CURRENT UNCERTAINTIES IN ASSESSING AEROSOL EFFECTS ON CLIMATE

▪ Abstract The effect of anthropogenic emissions from activities, such as fossil-fuel, biomass, and biofuel burning; transportation; and land-clearing; have a profound impact on the climate system. The impact of these activities is manifested in observed changes in temperature, precipitation, sea-level rise, melting of glaciers, air quality, health, and agriculture yields, to name a few. The obvious question to ask is the role that these different processes play in affecting climate and what action could one impose to curtail or constrain adverse human impacts on climate. Greenhouse gases have long been studied, as they play a major role in changing climate. But over the past 10–20 years, aerosols have emerged as the other big contenders in climate change studies. This review focuses on the current understanding of the effects of aerosols on climate, with an emphasis on the thermodynamical and indirect aerosol effects. We also examine available measurements that could be used to decipher the aerosol influ...

[1]  Dana E. Veron,et al.  First measurements of the Twomey indirect effect using ground‐based remote sensors , 2003 .

[2]  V. Ramanathan,et al.  South Asian Haze Forcing: Remote Impacts with Implications to ENSO and AO , 2003 .

[3]  Reto Knutti,et al.  Constraints on radiative forcing and future climate change from observations and climate model ensembles , 2002, Nature.

[4]  S. Menon,et al.  Role of sulfate aerosols in modifying the cloud albedo: a closure experiment , 2002 .

[5]  Harshvardhan,et al.  Influence of anthropogenic aerosol on cloud optical depth and albedo shown by satellite measurements and chemical transport modeling , 2002, Proceedings of the National Academy of Sciences of the United States of America.

[6]  Alexander Smirnov,et al.  High aerosol optical depth biomass burning events: A comparison of optical properties for different source regions , 2003 .

[7]  Joyce E. Penner Comment on “Control of fossil-fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming” by M. Z. Jacobson: COMMENTARY , 2003 .

[8]  Qun Xu,et al.  Abrupt change of the mid-summer climate in central east China by the influence of atmospheric pollution , 2001 .

[9]  V. Ramaswamy,et al.  Global sensitivity studies of the direct radiative forcing due to anthropogenic sulfate and black carbon aerosols , 1998 .

[10]  James G. Hudson,et al.  Evaluation of aerosol direct radiative forcing in MIRAGE , 2001 .

[11]  R. Welch,et al.  Global Survey of the Relationships of Cloud Albedo and Liquid Water Path with Droplet Size Using ISCCP , 1998 .

[12]  Cairns,et al.  Aerosol retrievals over the ocean using channel 1 and 2 AVHRR data: a sensitivity analysis and preliminary results , 2022 .

[13]  Michael Fromm,et al.  Transport of forest fire smoke above the tropopause by supercell convection , 2003 .

[14]  S. Menon,et al.  Role of sulfates in regional cloud–climate interactions 1 Paper was presented at the 12th International Conference on Clouds and Precipitation, Zurich, Switzerland, August 1996. 1 , 1998 .

[15]  Glenn E. Shaw,et al.  Indian Ocean Experiment: An integrated analysis of the climate forcing and effects of the great Indo-Asian haze , 2001 .

[16]  I. J. Ackermann,et al.  Comment on “Control of fossil-fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming” by M. Z. Jacobson: COMMENTARY , 2003 .

[17]  Andrei P. Sokolov,et al.  Quantifying Uncertainties in Climate System Properties with the Use of Recent Climate Observations , 2002, Science.

[18]  U. Lohmann,et al.  Comparing continental and oceanic cloud susceptibilities to aerosols , 2003 .

[19]  S. K. Satheesh,et al.  Large differences in tropical aerosol forcing at the top of the atmosphere and Earth's surface , 2000, Nature.

[20]  P. Daum,et al.  Anthropogenic aerosols: Indirect warming effect from dispersion forcing , 2002, Nature.

[21]  Lennart Bengtsson,et al.  Transient Climate Change Simulations with a Coupled Atmosphere–Ocean GCM Including the Tropospheric Sulfur Cycle , 1999 .

[22]  S. Twomey,et al.  Aerosols, clouds and radiation , 1991 .

[23]  Leon D. Rotstayn,et al.  Indirect forcing by anthropogenic aerosols: A global climate model calculation of the effective‐radius and cloud‐lifetime effects , 1999 .

[24]  V. Ramaswamy,et al.  A general circulation model study of the global carbonaceous aerosol distribution , 2002 .

