelength range. , 1979, Applied optics.

[8]  N. Menyuk,et al.  Development of a high‐repetition‐rate mini‐TEA CO2 laser , 1980 .

[9]  R. Harriss,et al.  Sources of atmospheric ammonia , 1982 .

[10]  E. Murray,et al.  Remote measurement of ethylene using a CO(2) differential-absorption lidar. , 1978, Applied optics.

[11]  Assessment of relative error sources in IR DIAL measurement accuracy. , 1983, Applied optics.

[12]  C. Bruce,et al.  Photoacoustic spectroscopy of NH(3) at the 9-microm and 10-microm (12)C(16)O(2) laser wavelengths. , 1978, Applied optics.

[13]  W. McClenny,et al.  CO(2) Laser Absorption Coefficients for Determining Ambient Levels of O(3), NH(3), and C(2)H(4). , 1974, Applied optics.

[14]  A G Kjelaas,et al.  Scintillation and multiwavelength coherence effects in a long-path laser absorption spectrometer. , 1978, Applied optics.

[15]  Kazuhiro Asai,et al.  Range‐resolved measurements of atmospheric ozone using a differential‐absorption CO2 laser radar , 1979 .

[16]  C. Jaussaud,et al.  Absorption coefficients of various pollutant gases at CO(2) laser wavelengths; application to the remote sensing of those pollutants. , 1978, Applied optics.

[17]  R. Tanner,et al.  Continuous determination of gaseous ammonia in the ambient atmosphere using fluorescence derivatization , 1981 .

[18]  N Menyuk,et al.  Temporal correlation measurements of pulsed dual CO(2) lidar returns. , 1981, Optics letters.