Radiocarbon dating by accelerator mass spectrometry: some recent results and applications

14C differs from other nuclides measured by accelerator mass spectrometry (AMS) in that an extensive database of dates already exists, AMS dates should therefore have comparable accuracy, and the measurement of isotopic ratios to better than 1 % , which was an important technical goal, has been reached. The main advantage of being able to date samples 1000 times smaller than previously lies in the extra selectivity that can be employed. This is reflected in the results and applications. Selection can apply at several levels; from objects th at formerly contained too little carbon, to the choice of archaeological material, to the extraction of specific chemical compounds from a complex environmental sample. This is particularly useful in removing uncertainty regarding the validity of a date, since a given sample may comprise carbon atoms from different sources each with their own 14C ‘age’. Examples from archaeological and environmental research illustrating these points are given. 14C dating by AMS differs from conventional radiocarbon dating by having the potential to measure much lower levels of 14C, and therefore should double the time span of the method. This potential has not yet been realized because of sample contamination effects, and work in progress to reduce these is described.

[1]  J. Gowlett,et al.  Radiocarbon dates from the chambered tomb at Hazleton (Glos.): a chronology for neolithic collective burial , 1987, Antiquity.

[2]  K. V. Rowsell,et al.  The chemistry and biochemistry of the amino acids : Edited by G.C. Barrett Chapman and Hall; London, 1985 x + 684 pages. £49.50 (hardback) , 1987 .

[3]  D. Brothwell,et al.  Lindow Man: The Body in the Bog , 1986 .

[4]  J. Gowlett,et al.  RADIOCARBON DATES FROM THE OXFORD AMS SYSTEM: ARCHAEOMETRY DATELIST 4 , 1986 .

[5]  J. Duplessy,et al.  Direct dating of the oxygen-isotope record of the last deglaciation by 14C accelerator mass spectrometry , 1986, Nature.

[6]  R. Beukens,et al.  Progress at the Isotrace Radiocarbon Facility , 1986, Radiocarbon.

[7]  M. Suter,et al.  Dating Polar Ice by 14C Accelerator Mass Spectrometry , 1986, Radiocarbon.

[8]  R. Gillespie,et al.  Routine AMS Dating of Bone and Shell Proteins , 1986, Radiocarbon.

[9]  H. Oeschger,et al.  14C Dating of Plant Macrofossils in Lake Sediment , 1986, Radiocarbon.

[10]  D. Donahue,et al.  Excess carbon-14 abundances in uranium ores: Possible evidence for emission from uranium-series isotopes , 1985 .

[11]  R. Gillespie,et al.  Status of the Oxford radiocarbon accelerator , 1984 .

[12]  L. A. Currie,et al.  Accelerator mass spectrometry sample preparation: Methods for 14C in 50–1000 microgram samples☆ , 1984 .

[13]  J. Southon,et al.  Performance of catalytically condensed carbon for use in accelerator mass spectrometry , 1984 .

[14]  R. Middleton A review of ion sources for accelerator mass spectrometry , 1984 .

[15]  M. Nessi,et al.  Precision measurements of 14C in AMS — some results and prospects , 1984 .

[16]  N. Conard,et al.  Computer controlled isotope ratio measurements and data analysis , 1984 .

[17]  M. Baillie,et al.  High-Precision 14C Measurement of Irish Oaks to Show the Natural Atmospheric 14C Variations of the AD Time Period , 1983, Radiocarbon.

[18]  M. Baillie,et al.  High-Precision 14C Measurement of Irish Oaks to Show the Natural 14C Variations from 200 BC to 4000 BC , 1983, Radiocarbon.

[19]  N. White,et al.  The Oxford Radiocarbon Accelerator Facility , 1983, Radiocarbon.

[20]  M. Stuiver A high-precision calibration of the AD radiocarbon time scale , 1982, Radiocarbon.

[21]  A. J. Walker,et al.  14C Interlaboratory Comparison in the UK: Experiment Design, Preparation and Preliminary Results , 1980, Radiocarbon.

[22]  William R. Stott,et al.  Carbon-14: Direct Detection at Natural Concentrations , 1977, Science.

[23]  C. Bennett,et al.  Radiocarbon Dating Using Electrostatic Accelerators: Negative Ions Provide the Key , 1977, Science.

[24]  G. Faure Principles of isotope geology , 1977 .

[25]  G. K. Wehner,et al.  Angular Distribution of Sputtered Material , 1960 .