Impact of excess NOx emissions from diesel cars on air quality, public health and eutrophication in Europe

Diesel cars have been emitting four to seven times more NOx in on-road driving than in type approval tests. These 'excess emissions' are a consequence of deliberate design of the vehicle's after-treatment system, as investigations during the 'Dieselgate' scandal have revealed. Here we calculate health and environmental impacts of these excess NOx emissions in all European countries for the year 2013. We use national emissions reported officially under the UNECE Convention for Long-range Transport of Atmospheric Pollutants and employ the EMEP MSC-W Chemistry Transport Model and the GAINS Integrated AssessmentModel to determine atmospheric concentrations and resulting impacts. We compare with impacts from hypothetical emissions where light duty diesel vehicles are assumed to emit only as much as their respective type approval limit value or as little as petrol cars of the same age. Excess NO2 concentrations can also have direct health impacts, but these overlap with the impacts from particulate matter ( PM) and are not included here. We estimate that almost 10 000 premature deaths from PM2.5 and ozone in the adult population (age>30 years) can be attributed to the NOx emissions from diesel cars and light commercial vehicles in EU28 plus Norway and Switzerland in 2013. About 50% of these could have been avoided if diesel limits had been achieved also in on-road driving; and had diesel cars emitted as little NOx as petrol cars, 80% of these premature deaths could have been avoided. Ecosystem eutrophication impacts (critical load exceedances) from the same diesel vehicles would also have been reduced at similar rates as for the health effects.

[1]  P. Thunis,et al.  Modelling NO 2 concentrations at the street level in the GAINS integrated assessment model: projections under current legislation , 2013 .

[2]  T. Borsdorff,et al.  Carbon monoxide (CO) and ethane (C2H6) trends from ground-based solar FTIR measurements at six European stations, comparison and sensitivity analysis with the EMEP model , 2011 .

[3]  G. Kadijk,et al.  Determination of Dutch NOx emission factors for Euro-5 diesel passenger cars , 2012 .

[4]  D. Simpson,et al.  Improving the spatial resolution of air-quality modelling at a European scale – development and evaluation of the Air Quality Re-gridder Model (AQR v1.1) , 2016 .

[5]  Bart Degraeuwe,et al.  Impact of passenger car NOx emissions and NO2 fractions on urban NO2 pollution – Scenario analysis for the city of Antwerp, Belgium , 2016 .

[6]  Michael Schulz,et al.  A multi-model analysis of vertical ozone profiles , 2009 .

[7]  Jean-Paul Hettelingh,et al.  Multi-Effect Critical Loads Used in Multi-Pollutant Reduction Agreements in Europe , 2001 .

[8]  Mathieu Vrac,et al.  Future air quality in Europe: a multi-model assessment of projected exposure to ozone , 2012 .

[9]  J. D. Whyatt,et al.  Evaluation of the performance of different atmospheric chemical transport models and inter-comparison of nitrogen and sulphur deposition estimates for the UK , 2015 .

[10]  F. Meleux,et al.  Air quality trends in Europe over the past decade: a first multi-model assessment , 2011 .

[11]  W. Vries,et al.  Critical Loads and Dynamic Risk Assessments: Nitrogen, Acidity and Metals in Terrestrial and Aquatic Ecosystems , 2015 .

[12]  Georgios Fontaras,et al.  Development and review of Euro 5 passenger car emission factors based on experimental results over various driving cycles. , 2014, The Science of the total environment.

[13]  M. Chin,et al.  Global and Regional Radiative Forcing from 20 Reductions in BC, OC and SO4 an HTAP2 Multi-Model Study , 2016 .

[14]  Li Du,et al.  Impacts and mitigation of excess diesel-related NOx emissions in 11 major vehicle markets , 2017, Nature.

[15]  Markus Amann,et al.  Modelling PM2.5 impact indicators in Europe: Health effects and legal compliance , 2015, Environ. Model. Softw..

[16]  D. Simpson,et al.  Comparison of modelled and monitored deposition fluxes of sulphur and nitrogen to ICP-forest sites in Europe , 2005 .

[17]  Philippe Thunis,et al.  Performance of European chemistry transport models as function of horizontal resolution , 2015 .

[18]  J.-P. Hettelingh,et al.  Characterization of Critical Load Exceedances in Europe , 2001 .

[19]  P Grennfelt,et al.  From Acid Rain to Climate Change , 2012, Science.

[20]  Irene C. Dedoussi,et al.  Public health impacts of excess NOx emissions from Volkswagen diesel passenger vehicles in Germany , 2017 .

[21]  J. Andersson,et al.  Have vehicle emissions of primary NO2 peaked? , 2016, Faraday discussions.

[22]  L. Hou,et al.  Public Health Impact and Economic Costs of Volkswagen’s Lack of Compliance with the United States’ Emission Standards , 2016, International journal of environmental research and public health.

[23]  Jens Borken-Kleefeld,et al.  Real-driving emissions from cars and light commercial vehicles - Results from 13 years remote sensing at Zurich/CH , 2014 .

[24]  Hilde Fagerli,et al.  Can we explain the trends in European ozone levels , 2005 .

[25]  Mark A. Sutton,et al.  Governing processes for reactive nitrogen compounds in the European atmosphere , 2012 .

[26]  John German,et al.  NOₓ Control Technologies for Euro 6 Diesel Passenger Cars: Market Penetration and Experimental Performance Assessment , 2015 .

[27]  M. Gauß,et al.  The EMEP MSC-W chemical transport model -- technical description , 2012 .

[28]  D. Simpson,et al.  Deposition and emissions of reactive nitrogen over European forests: A modelling study , 2006 .