Transport, vertical structure and radiative properties of dust events in southeast China determined from ground and space sensors

Two dust events were detected over the Yangtze Delta region of China during March 14e17 and April 25e26 in 2009 where such dust events are uncommon. The transport behavior, spatio-temporal evolution, vertical structure, direct radiative effects, as well as induced heating rates, are investigated using a combination of ground-based and satellite-based measurements, a back-trajectory analysis, an aerosol model and a radiative transfer model. Back-trajectories, wind fields and aerosol model analyses show that the first dust originated in northern/northwestern China and the second generated in the Taklimakan desert in northwest China, and traveled across the Hexi corridor and Loess Plateau to the Yangtze Delta region (the so-called “dust corridor”). The mean lidar extinction-to-backscatter ratio (LR) during the two dust events was 38.7 � 10.4 sr and 42.7 � 15.2 sr, respectively. The mean aerosol depolarization ratio ( da )f or thefirst dust event was 0.16 � 0.07, with a maximum value of 0.32. For the second, the mean da was around 0.19 � 0.06, with a maximum value of 0.29. Aerosol extinction coefficient and da profiles for the two events were similar: two aerosol layers consisting of dust aerosols and a mixture of dust and anthropogenic pollution aerosols. The topmost aerosol layer is above 3.5 km. The maximum mean aerosol extinction coefficients were 0.5 km �1 and 0.54 km �1 at about 0.7 km and 1.1 km, respectively. Significant effects of cooling at the surface and heating in the atmosphere were found during these dust events. Diurnal mean shortwave radiative forcings (efficiencies) at the surface, the top-of-the-atmosphere and within the atmosphere were � 36.8 (� 80.0), � 13.6 (� 29.6) and 23.2 (50.4) Wm �2 , respectively, during the first dust event, and � 48.2 (� 70.9), � 21.4 (� 31.5) and 26.8 (39.4) Wm �2 , respectively, during the second dust event. Maximum heating rates occurred at 0.7 km during the first dust event and at 1.1 km during the second dust event, with a maximum value of 2.74 K day �1 for each

[1]  Chan Bong Park,et al.  Measurement of Asian dust by using multiwavelength lidar , 2001, SPIE Asia-Pacific Remote Sensing.

[2]  Zhaoyan Liu,et al.  Observation of Aerosols and Clouds Using a Two-Wavelength Polarization Lidar during the Nauru99 Experiment , 2000 .

[3]  A. da Silva,et al.  Quantification of dust-forced heating of the lower troposphere , 1998, Nature.

[4]  Rachel T. Pinker,et al.  Aerosol radiative forcing during dust events over New Delhi, India , 2008 .

[5]  R. Betts,et al.  Changes in Atmospheric Constituents and in Radiative Forcing. Chapter 2 , 2007 .

[6]  P. Formenti,et al.  Variability of aerosol vertical distribution in the Sahel , 2010 .

[7]  Qiang Fu,et al.  Dust aerosol vertical structure measurements using three MPL lidars during 2008 China-U.S. joint dust field experiment , 2010, Journal of Geophysical Research.

[8]  B. Holben,et al.  Preface to special section on East Asian Studies of Tropospheric Aerosols: An International Regional Experiment (EAST‐AIRE) , 2007 .

[9]  A. Adriani,et al.  Comparison of various linear depolarization parameters measured by lidar. , 1999, Applied optics.

[10]  Albert Ansmann,et al.  Particle backscatter, extinction, and lidar ratio profiling with Raman lidar in south and north China. , 2007, Applied optics.

[11]  Hiroaki Kuze,et al.  An intercomparison of lidar‐derived aerosol optical properties with airborne measurements near Tokyo during ACE‐Asia , 2003 .

[12]  Detlef Müller,et al.  Seasonal characteristics of lidar ratios measured with a Raman lidar at Gwangju, Korea in spring and autumn , 2008 .

[13]  Remo Guidieri Res , 1995, RES: Anthropology and Aesthetics.

[14]  Chih-Wei Chiang,et al.  Lidar measurements of Asian dust storms and dust cloud interactions , 2007 .

[15]  NOTES AND CORRESPONDENCE Micropulse Lidar Signals: Uncertainty Analysis , 2002 .

[16]  Takashi Shibata,et al.  Case study of Raman lidar measurements of Asian dust events in 2000 and 2001 at Nagoya and Tsukuba, Japan , 2002 .

[17]  P. Levelt,et al.  Aerosols and surface UV products from Ozone Monitoring Instrument observations: An overview , 2007 .

[18]  F. Valero,et al.  Surface aerosol radiative forcing at Gosan during the ACE‐Asia campaign , 2003 .

[19]  A. Smirnov,et al.  AERONET-a federated instrument network and data archive for aerosol Characterization , 1998 .

[20]  Sang Woo Kim,et al.  Estimation of the radiative forcing by key aerosol types in worldwide locations using a column model and AERONET data , 2005 .

[21]  T. Eck,et al.  Variability of Absorption and Optical Properties of Key Aerosol Types Observed in Worldwide Locations , 2002 .

[22]  Chung-te Lee,et al.  Aerosol characteristics from the Taiwan aerosol supersite in the Asian yellow-dust periods of 2002 , 2006 .

[23]  Chih-Wei Chiang,et al.  An iterative calculation to derive extinction-to-backscatter ratio based on lidar measurements , 2008 .

