Stochastic analysis of solute transport in heterogeneous, dual‐permeability media

[1] A Eulerian perturbation method is applied to study the influence of medium heterogeneity on nonreactive chemical transport in a saturated, fractured porous medium under steady state flow conditions. A dual-permeability model is used to describe the flow and solute transport in the fractured medium [, 1993a, 1993b]. The model involves two overlaying continua at the macroscopic level, a fracture pore system, and a less permeable matrix pore system. Solute advection and dispersion take place in both pore systems. A first-order mass diffusion model is used to describe the mass diffusion between fracture and matrix regions. The hydraulic conductivities in both fracture and matrix regions, Kf and Km, and the interregional mass diffusion coefficient, a, are assumed to be spatial random variables to account for heterogeneity of the medium. A closed form analytical solution for the mean concentrations in the fracture and matrix regions is explicitly given in Fourier and Laplace transforms and numerically inverted to real space via fast Fourier transform. The simulation results demonstrate the significant effects of heterogeneous distributions of Kf, Km, and a on solute transport process. Sensitivity studies show the dominant influence of heterogeneity in fracture in comparison with that in matrix. In some special scenarios of heterogeneity the dual-permeability model can be simplified to a mobile/immobile model [, 2000] or a one-domain model [, 1993]. The developed analytical solution provides a general tool to investigate the effects of various heterogeneities on solute transport in fractured porous media and to analyze the errors introduced through various model simplifications.

[1]  M. V. Genuchten,et al.  Mass transfer studies in sorbing porous media. I. Analytical solutions , 1976 .

[2]  H. Einstein,et al.  Characterisation of Fracture Apertures - Methods And Parameters , 1995 .

[3]  Geoffrey Ingram Taylor,et al.  Diffusion by Continuous Movements , 1922 .

[4]  Horst H. Gerke,et al.  Evaluation of a first-order water transfer term for variably saturated dual-porosity flow models , 1993 .

[5]  Bill X. Hu,et al.  Nonlocal reactive transport in heterogeneous dual‐porosity media with rate‐limited sorption and interregional mass diffusion , 2001 .

[6]  M. V. Genuchten,et al.  A dual-porosity model for simulating the preferential movement of water and solutes in structured porous media , 1993 .

[7]  R. L. Naff On the nature of the dispersive flux in saturated heterogeneous porous media. , 1990 .

[8]  Robert Bibby,et al.  Mass transport of solutes in dual‐porosity media , 1981 .

[9]  S. P. Neuman,et al.  Reconstruction and geostatistical analysis of multiscale fracture apertures in a large block of welded tuff , 1992 .

[10]  Allen F. Moench,et al.  Double‐Porosity Models for a Fissured Groundwater Reservoir With Fracture Skin , 1984 .

[11]  E. Sudicky,et al.  The interpretation of a tracer experiment conducted in a single fracture under conditions of natural groundwater flow , 1999 .

[12]  Stephen R. Brown Simple mathematical model of a rough fracture , 1995 .

[13]  G. Dagan Stochastic modeling of groundwater flow by unconditional and conditional probabilities: 2. The solute transport , 1982 .

[14]  G. Dagan Solute transport in heterogeneous porous formations , 1984, Journal of Fluid Mechanics.

[15]  John F. Brady,et al.  Anomalous diffusion in heterogeneous porous media , 1988 .

[16]  S. P. Neuman,et al.  Eulerian-Lagrangian analysis of transport conditioned on hydraulic data 3. Spatial moments, travel time distribution, mass flow rate, and cumulative release across a compliance surface , 1995 .

[17]  K. H. Coats,et al.  Dead-End Pore Volume and Dispersion in Porous Media , 1964 .

[18]  Alexander Y. Sun,et al.  Stochastic analysis of transient saturated flow through heterogeneous fractured porous media: A double‐permeability approach , 2000 .

[19]  G. Dagan Flow and transport in porous formations , 1989 .

[20]  Bill X. Hu,et al.  Nonlocal nonreactive transport in heterogeneous porous media with interregional mass diffusion , 2000 .

[21]  J. Gale,et al.  Comparison of coupled fracture deformation and fluid flow models with direct measurements of fracture pore structure and stress-flow properties , 1987 .

[22]  Stephen R. Brown,et al.  Correlation between the surfaces of natural rock joints , 1986 .

[23]  Eva Hakami,et al.  Aperture measurements and flow experiments on a single natural fracture , 1996 .

[24]  J. H. Cushman,et al.  Hierarchical Approaches to Transport in Heterogeneous Porous Media , 1991 .

[25]  Ralph E. Showalter,et al.  Diffusion models for fractured media , 1990 .

[26]  J. H. Cushman,et al.  A FAST FOURIER TRANSFORM STOCHASTIC ANALYSIS OF THE CONTAMINANT TRANSPORT PROBLEM , 1993 .

[27]  C. Axness,et al.  Three‐dimensional stochastic analysis of macrodispersion in aquifers , 1983 .

[28]  P. Witherspoon,et al.  Porous media equivalents for networks of discontinuous fractures , 1982 .

[29]  Todd Arbogast,et al.  Derivation of the double porosity model of single phase flow via homogenization theory , 1990 .

[30]  M. Brusseau,et al.  Nonideal transport of reactive solutes in heterogeneous porous media: 6. Microscopic and macroscopic approaches for incorporating heterogeneous rate‐limited mass transfer , 2000 .