[25]  Thomas W. Kirchstetter,et al.  Origin of carbonaceous aerosols over the tropical Indian Ocean: Biomass burning or fossil fuels? , 2000 .

[26]  K. Trenberth,et al.  Modern Global Climate Change , 2003, Science.

[27]  J. Houghton,et al.  Climate change 2001 : the scientific basis , 2001 .

[28]  F. Bréon,et al.  Aerosol Effect on Cloud Droplet Size Monitored from Satellite , 2002, Science.

[29]  P. J. Rasch,et al.  Radiative forcing due to sulfate aerosols from simulations with the National Center for Atmospheric Research Community Climate Model, Version 3 , 2000 .

[30]  L. Schüller,et al.  Retrieval of microphysical, geometrical, and radiative properties of marine stratocumulus from remote sensing , 2003 .

[31]  W. Cotton,et al.  Autoconversion rate bias in stratiform boundary layer cloud parameterizations , 2002 .

[32]  P. Chylek,et al.  Enhanced Absorption of Solar Radiation By Cloud Droplets Containing Soot Particles In Their Surface , 1992 .

[33]  J. Curry,et al.  Retrieval of cloud droplet size from visible and microwave radiometric measurements during INDOEX: Implication to aerosols' indirect radiative effect , 2003 .

[34]  D. Blake,et al.  Aerosols from biomass burning over the tropical South Atlantic region: Distributions and impacts , 1996 .

[35]  Teruyuki Nakajima,et al.  A possible correlation between satellite‐derived cloud and aerosol microphysical parameters , 2001 .

[36]  G. Myhre,et al.  Estimation of the direct radiative forcing due to sulfate and soot aerosols , 1998 .

[37]  J. Hansen,et al.  Trends of measured climate forcing agents , 2001, Proceedings of the National Academy of Sciences of the United States of America.

[38]  Estimation of the direct radiative forcing due to sulfate and soot aerosols , 1998 .

[39]  Graham Feingold,et al.  Explanation of discrepancies among satellite observations of the aerosol indirect effects , 2003 .

[40]  A. Jones,et al.  The response of the climate system to the indirect effects of anthropogenic sulfate aerosol , 2001 .

[41]  D. Koch Transport and direct radiative forcing of carbonaceous and sulfate aerosols in the GISS GCM , 2001 .

[42]  Yinon Rudich,et al.  Influence of the Kuwait oil fires plume (1991) on the microphysical development of clouds , 2003 .

[43]  Teruyuki Nakajima,et al.  A Study of the Aerosol Effect on a Cloud Field with Simultaneous Use of GCM Modeling and Satellite Observation , 2004 .

[44]  V. Ramanathan,et al.  Reduction of tropical cloudiness by soot , 2000, Science.

[45]  O. Boucher,et al.  A satellite view of aerosols in the climate system , 2002, Nature.

[46]  B. Holben,et al.  Baseline maritime aerosol: Methodology to Derive the optical thickness and scattering properties , 2001 .

[47]  Leon D. Rotstayn,et al.  Indirect Aerosol Forcing, Quasi Forcing, and Climate Response , 2001 .

[48]  F. Giorgi,et al.  Correlation between model‐calculated anthropogenic aerosols and satellite‐derived cloud optical depths: Indication of indirect effect? , 2002 .

[49]  C. N. Hewitt,et al.  The application of proton transfer reaction-mass spectrometry (PTR-MS) to the monitoring and analysis of volatile organic compounds in the atmosphere. , 2003, Journal of environmental monitoring : JEM.

[50]  C. Land,et al.  A Comparison of Model- and Satellite-Derived Aerosol Optical Depth and Reflectivity , 2002 .

[51]  J. Hansen,et al.  Global Warming Continues , 2002, Science.

[52]  Victor Brovkin,et al.  Assessing climate forcings of the Earth system for the past millennium , 2003 .

[53]  J. Hansen,et al.  Carbonaceous aerosols in the industrial era , 2004 .

[54]  J. Hansen,et al.  Large historical changes of fossil‐fuel black carbon aerosols , 2003 .

[55]  Makiko Sato,et al.  Global atmospheric black carbon inferred from AERONET , 2003, Proceedings of the National Academy of Sciences of the United States of America.

[56]  Joyce E. Penner,et al.  Indirect effect of sulfate and carbonaceous aerosols: A mechanistic treatment , 2000 .

[57]  G. Meehl Influence of the land surface in the Asian summer monsoon , 1994 .

