Attosecond control of ionization by wave-packet interference.

A train of attosecond pulses, synchronized to an infrared (IR) laser field, is used to create a series of electron wave packets (EWPs) that are below the ionization threshold in .helium. The ionization probability is found to strongly oscillate with the delay between the IR and attosecond fields twice per IR laser cycle. Calculations that reproduce the experimental results demonstrate that this ionization control results from interference between transiently bound EWPs created by different pulses in the train. In this way, we are able to observe, for the first time, attosecond wave-packet interference in a strongly driven atomic system.

[1]  P. Johnsson,et al.  Attosecond electron wave packet interferometry , 2006 .

[2]  E. Goulielmakis,et al.  Direct Measurement of Light Waves , 2004, Science.

[3]  Gallagher,et al.  Ramsey fringes in atomic Rydberg wave packets. , 1992, Physical review. A, Atomic, molecular, and optical physics.

[4]  Anders Persson,et al.  Amplitude and phase control of attosecond light pulses. , 2005, Physical review letters.

[5]  P. Balcou,et al.  Attosecond electron wave packet dynamics in strong laser fields. , 2005, Physical review letters.

[6]  U. Heinzmann,et al.  Time-resolved atomic inner-shell spectroscopy , 2002, Nature.

[7]  P. Balcou,et al.  Observation of a Train of Attosecond Pulses from High Harmonic Generation , 2001, Science.

[8]  Schafer,et al.  Energy analysis of time-dependent wave functions: Application to above-threshold ionization. , 1990, Physical review. A, Atomic, molecular, and optical physics.

[9]  K. Schafer,et al.  Time-Dependent Studies of Multiphoton Processes , 1992 .

[10]  Strong species dependence of high order photoelectron production in alkali metal atoms , 2000, Physical review letters.

[11]  Sheehy,et al.  Precision measurement of strong field double ionization of helium. , 1994, Physical review letters.

[12]  L. Poletto,et al.  Controlling attosecond electron dynamics by phase-stabilized polarization gating , 2006 .

[13]  P. Bucksbaum,et al.  Role of the ponderomotive potential in above-threshold ionization , 1987 .

[14]  David H. Parker,et al.  Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen , 1997 .

[15]  Andrew G. Glen,et al.  APPL , 2001 .

[16]  M. Vrakking An iterative procedure for the inversion of two-dimensional ion/photoelectron imaging experiments , 2001 .

[17]  H. G. Muller,et al.  Reconstruction of attosecond harmonic beating by interference of two-photon transitions , 2002 .

[18]  U. Kleineberg,et al.  Atomic transient recorder , 2004, Nature.

[19]  U. Kleineberg,et al.  Steering Attosecond Electron Wave Packets with Light , 2002, Science.

[20]  K. Kulander,et al.  Effective potentials for time-dependent calculations of multiphoton processes in atoms , 1991 .

[21]  Schafer,et al.  High-order harmonic generation from atoms and ions in the high intensity regime. , 1992, Physical review letters.

[22]  Ferenc Krausz,et al.  X-ray Pulses Approaching the Attosecond Frontier , 2001, Science.

[23]  Graham R. Fleming,et al.  Fluorescence‐detected wave packet interferometry: Time resolved molecular spectroscopy with sequences of femtosecond phase‐locked pulses , 1991 .