Kondo effect in an integer-spin quantum dot

The Kondo effect—a many-body phenomenon in condensed-matter physics involving the interaction between a localized spin and free electrons—was discovered in metals containing small amounts of magnetic impurities, although it is now recognized to be of fundamental importance in a wide class of correlated electron systems. In fabricated structures, the control of single, localized spins is of technological relevance for nanoscale electronics. Experiments have already demonstrated artificial realizations of isolated magnetic impurities at metallic surfaces, nanoscale magnets, controlled transitions between two-electron singlet and triplet states, and a tunable Kondo effect in semiconductor quantum dots. Here we report an unexpected Kondo effect in a few-electron quantum dot containing singlet and triplet spin states, whose energy difference can be tuned with a magnetic field. We observe the effect for an even number of electrons, when the singlet and triplet states are degenerate. The characteristic energy scale is much larger than in the ordinary spin-1/2 case.

[1]  N. Wingreen,et al.  Tunneling into a single magnetic atom: spectroscopic evidence of the kondo resonance , 1998, Science.

[2]  Michel Devoret,et al.  Single Charge Tunneling , 1992 .

[3]  B. Delley,et al.  Kondo Scattering Observed at a Single Magnetic Impurity , 1998 .

[4]  D. Cox,et al.  Electronic Pairing in Exotic Superconductors , 1995 .

[5]  Direct coulomb and exchange interaction in artificial atoms , 2000, Physical review letters.

[6]  D. Kern,et al.  Spectroscopy, Electron-Electron Interaction, and Level Statistics in a Disordered Quantum Dot , 1994 .

[7]  A. Hewson,et al.  The Kondo Problem to Heavy Fermions by Alexander Cyril Hewson , 1993 .

[8]  T. Ng,et al.  On-site Coulomb repulsion and resonant tunneling. , 1988, Physical review letters.

[9]  Kouwenhoven,et al.  A tunable kondo effect in quantum dots , 1998, Science.

[10]  Suppression of the Kondo effect in quantum dots by even-odd asymmetry. , 1994, Physical review. B, Condensed matter.

[11]  Paul L. McEuen,et al.  Electron Transport in Quantum Dots , 1997 .

[12]  Yasuhiro Funabashi,et al.  Phase Relaxation and Non-Equilibrium Transport Properties through Multilevel Quantum Dot , 1999 .

[13]  Meir,et al.  Anderson model out of equilibrium: Noncrossing-approximation approach to transport through a quantum dot. , 1994, Physical review. B, Condensed matter.

[14]  M. Springford The Kondo problem to heavy fermions , 1993 .

[15]  The Kondo effect in single-electron transistor , 1998 .

[16]  K. Klitzing,et al.  A quantum dot in the limit of strong coupling to reservoirs , 1998 .

[17]  Kondo Effect in Single Quantum Dot Systems — Study with Numerical Renormalization Group Method — , 1998, cond-mat/9805067.

[18]  Alex C. Hewson,et al.  The Kondo Problem to Heavy Fermions , 1993 .

[19]  Shimizu,et al.  Correlated electron transport through a quantum dot: The multiple-level effect. , 1993, Physical review. B, Condensed matter.

[20]  P. Nozières,et al.  Kondo effect in real metals , 1980 .

[21]  L. Sohn,et al.  Mesoscopic electron transport , 1997 .

[22]  K. Eberl,et al.  Absence of odd-even parity behavior for Kondo resonances in quantum dots. , 2000, Physical review letters.

[23]  D. Mattis Symmetry of Ground State in a Dilute Magnetic Metal Alloy , 1967 .

[24]  M. Manninen,et al.  Ellipsoidal deformation of vertical quantum dots , 1999, cond-mat/9905135.

[25]  D. DiVincenzo,et al.  Quantum computation with quantum dots , 1997, cond-mat/9701055.

[26]  David P. DiVincenzo,et al.  Complex dynamics of mesoscopic magnets , 1995 .

[27]  L. Glazman,et al.  Resonant Kondo transparency of a barrier with quasilocal impurity states , 1988 .