Rigorous modal analysis of plasmonic nanoresonators

The specificity of modal-expansion formalisms is their capabilities to model the physical properties in the natural resonance-state basis of the system in question, leading to a transparent interpretation of the numerical results. In electromagnetism, modal-expansion formalisms are routinely used for optical waveguides. In contrast, they are much less mature for analyzing open non-Hermitian systems, such as micro and nanoresonators. Here, by accounting for material dispersion with auxiliary fields, we considerably extend the capabilities of these formalisms, in terms of computational effectiveness, number of states handled and range of validity. We implement an efficient finite element solver to compute the resonance states, and derive new closed-form expressions of the modal excitation coefficients for reconstructing the scattered fields. Together, these two achievements allow us to perform rigorous modal analysis of complicated plasmonic resonators, being not limited to a few resonance states, with straightforward physical interpretations and remarkable computation speeds. We particularly show that, when the number of states retained in the expansion increases, convergence towards accurate predictions is achieved, offering a solid theoretical foundation for analyzing important issues, e.g. Fano interference, quenching, coupling with the continuum, which are critical in nanophotonic research.

[1]  Paul Urbach,et al.  Efficient computation of the spontaneous decay rate of arbitrarily shaped 3D nanosized resonators: a Krylov model-order reduction approach , 2016 .

[2]  Lukas Novotny,et al.  Principles of Nano-Optics by Lukas Novotny , 2006 .

[3]  Aaswath Raman,et al.  Photonic band structure of dispersive metamaterials formulated as a Hermitian eigenvalue problem. , 2010, Physical review letters.

[4]  P Lalanne,et al.  Efficient and intuitive method for the analysis of light scattering by a resonant nanostructure. , 2013, Optics express.

[5]  Benjamin Vial,et al.  Quasimodal expansion of electromagnetic fields in open two-dimensional structures , 2013, 1311.3244.

[6]  Bernhard J. Hoenders,et al.  On the completeness of the natural modes for quantum mechanical potential scattering , 1979 .

[7]  J. Joannopoulos,et al.  Temporal coupled-mode theory for the Fano resonance in optical resonators. , 2003, Journal of the Optical Society of America. A, Optics, image science, and vision.

[8]  P. Nordlander,et al.  The Fano resonance in plasmonic nanostructures and metamaterials. , 2010, Nature materials.

[9]  Jean-Jacques Greffet,et al.  Surface plasmon Fourier optics , 2009, 0902.1926.

[10]  Shanhui Fan,et al.  Temporal coupled-mode theory and the presence of non-orthogonal modes in lossless multimode cavities , 2004, IEEE Journal of Quantum Electronics.

[11]  H Giessen,et al.  From Dark to Bright: First-Order Perturbation Theory with Analytical Mode Normalization for Plasmonic Nanoantenna Arrays Applied to Refractive Index Sensing. , 2016, Physical review letters.

[12]  P. Lalanne,et al.  Photonic and plasmonic nanoresonators: a modal approach , 2015, SPIE NanoScience + Engineering.

[13]  Alexander B. Yakovlev,et al.  Operator Theory for Electromagnetics , 2002 .

[14]  S Hughes,et al.  Generalized effective mode volume for leaky optical cavities. , 2012, Optics letters.

[15]  E. Muljarov,et al.  Resonant-state expansion of dispersive open optical systems: Creating gold from sand , 2015, 1510.01182.

[16]  Shanhui Fan,et al.  Temporal coupled-mode theory and the presence of non-orthogonal modes in lossless multimode cavities , 2004 .

[17]  C. V. Vishveshwara,et al.  Scattering of Gravitational Radiation by a Schwarzschild Black-hole , 1970, Nature.

[18]  David A. Powell,et al.  Resonant dynamics of arbitrarily shaped meta-atoms , 2014, 1405.3759.

[19]  R. Ge,et al.  Design of an efficient single photon source from a metallic nanorod dimer: a quasi-normal mode finite-difference time-domain approach. , 2014, Optics letters.

