Single crystals of europium(III) scandate(III), with ideal formula EuScO3, were grown from the melt using the micro-pulling-down method. The title compound crystallizes in an orthorhombic distorted perovskite-type structure, where Eu occupies the eightfold coordinated A sites (site symmetry m) and Sc resides on the centres of corner-sharing [ScO6] octahedra (B sites with site symmetry ). The structure of EuScO3 has been reported previously based on powder diffraction data [Liferovich & Mitchell (2004). J. Solid State Chem. 177, 2188–2197]. The results of the current redetermination based on single-crystal diffraction data shows an improvement in the precision of the structral and geometric parameters and reveals a defect-type structure. Site-occupancy refinements indicate an Eu deficiency on the A site coupled with O defects on one of the two O-atom positions. The crystallochemical formula of the investigated sample may thus be written as A(□0.032Eu0.968)BScO2.952.
[1]
B. Veličkov,et al.
Crystal chemistry of GdScO3, DyScO3, SmScO3 and NdScO3
,
2007
.
[2]
R. Fornari,et al.
Dopant segregations in oxide single-crystal fibers grown by the micro-pulling-down method
,
2007
.
[3]
G. Sheldrick.
A short history of SHELX.
,
2008,
Acta crystallographica. Section A, Foundations of crystallography.
[4]
Yusheng Zhao,et al.
Thermal expansion and structural distortion of perovskite — data for NaMgF3 perovskite. Part I
,
1993
.
[5]
R. Mitchell,et al.
A structural study of ternary lanthanide orthoscandate perovskites
,
2004
.
[6]
R. Uecker,et al.
Redetermination of terbium scandate, revealing a defect-type perovskite derivative
,
2008,
Acta crystallographica. Section E, Structure reports online.