Variations in modeled atmospheric transport of carbon dioxide and the consequences for CO2 inversions

Carbon dioxide concentrations due to fossil fuel burning and CO 2 exchange with the terrestrial biosphere have been modeled with 12 different three-dimensional atmospheric transport models. The models include both on-line and off-line types and use a variety of advection algorithms and subgrid scale parameterizations. A range of model resolutions is also represented. The modeled distributions show a large range of responses. For the experiment using the fossil fuel source, the annual mean meridional gradient at the surface vases by a factor of 2. This suggests a factor of 2 variation in the efficiency of surface interhemispheric exchange as much due to differences in model vertical transport as to horizontal differences. In the upper troposphere, zonal mean gradients within the northern hemisphere vary in sign. In the terrestrial biotic source experiment, the spatial distribution of the amplitude and the phase of the seasonal cycle of surface CO 2 concentration vary little between models. However, the magnitude of the amplitudes varies similarly to the fossil case. Differences between modeled and observed seasonal cycles in the northern extratropics suggest that the terrestrial biotic source is overestimated in late spring and underestimated in winter. The annual mean response to the seasonal source also shows large differences in magnitude. The uncertainty in hemispheric carbon budgets implied by the differences in interhemispheric exchange times is comparable to those quoted by the Intergovernmental Panel on Climate Change for fossil fuel and ocean uptake and smaller than those for terrestrial fluxes. We outline approaches which may reduce this component in CO 2 budget uncertainties.

[1]  Ian G. Enting,et al.  A synthesis inversion of the concentration and δ 13 C of atmospheric CO 2 , 1995 .

[2]  Pieter P. Tans,et al.  Evidence for interannual variability of the carbon cycle from the National Oceanic and Atmospheric Administration/Climate Monitoring and Diagnostics Laboratory Global Air Sampling Network , 1994 .

[3]  Shoichi Taguchi,et al.  A three‐dimensional model of atmospheric CO2 transport based on analyzed winds: Model description and simulation results for TRANSCOM , 1996 .

[4]  John A. Taylor A stochastic Lagrangian atmospheric transport model to determine global CO2 sources and sinks–a preliminary discussion , 1989 .

[5]  David Rind,et al.  Chemistry of the Global Troposphere' Fluorocarbons as Tracers of Air Motion , 2007 .

[6]  D. Randall,et al.  Latitudinal gradient of atmospheric CO2 due to seasonal exchange with land biota , 1995, Nature.

[7]  Philippe Ciais,et al.  Partitioning of ocean and land uptake of CO2 as inferred by δ13C measurements from the NOAA Climate Monitoring and Diagnostics Laboratory Global Air Sampling Network , 1995 .

[8]  G. Russell,et al.  Three‐dimensional tracer model study of atmospheric CO2: Response to seasonal exchanges with the terrestrial biosphere , 1983 .

[9]  M. Wahlen,et al.  Interannual extremes in the rate of rise of atmospheric carbon dioxide since 1980 , 1995, Nature.

[10]  Philip J. Rasch,et al.  The seasonal cycle of atmospheric CO2: A study based on the NCAR Community Climate Model (CCM2) , 1996 .

[11]  C. Tucker,et al.  A three dimensional model of atmospheric CO2 transport based on observed winds: 3. Seasonal cycle and synoptic time scale variations , 1989 .

[12]  G. Russell,et al.  A New Finite-Differencing Scheme for the Tracer Transport Equation , 1981 .

[13]  I. Fung,et al.  Observational Contrains on the Global Atmospheric Co2 Budget , 1990, Science.

[14]  W. Moxim,et al.  Tracer simulation using a global general circulation model: Results from a midlatitude instantaneous source experiment , 1978 .

[15]  I. G. Enting,et al.  On the use of smoothing splines to filter CO2 data , 1987 .

[16]  Radon‐222 as a test of convective transport in a general circulation model , 1990 .

[17]  D. Jacob,et al.  Atmospheric distribution of 85Kr simulated with a general circulation model , 1987 .

[18]  Martin Heimann,et al.  The global atmospheric tracer model TM3 , 1995 .

[19]  P. Bousquet,et al.  Radon-222 measurements during the Tropoz II campaign and comparison with a global atmospheric transport model , 1996 .

[20]  Ian G. Enting,et al.  Future emissions and concentrations of carbon dioxide: Key ocean / atmosphere / land analyses , 1994 .

[21]  Inez Y. Fung,et al.  Application of Advanced Very High Resolution Radiometer vegetation index to study atmosphere‐biosphere exchange of CO2 , 1987 .

[22]  R. Law,et al.  APPLICATION OF AN ATMOSPHERIC TRACER MODEL TO HIGH SOUTHERN LATITUDES , 1992 .

[23]  Takakiyo Nakazawa,et al.  Temporal and spatial variations of upper tropospheric and lower stratospheric carbon dioxide , 1991 .