[24]  S. Hsu,et al.  Southeastward Transport of Asian Dust: Source, Transport and its Contributions to Taiwan , 2009 .

[25]  James R. Johnson,et al.  Lidar measurements during Aerosols99 , 2001 .

[26]  F. Valero,et al.  Spectral aerosol radiative forcing at the surface during the Indian Ocean Experiment (INDOEX) , 2002 .

[27]  James D. Spinhirne,et al.  Compact Eye Safe Lidar Systems , 1995 .

[28]  Alexander Smirnov,et al.  Ground-Based Lidar Measurements of Aerosols During ACE-2 Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements , 2000 .

[29]  Albert Mendoza,et al.  Novel polarization-sensitive micropulse lidar measurement technique. , 2007, Optics express.

[30]  Patrick Chazette,et al.  Radiative budget in the presence of multi-layered aerosol structures in the framework of AMMA SOP-0 , 2008 .

[31]  G. McFarquhar,et al.  Effects of aerosols on trade wind cumuli over the Indian Ocean: Model simulations , 2006 .

[32]  Tianliang Zhao,et al.  Long range trans-Pacific transport and deposition of Asian dust aerosols. , 2008, Journal of environmental sciences.

[33]  K. O. Ogunjobi,et al.  Aerosol characteristics and surface radiative forcing components during a dust outbreak in Gwangju, Republic of Korea , 2008, Environmental monitoring and assessment.

[34]  K. Liou,et al.  Surface aerosol radiative forcing derived from collocated ground-based radiometric observations during PRIDE, SAFARI, and ACE-Asia. , 2003, Applied optics.

[35]  Soon-Chang Yoon,et al.  Asian dust event observed in Seoul, Korea, during 29-31 May 2008: analysis of transport and vertical distribution of dust particles from lidar and surface measurements. , 2010, The Science of the total environment.

[36]  Giorgio Fiocco,et al.  Influence of the vertical profile of Saharan dust on the visible direct radiative forcing , 2005 .

[37]  David D. Turner,et al.  Full-Time, Eye-Safe Cloud and Aerosol Lidar Observation at Atmospheric Radiation Measurement Program Sites: Instruments and Data Analysis , 2013 .

[38]  D. Winker,et al.  A height resolved global view of dust aerosols from the first year CALIPSO lidar measurements , 2008 .

[39]  Yan Yin,et al.  East Asian Studies of Tropospheric Aerosols and their Impact on Regional Climate (EAST‐AIRC): An overview , 2011 .

[40]  M. V. Ramana,et al.  Warming trends in Asia amplified by brown cloud solar absorption , 2007, Nature.

[41]  Oleg Dubovik,et al.  Global aerosol optical properties and application to Moderate Resolution Imaging Spectroradiometer aerosol retrieval over land , 2007 .

[42]  David S. Covert,et al.  Variability of aerosol optical properties derived from in situ aircraft measurements during ACE‐Asia , 2003 .

[43]  S. K. Satheesh,et al.  Impact of dust aerosols on Earth–atmosphere clear‐sky albedo and its short wave radiative forcing over African and Arabian regions , 2006 .

[44]  W. Hao,et al.  First observation‐based estimates of cloud‐free aerosol radiative forcing across China , 2010 .

[45]  Chih-Wei Chiang,et al.  Lidar depolarization measurements for aerosol source and property studies over Chungli (24.58° N, 121.1° E) , 2008 .

[46]  Sang Woo Kim,et al.  Estimation of Direct Radiative Forcing of Asian Dust Aerosols with Sun/Sky Radiometer and Lidar Measurements at Gosan, Korea , 2004 .

[47]  Ellsworth J. Welton,et al.  Measurements of aerosol vertical profiles and optical properties during INDOEX 1999 using micropulse lidars , 2002 .

[48]  Nobuo Sugimoto,et al.  Continuous observations of Asian dust and other aerosols by polarization lidars in China and Japan during ACE-Asia , 2004 .

[49]  D. Winker,et al.  Initial performance assessment of CALIOP , 2007 .

[50]  Xiangao Xia,et al.  Aerosol optical properties and radiative effects in the Yangtze Delta region of China , 2007, Journal of Geophysical Research.

[51]  D. Winker,et al.  Effective lidar ratios of dense dust layers over North Africa derived from the CALIOP measurements , 2011 .

[52]  F. G. Fernald Analysis of atmospheric lidar observations: some comments. , 1984, Applied optics.

[53]  Catherine Gautier,et al.  SBDART: A Research and Teaching Software Tool for Plane-Parallel Radiative Transfer in the Earth's Atmosphere. , 1998 .

[54]  Zhanqing Li,et al.  Seasonal statistical characteristics of aerosol optical properties at a site near a dust region in China , 2008 .

[55]  A. Ansmann,et al.  Aerosol-type-dependent lidar ratios observed with Raman lidar , 2007 .

[56]  Patrick Minnis,et al.  Long-range transport and vertical structure of Asian dust from CALIPSO and surface measurements during PACDEX , 2008 .

[57]  Zhaoyan Liu,et al.  Extinction-to-backscatter ratio of Asian dust observed with high-spectral-resolution lidar and Raman lidar. , 2002, Applied optics.

[58]  H. Gadhavi,et al.  Airborne lidar study of the vertical distribution of aerosols over Hyderabad, an urban site in central India, and its implication for radiative forcing calculations , 2006 .