[58]  D. Rosenfeld,et al.  Sensitivity of the global circulation to the suppression of precipitation by anthropogenic aerosols , 2003 .

[59]  Hanna Pawlowska,et al.  Cloud microphysical and radiative properties for parameterization and satellite monitoring of the indirect effect of aerosol on climate , 2003 .

[60]  Joyce E. Penner,et al.  Soot and smoke aerosol may not warm climate , 2002 .

[61]  Melanie A. Wetzel,et al.  Chemical and microphysical properties of marine stratiform cloud in the North Atlantic , 1998 .

[62]  Ulrike Lohmann,et al.  Impact of the Mount Pinatubo eruption on cirrus clouds formed by homogeneous freezing in the ECHAM4 GCM , 2003 .

[63]  George Tselioudis,et al.  GCM Simulations of the Aerosol Indirect Effect: Sensitivity to Cloud Parameterization and Aerosol Burden , 2002 .

[64]  R. Dickerson,et al.  Analysis of black carbon and carbon monoxide observed over the Indian Ocean: Implications for emissions and photochemistry , 2002 .

[65]  J. Hansen,et al.  Radiative forcing and climate response , 1997 .

[66]  D. Rosenfeld TRMM observed first direct evidence of smoke from forest fires inhibiting rainfall , 1999 .

[67]  A simple thermodynamic model for seasonal variation of monsoon rainfall , 2001 .

[68]  J. Seinfeld,et al.  Airborne measurements of atmospheric carbonaceous aerosols during ACE-Asia , 2002 .

[69]  H. Douville,et al.  Impact of CO2 doubling on the Asian summer monsoon: robust versus model-dependent responses , 2000 .

[70]  Yoram J. Kaufman,et al.  Analysis of smoke impact on clouds in Brazilian biomass burning regions: An extension of Twomey's approach , 2001 .

[71]  François-Marie Bréon,et al.  Cloud droplet effective radius from spaceborne polarization measurements , 1998 .

[72]  Sonoyo Mukai,et al.  A study of the direct and indirect effects of aerosols using global satellite data sets of aerosol and cloud parameters , 2003 .

[73]  Olga Khersonsky,et al.  Treating clouds with a grain of salt , 2002 .

[74]  U. Lohmann,et al.  Nonlinear Aspects of the Climate Response to Greenhouse Gas and Aerosol Forcing , 2004 .

[75]  Leon D. Rotstayn,et al.  Tropical Rainfall Trends and the Indirect Aerosol Effect , 2002 .

[76]  A. Salam,et al.  Aerosol chemical characteristics of an island site in the Bay of Bengal (Bhola-Bangladesh). , 2003, Journal of environmental monitoring : JEM.

[77]  L. Schüller,et al.  Radiative Properties of Boundary Layer Clouds: Droplet Effective Radius versus Number Concentration , 2000 .

[78]  J. Hansen,et al.  Climate Effects of Black Carbon Aerosols in China and India , 2002, Science.

[79]  U. Lohmann Possible Aerosol Effects on Ice Clouds via Contact Nucleation , 2002 .

[80]  J. Coakley,et al.  Limits to the Aerosol Indirect Radiative Effect Derived from Observations of Ship Tracks , 2002 .

[81]  Rosenfeld,et al.  Suppression of rain and snow by urban and industrial air pollution , 2000, Science.

[82]  M. Jacobson Control of fossil‐fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming , 2002 .

[83]  Yoram J. Kaufman,et al.  Will aerosol measurements from Terra and Aqua Polar Orbiting satellites represent the daily aerosol abundance and properties? , 2000 .

[84]  J. Hansen A Brighter Future , 2002 .

[85]  Toshiki Iwasaki,et al.  A Possible Link of Aerosol and Cloud Radiations to Asian Summer Monsoon and Its Implication in Long , 1998 .

[86]  Harshvardhan,et al.  Aerosol Influence on Cloud Microphysics Examined by Satellite Measurements and Chemical Transport Modeling , 2002 .

[87]  L. Gomes,et al.  Variability of aerosol size‐resolved composition at an Indian coastal site during the Indian Ocean Experiment (INDOEX) intensive field phase , 2003 .

[88]  J. Hansen,et al.  Soot climate forcing via snow and ice albedos. , 2004, Proceedings of the National Academy of Sciences of the United States of America.

[89]  Andrew S. Jones,et al.  Indirect sulphate aerosol forcing in a climate model with an interactive sulphur cycle , 2001 .

