Secondary scintillation yield of Xenon with sub-percent levels of CO2 additive: efficiently reducing electron diffusion in HPXe optical TPCs for rare-event detection

We have measured the electroluminescence (EL) yield of Xe-CO2 mixtures, with sub-percent CO2 concentrations. We demonstrate that the EL production is still high in these mixtures, 70% and 35% relative to that produced in pure xenon, for CO2 concentrations around 0.05% and 0.1%, respectively. The contribution of the statistical fluctuations in EL production to the energy resolution increases with increasing CO2 concentration and, for our gas proportional scintillation counter, it is smaller than the contribution of the Fano factor for concentrations below 0.1% CO2. Xe-CO2 mixtures are important alternatives to pure xenon in TPCs based on EL signal amplification with applications in the important field of rare event detection such as directional dark matter, double electron capture and double beta decay detection. The addition of CO2 to pure xenon at the level of 0.05-0.1% can reduce significantly the scale of electron diffusion from 10 mm/sqrt(m) to 2.5 mm/sqrt(m), with high impact on the HPXe TPC discrimination efficiency of the events through pattern recognition of the topology of primary ionisation trails.

[1]  L. M. Moutinho,et al.  Microscopic simulation of xenon-based optical TPCs in the presence of molecular additives , 2017, 1705.09481.

[2]  L. M. Moutinho,et al.  Background rejection in NEXT using deep neural networks , 2016, 1609.06202.

[3]  F. V. Massoli,et al.  Search for two-neutrino double electron capture of 124 Xe with XENON100 , 2016, 1609.03354.

[4]  M. Decowski,et al.  Search for Majorana Neutrinos Near the Inverted Mass Hierarchy Region with KamLAND-Zen. , 2016, Physical review letters.

[5]  Pengwei Xie,et al.  Dark Matter Results from First 98.7 Days of Data from the PandaX-II Experiment. , 2016, Physical review letters.

[6]  M. K. Lee,et al.  Search for two-neutrino double electron capture on 124 Xe with the XMASS-I detector , 2015, 1510.00754.

[7]  J. Galan Microbulk MicrOMEGAs for the search of 0νββ of 136Xe in the PandaX-III experiment , 2015, 1512.09034.

[8]  A. Gangapshev,et al.  A technique for searching for the 2K capture in 124Xe with a copper proportional counter , 2015 .

[9]  L. M. Moutinho,et al.  Sensitivity of NEXT-100 to neutrinoless double beta decay , 2015, 1511.09246.

[10]  J. Gomez-Cadenas,et al.  An homeopathic cure to pure Xenon large diffusion , 2015, 1511.07189.

[11]  L. M. Moutinho,et al.  First proof of topological signature in the high pressure xenon gas TPC with electroluminescence amplification for the NEXT experiment , 2015, 1507.05902.

[12]  D. C. Herrera,et al.  Modelling the behaviour of microbulk Micromegas in xenon/trimethylamine gas , 2015, 1506.05077.

[13]  L. M. Moutinho,et al.  Accurate γ and MeV-electron track reconstruction with an ultra-low diffusion Xenon/TMA TPC at 10 atm , 2015, 1504.03678.

[14]  A. Para,et al.  Dark matter directionality revisited with a high pressure xenon gas detector , 2015, 1503.03937.

[15]  D. Tosi,et al.  An RF-only ion-funnel for extraction from high-pressure gases , 2014, 1412.1144.

[16]  L. M. Moutinho,et al.  Characterisation of NEXT-DEMO using xenon Kα X-rays , 2014, 1407.3966.

[17]  M. Weber,et al.  Search for Majorana neutrinos with the first two years of EXO-200 data , 2014, Nature.

[18]  R. Webb,et al.  First results from the LUX dark matter experiment at the Sanford underground research facility. , 2013, Physical review letters.

[19]  D. Nygren,et al.  Columnar recombination: a tool for nuclear recoil directional sensitivity in a xenon-based direct detection WIMP search , 2013 .

[20]  N. Yahlali,et al.  Operation and first results of the NEXT-DEMO prototype using a silicon photomultiplier tracking array , 2013, 1306.0471.

[21]  E Aprile,et al.  Dark matter results from 225 live days of XENON100 data. , 2012, Physical review letters.

[22]  L. Fernandes,et al.  Secondary scintillation yield from GEM and THGEM gaseous electron multipliers for direct dark matter search , 2012 .

[23]  I. Giomataris,et al.  Micromegas operation in high pressure xenon: charge and scintillation readout , 2010, 1009.2960.

[24]  T. Lux,et al.  Secondary scintillation yield in high-pressure xenon gas for neutrinoless double beta decay (0νββ) search , 2010 .

[25]  A. Breskin,et al.  Measurements of photoelectron extraction efficiency from CsI into mixtures of Ne with CH4, CF4, CO2 and N2 , 2009, 0909.2965.

[26]  A. Breskin,et al.  Secondary scintillation yield from gaseous micropattern electron multipliers in direct Dark Matter detection , 2009 .

[27]  J. Lopes,et al.  Secondary scintillation yield in pure argon , 2008 .

[28]  K. Giboni,et al.  Secondary scintillation yield in pure xenon , 2007, physics/0702142.

[29]  P. C. P. S. Sim,et al.  A new method for pulse analysis of driftless-gas proportional scintillation counters , 2003 .

[30]  C. Conde,et al.  Development of portable gas proportional scintillation counters for x-ray spectrometry , 2001 .

[31]  C. Conde,et al.  Driftless gas proportional scintillation counter pulse analysis using digital processing techniques , 2001 .

[32]  C. Conde,et al.  An argon gas proportional scintillation counter with UV avalanche photodiode scintillation readout , 2000, 2000 IEEE Nuclear Science Symposium. Conference Record (Cat. No.00CH37149).

[33]  C. Conde,et al.  A xenon gas proportional scintillation counter with a UV-sensitive large-area avalanche photodiode , 2000, 2000 IEEE Nuclear Science Symposium. Conference Record (Cat. No.00CH37149).

[34]  V. Morgunov,et al.  Low-Background Experiments with High Pressure Gas Scintillation Proportional Detector , 1997, physics/9704021.

[35]  C. Conde,et al.  Three-dimensional Monte Carlo calculation of the VUV electroluminescence and other electron transport parameters in xenon , 1994 .

[36]  Anthony J. Peacock,et al.  Fano factor implications from gas scintillation proportional counter measurements , 1989 .

[37]  D. Anderson,et al.  A large area, gas scintillation proportional counter , 1979 .