Nonlinear optical limiting of the azo dye methyl-red doped nematic liquid crystalline films

We describe the nonlinear optical limiting behaviors of the azo dye methyl-red-doped nematic liquid crystalline (NLC) films and report the phenomena of the formation of an interesting dark spot and a dynamic self-action diffraction ring pattern in the far field beyond the sample cell. We present the method of measuring the optical limiting characteristics of the methyl-red-dye-doped NLC films with typical test results obtained in the experiments. We theoretically analyze the optical limiting mechanisms of the methyl-red-dye-doped NLC films and discuss the advantages and restrictions of the methyl-red dye doped liquid crystal limiters, and propose several possible solutions to overcome these restrictions.

[1]  Svetlana G. Lukishova,et al.  NONLINEAR OPTICAL RESPONSE OF CYANOBIPHENYL LIQUID CRYSTALS TO HIGH-POWER, NANOSECOND LASER RADIATION , 2000 .

[2]  M. Wood,et al.  Extremely nonlinear photosensitive liquid crystals for image sensing and sensor protection. , 1999, Optics express.

[3]  H. Ming,et al.  Nonlinear optical and optical-limiting properties of Azobenzene liquid crystal polymer , 2002 .

[4]  X Zhang,et al.  Nolinear optical liquid cored fiber array and liquid crystal film fo ps-cw frequency agile laser optical limiting application. , 1998, Optics express.

[5]  I. Khoo,et al.  Optically induced space-charge fields, dc voltage, and extraordinarily large nonlinearity in dye-doped nematic liquid crystals. , 1998, Optics letters.

[6]  M. Wood,et al.  Nonlinear absorption and optical limiting of laser pulses in a liquid-cored fiber array , 1998 .

[7]  T. F. Boggess,et al.  A review of optical limiting mechanisms and devices using organics, fullerenes, semiconductors and other materials , 1993 .

[8]  L. Deng,et al.  Optical limiting behavior of nanosized polyicosahedral gold-silver clusters based on third-order nonlinear optical effects. , 2001, Journal of the American Chemical Society.

[9]  Oriano Francescangeli,et al.  REVIEW ARTICLE: Effects of light on molecular orientation of liquid crystals , 1999 .

[10]  I. Khoo,et al.  Nonlinear optical propagation and self-limiting effect in liquid-crystalline fibers , 1994 .

[11]  A new self-diffraction pattern formation in defocusing liquid media , 1997 .

[12]  Stephen D. Durbin,et al.  Optical-Field-Induced Birefringence and Freedericksz Transition in a Nematic Liquid Crystal , 1981 .

[13]  S. Arakelian,et al.  Laser-induced diffraction rings from a nematic-liquid-crystal film. , 1981, Optics letters.

[14]  N. Rosanov,et al.  Analysis of dark spot formation in absorbing liquid media , 1998 .

[15]  Iam-Choon Khoo,et al.  Self‐phase modulation and optical limiting of a low‐power CO2 laser with a nematic liquid‐crystal film , 1988 .

[16]  T. C. Damen,et al.  THE THERMAL LENS EFFECT AS A POWER‐LIMITING DEVICE , 1967 .

[17]  Svetlana G. Lukishova Cumulative self-phase modulation in planar nematics driven by 532-nm nanosecond laser pulses , 1999, Optics & Photonics.

[18]  J. P. Gordon,et al.  Long‐Transient Effects in Lasers with Inserted Liquid Samples , 1965 .

[19]  I. Jánossy,et al.  Low-Power Optical Reorientation in Dyed Nematics , 1991 .

[20]  I. Khoo,et al.  Passive optical self-limiter using laser-induced axially asymmetric and symmetric transverse self-phase modulations in nematic liquid crystals. , 1986, Optics letters.

[21]  Iam-Choon Khoo,et al.  Liquid Crystals: Physical Properties and Nonlinear Optical Phenomena , 1994 .

[22]  H. Ono,et al.  Controllable optical intensity limiting of a He-Ne laser with host-guest liquid crystals , 1997 .

[23]  E. Sharp,et al.  Studies of the Nonlinear Switching Properties of Liquid Crystals with Picosecond Pulses , 1985 .

[24]  Hua-Kuang Liu,et al.  Adaptive grating optical limiting with organic photonic materials , 2001, SPIE OPTO.

[25]  F. Simoni,et al.  Power limiting and optical switching with nematic liquid-crystal films , 1986 .

[26]  I. Khoo A REVIEW OF NONLINEAR OPTICAL PROPERTIES OF NEMATIC LIQUID CRYSTALS , 1999 .