THE LOS ANGELES INTERNATIONAL AIRPORT AS A SOURCE OF ULTRAFINE PARTICLES AND OTHER POLLUTANTS TO NEARBY COMMUNITIES

Abstract Air monitoring was performed in the vicinity of the Los Angeles International Airport (LAX) during the spring of 2003. The purpose of this monitoring was to determine the extent of airport emissions on downwind ambient air in a mixed use neighborhood that includes residences. A mobile air monitoring platform was developed and deployed to measure ultrafine particle numbers (UFP), size distributions, particle length, black carbon (BC), oxides of nitrogen (NOx), and particle-phase polycyclic aromatic hydrocarbons (PM-PAH). Pollutant levels were low at a coastal site upwind of the airport, with UFP ranging between 580 and 3800 counts cm−3, oxides of nitrogen (NOx) from 4 to 22 ppb, black carbon from 0.2 to 0.6 μg m−3, and PM-PAH ranged from 18 to 36 ng m−3. Markedly higher UFP counts, with average counts of approximately 50,000 cm−3, were observed at a site 500 m downwind of the airport, which was strongly influenced by aircraft landings and where the community interfaced with airport facilities. Black carbon, PM-PAH, and NOx levels were elevated to a lesser extent at downwind locations. Transient peaks in UFP corresponding to aircraft landings and takeoffs were evident. A maximum UFP count reached 4.8 million particles cm−3 downwind of a runway used by jet aircraft for takeoffs. Particle size distributions differed substantially between upwind and downwind locations. The particle numbers at the upwind site were dominated by particles of approximately 90 nm diameter while downwind sites were dominated by particles peaking at approximately 10–15 nm. Additional data obtained from a study of UFP levels conducted subsequently by a co-author indicates that aircraft-generated UFP persist up to 900 m from an LAX runway [Biswas, S., Fine, P.M., Geller, M.D., Hering, S.V., Sioutas, C., 2005. Performance evaluation of a recently developed water-based condensation particle counter. Aerosol Science and Technology 39, 419–427]. Considered together, these observations suggest that airport operations are associated with elevated levels of UFP much further downwind in the neighboring community than would have been predicted by prior studies of UFP from roadway-traffic.

[1]  H. Burtscher,et al.  In situ measurement of adsorption and condensation of a polyaromatic hydrocarbon on ultrafine C particles by means of photoemission , 1986 .

[2]  Ernest Weingartner,et al.  Fine and ultrafine particles in the Zürich (Switzerland) area measured with a mobile laboratory: an assessment of the seasonal and regional variation throughout a year , 2003 .

[3]  Richard C. Flagan,et al.  Scanning Electrical Mobility Spectrometer , 1989 .

[4]  J D Spengler,et al.  Respiratory health and PM10 pollution. A daily time series analysis. , 1991, The American review of respiratory disease.

[5]  M F Hoylaerts,et al.  Passage of intratracheally instilled ultrafine particles from the lung into the systemic circulation in hamster. , 2001, American journal of respiratory and critical care medicine.

[6]  G. Oberdörster,et al.  Pulmonary effects of inhaled ultrafine particles , 2000, International archives of occupational and environmental health.

[7]  M. Johnson,et al.  Development of techniques to characterize particulates emitted from gas turbine exhausts , 2003 .

[8]  M. Utell,et al.  Acute health effects of ambient air pollution: the ultrafine particle hypothesis. , 2000, Journal of aerosol medicine : the official journal of the International Society for Aerosols in Medicine.

[9]  P. Hopke,et al.  On-Road Exposure to Highway Aerosols. 1. Aerosol and Gas Measurements , 2004, Inhalation toxicology.

[10]  Pasi Aalto,et al.  Aerosol Particle Number Concentration Measurements in Five European Cities Using TSI-3022 Condensation Particle Counter over a Three-Year Period during Health Effects of Air Pollution on Susceptible Subpopulations , 2005, Journal of the Air & Waste Management Association.