[90]  Leon D. Rotstayn,et al.  On the “tuning” of autoconversion parameterizations in climate models , 2000 .

[91]  J. Penner,et al.  Cloud susceptibility and the first aerosol indirect forcing: Sensitivity to black carbon and aerosol concentrations , 2002 .

[92]  M. Mishchenko,et al.  Retrieval of aerosol properties over the ocean using multispectral and multiangle Photopolarimetric measurements from the Research Scanning Polarimeter , 2001 .

[93]  T. Takemura,et al.  Significance of direct and indirect radiative forcings of aerosols in the East China Sea region , 2003 .

[94]  M. Jacobson A physically‐based treatment of elemental carbon optics: Implications for global direct forcing of aerosols , 2000 .

[95]  R. Welch,et al.  Near‐global survey of cloud column susceptibilities using ISCCP data , 2000 .

[96]  V. Ramanathan,et al.  Effects of the south Asian absorbing haze on the northeast monsoon and surface-air heat exchange , 2002 .

[97]  B. Albrecht Aerosols, Cloud Microphysics, and Fractional Cloudiness , 1989, Science.

[98]  A. Lacis,et al.  Aerosol retrievals over the ocean by use of channels 1 and 2 AVHRR data: sensitivity analysis and preliminary results. , 1999, Applied optics.

[99]  A. Salam,et al.  Aerosol chemical characteristics of a mega-city in Southeast Asia (Dhaka–Bangladesh) , 2003 .

[100]  Larry W. Thomason,et al.  Climate forcings in Goddard Institute for Space Studies SI2000 simulations , 2002 .

[101]  M. Wise,et al.  An integrated assessment of climate change and the accelerated introduction of advanced energy technologies , 1997 .

[102]  D. Streets,et al.  A technology‐based global inventory of black and organic carbon emissions from combustion , 2004 .

[103]  Qingyuan Han,et al.  Three Different Behaviors of Liquid Water Path of Water Clouds in Aerosol-Cloud Interactions , 2002 .

[104]  G. Carmichael,et al.  Biomass burning in Asia: Annual and seasonal estimates and atmospheric emissions , 2003 .

[105]  T. Kirchstetter,et al.  Carbonaceous aerosols over the Indian Ocean during the Indian Ocean Experiment (INDOEX): Chemical characterization, optical properties, and probable sources , 2002 .

[106]  O. Boucher,et al.  Estimates of the direct and indirect radiative forcing due to tropospheric aerosols: A review , 2000 .

[107]  S. Twomey The Influence of Pollution on the Shortwave Albedo of Clouds , 1977 .

[108]  Yoram J. Kaufman,et al.  Interannual variation of ambient aerosol characteristics on the east coast of the United States , 1999 .

[109]  Y. Kaufman,et al.  The effect of smoke particles on clouds and climate forcing , 1997 .

[110]  J. Coakley,et al.  Enhancement of cloud cover and suppression of nocturnal drizzle in stratocumulus polluted by haze , 2003 .

[111]  C. Timmreck,et al.  Impact of the Mt. Pinatubo eruption on cirrus clouds formed by homogeneous freezing in the ECHAM GCM , 2003 .

[112]  V. Ramanathan,et al.  Aerosols, Climate, and the Hydrological Cycle , 2001, Science.

[113]  Glen Lesins,et al.  Stronger Constraints on the Anthropogenic Indirect Aerosol Effect , 2002, Science.

[114]  Joyce E. Penner,et al.  Comment on “Control of fossil‐fuel particulate black carbon and organic matter, possibly the most effective method of slowing global warming” by M. Z. Jacobson , 2003 .

[115]  W. P. Ball,et al.  Characterization of carbonaceous aerosols outflow from India and Arabia: Biomass/biofuel burning and fossil fuel combustion , 2003 .

[116]  George A. Isaac,et al.  Physical and chemical observations in marine stratus during the 1993 North Atlantic Regional Experiment: Factors controlling cloud droplet number concentrations , 1996 .

[117]  Johannes Quaas,et al.  Evaluating aerosol//cloud//radiation process parameterizations with single-column models and Second Aerosol Characterization Experiment (ACE-2) cloudy column observations , 2003 .

[118]  R. M. Mitchell,et al.  Absorption feedback in stratocumulus clouds Influence on cloud top albedo , 1994 .

[119]  Alexander Khain,et al.  The Role of Sea Spray in Cleansing Air Pollution over Ocean via Cloud Processes , 2002, Science.