Storage-stable styrene-butadiene-styrene triblock copolymer (SBS)-modified asphalt was prepared by dynamic vulcanization. The vulcanization characteristics of the asphalt/SBS/sulfur blend were studied using a strain-controlled rheometer. The vulcanization of SBS in the asphalt resulted in a marked increase in the torque of the blend. In addition, the vulcanization of a butadiene rubber (BR)/sulfur blend was significantly influenced by the addition of asphalt through a curemeter. The existence of asphalt can accelerate the vulcanization of BR/sulfur blend and reduce its reversion. The preparation process of storage-stable SBS-modified asphalt by dynamic vulcanization was identified by a plot of the electric current versus time. The addition of sulfur to the SBS-modified asphalts resulted in the formation of chemically vulcanized network structures in the modified binders. The physical properties of the SBS-modified asphalt containing sulfur were compared to those of the modified binders without sulfur. The storage stability of the SBS-modified asphalt was effectively improved by the addition of sulfur. The rheological properties of the SBS-modified asphalts before and after adding sulfur were characterized by using dynamic shear rheometry and a rotational viscometer. As indicated by the monitored morphology, the compatibility and high-temperature storage stability of SBS-modified asphalts were improved by the addition of sulfur.
[1]
A. Coran.
Vulcanization: Conventional and Dynamic
,
1995
.
[2]
Y. Shahab,et al.
MODIFICATION OF ASPHALT BY CHEMICAL TREATMENT WITH SULPHUR
,
1994
.
[3]
J. L. Koenig,et al.
A review of sulfur crosslinking fundamentals for accelerated and unaccelerated vulcanization
,
1993
.
[4]
Xiaohu Lu,et al.
Rheological characterization of styrene-butadiene-styrene copolymer modified bitumens
,
1997
.
[5]
Carlo Giavarini,et al.
REACTION OF VISBREAKER BITUMENS WITH SULFUR
,
1997
.
[6]
Xiaohu Lu,et al.
Influence of styrene-butadiene-styrene polymer modification on bitumen viscosity
,
1997
.
[7]
L. H. Lewandowski,et al.
Polymer Modification of Paving Asphalt Binders
,
1994
.
[8]
N. J. Morrison,et al.
Temperature Effects on the Stability of Intermediates and Crosslinks in Sulfur Vulcanization
,
1984
.