[11]  Scott Fruin,et al.  Mobile platform measurements of ultrafine particles and associated pollutant concentrations on freeways and residential streets in Los Angeles , 2005 .

[12]  M. Green Air pollution and health , 1995 .

[13]  Yifang Zhu,et al.  Penetration of freeway ultrafine particles into indoor environments , 2005 .

[14]  R. Burnett,et al.  Lung cancer, cardiopulmonary mortality, and long-term exposure to fine particulate air pollution. , 2002, JAMA.

[15]  Y. Moriguchi,et al.  Size Distribution and Characterization of Ultrafine Particles in Roadside Atmosphere , 2004, Journal of environmental science and health. Part A, Toxic/hazardous substances & environmental engineering.

[16]  Yifang Zhu,et al.  Concentration and Size Distribution of Ultrafine Particles Near a Major Highway , 2002, Journal of the Air & Waste Management Association.

[17]  D. Dockery,et al.  Epidemiologic evidence of cardiovascular effects of particulate air pollution. , 2001, Environmental health perspectives.

[18]  B. Wehner,et al.  Particle number size distributions in a street canyon and their transformation into the urban-air background: measurements and a simple model study , 2002 .

[19]  David Y. H. Pui,et al.  Use of Continuous Measurements of Integral Aerosol Parameters to Estimate Particle Surface Area , 2001 .

[20]  T. Novakov,et al.  The aethalometer — An instrument for the real-time measurement of optical absorption by aerosol particles , 1983 .

[21]  Robert C. Brown,et al.  Effect of aircraft exhaust sulfur emissions on near field plume aerosols , 1996 .

[22]  R. Burnett,et al.  Spatial Analysis of Air Pollution and Mortality in Los Angeles , 2005, Epidemiology.

[23]  J. Pleil,et al.  Real-time and integrated measurement of potential human exposure to particle-bound polycyclic aromatic hydrocarbons (PAHs) from aircraft exhaust. , 2000, Environmental health perspectives.

[24]  韓國航空大學 航空 械工學科 美聯邦航空廳(Federal Aviation Administration)의 航空機 製作檢査 制度의 現況 , 1979 .

[25]  H. Saxe,et al.  Air pollution from ships in three Danish ports , 2004 .

[26]  S. Hering,et al.  Performance Evaluation of a Recently Developed Water-Based Condensation Particle Counter , 2005 .

[27]  Daniel Wang,et al.  Identification and characterization of inland ship plumes over Vancouver, BC , 2006 .

[28]  Lidia Morawska,et al.  Concentrations of submicrometre particles from vehicle emissions near a major road , 2000 .

[29]  T. F. Lyon,et al.  Chemical composition and photochemical reactivity of exhaust from aircraft turbine engines , 1994 .

[30]  D. Weisenstein,et al.  A unified model for ultrafine aircraft particle emissions , 2000 .

[31]  R. Turco,et al.  The formation and evolution of aerosols in stratospheric aircraft plumes: Numerical simulations and comparisons with observations , 1998 .

[32]  Constantinos Sioutas,et al.  Seasonal and spatial trends in particle number concentrations and size distributions at the children's health study sites in Southern California , 2006, Journal of Exposure Science and Environmental Epidemiology.

[33]  Sara Janhäll,et al.  Roadside measurements of fine and ultrafine particles at a major road north of Gothenburg , 2002 .

[34]  Richard C. Miake-Lye,et al.  Particulate Emissions from in-use Commercial Aircraft , 2005 .

[35]  Kevin J. Hughes,et al.  Particle emissions from aircraft engines - a survey of the European project PartEmis , 2005 .

[36]  Liisa Pirjola,et al.  “Sniffer”—a novel tool for chasing vehicles and measuring traffic pollutants , 2004 .

[37]  Reinhold Busen,et al.  Jet engine exhaust chemiion measurements: Implications for gaseous SO3 and H2SO4 , 1998 .

[38]  Jugal K. Agarwal,et al.  Continuous flow, single-particle-counting condensation nucleus counter , 1980 .