A spectral analysis of coronal Faraday rotation (FR) data obtained with the linearly polarized signals of the two Heliosspacecraft reveals that about one-third of the temporal FR spectra contain a distinct spectral line superposed onto the background power-law spectrum. The most prevalent frequency of this quasi-harmonic component (QHC) is about 4 mHz, corresponding to a 4–5 min periodic oscillation of the coronal magnetic field. Physical reasons for the existence of QHC Alfvén fluctuations in the inner solar wind are discussed. FR fluctuations (FRF) are considered to arise from both a turbulent background as well as an isolated Alfvén wave train of finite extent and duration. An estimate can be made for the conditions under which the isolated wave train is observed above the ever present background. It is shown that the wave train must have a sufficiently long duration and transverse wavelength. It is suggested that the QHC at periods near 4–5 min in the FRF spectra are most probably produced by outward-propagating Alfvén waves excited initially in the anisotropic structures of the chromospheric network.