[20]  Andrew G. Glen,et al.  APPL , 2001 .

[21]  R. W. Christy,et al.  Optical Constants of the Noble Metals , 1972 .

[22]  Philippe Lalanne,et al.  Modal Analysis of the Ultrafast Dynamics of Optical Nanoresonators , 2017 .

[23]  Philippe Lalanne,et al.  Light Interaction with Photonic and Plasmonic Resonances , 2017, Laser & Photonics Reviews.

[24]  S. E. Mirnia,et al.  Fano resonance on plasmonic nanostructures , 2012, 2012 IEEE 3rd International Conference on Photonics.

[25]  David A. Powell,et al.  Interference between the modes of an all-dielectric meta-atom , 2016, 1610.04980.

[26]  Karl Meerbergen,et al.  The Quadratic Eigenvalue Problem , 2001, SIAM Rev..

[27]  E. Muljarov,et al.  Brillouin-Wigner perturbation theory in open electromagnetic systems , 2010, 1205.4924.

[28]  D. Bergman,et al.  Coherent control of femtosecond energy localization in nanosystems. , 2002, Physical review letters.

[29]  H. Haus,et al.  Coupled-mode theory , 1991, Proc. IEEE.

[30]  K. Drexhage,et al.  IV Interaction of Light with Monomolecular Dye Layers , 1974 .

[31]  Zach DeVito,et al.  Opt , 2017 .

[32]  Harald Giessen,et al.  Simple analytical expression for the peak-frequency shifts of plasmonic resonances for sensing. , 2015, Nano letters.

[33]  Nicolò Accanto,et al.  Ultrafast meets ultrasmall: controlling nanoantennas and molecules , 2016 .

[34]  Frank Olyslager Discretization of Continuous Spectra Based on Perfectly Matched Layers , 2004, SIAM J. Appl. Math..

[35]  A. Siegert On the Derivation of the Dispersion Formula for Nuclear Reactions , 1939 .

[36]  E. Muljarov,et al.  Exact mode volume and Purcell factor of open optical systems , 2014, 1409.6877.

[38]  A Taflove,et al.  Direct time integration of Maxwell's equations in linear dispersive media with absorption for scattering and propagation of femtosecond electromagnetic pulses. , 1991, Optics letters.

[39]  Young,et al.  Completeness and orthogonality of quasinormal modes in leaky optical cavities. , 1994, Physical review. A, Atomic, molecular, and optical physics.

[40]  Carl E. Baum,et al.  On the Singularity Expansion Method for the Solution of Electromagnetic Interaction Problems , 1971 .

[41]  P Lalanne,et al.  Theory of the spontaneous optical emission of nanosize photonic and plasmon resonators. , 2013, Physical review letters.

[42]  Xuezhi Zheng,et al.  Line Position and Quality Factor of Plasmonic Resonances Beyond the Quasi-Static Limit: A Full-Wave Eigenmode Analysis Route , 2013, IEEE Journal of Selected Topics in Quantum Electronics.

[43]  Richard M. More,et al.  Properties of Resonance Wave Functions , 1973 .

[44]  Philippe Lalanne,et al.  Near-to-Far Field Transformations for Radiative and Guided Waves , 2016 .

[45]  K. Pang,et al.  Dyadic formulation of morphology-dependent resonances. I. Completeness relation , 1999 .

[46]  Young,et al.  Completeness and time-independent perturbation of the quasinormal modes of an absorptive and leaky cavity. , 1994, Physical Review A. Atomic, Molecular, and Optical Physics.

[47]  L. Novotný,et al.  Enhancement and quenching of single-molecule fluorescence. , 2006, Physical review letters.

[48]  G. Miano,et al.  Analysis of dynamics of excitation and dephasing of plasmon resonance modes in nanoparticles. , 2007, Physical review letters.

[49]  N. Moiseyev,et al.  Non-Hermitian Quantum Mechanics: Frontmatter , 2011 .