Nuclear spin-lattice relaxation in spin-Peierls systems in magnetic fields: model calculations and application to TTF-AuS4C4(CF3)4

The authors have performed proton and fluorine nuclear relaxation measurements on the spin-Peierls system TTF-AuBDT in magnetic fields below and above the threshold of the field-induced phase transition. They present a calculation of the relaxation rates based on a Luttinger model approach, on the basis of which the data in the dimerised low-field phase are analysed. The results of this model are compared with a perturbative approach used by Ehrenfreund and Smith (1977). The authors calculations yield qualitatively different results and the field dependence of the relaxation rates is described better.

[1]  L. Regnault,et al.  Structural studies of the spin-Peierls system TTF(Au)BDT , 1985 .

[2]  Brom.,et al.  Evidence for an incommensurate high-field phase in the spin-Peierls system tetrathiafulvalene-AuS4C4(CF3) 4. , 1985, Physical review letters.

[3]  G. Kramer,et al.  An NMR and Specific Heat Study of the Spin-Peierls system TTF-Aubdt , 1985 .

[4]  J. Northby,et al.  Field‐dependent specific heat study of the spin‐Peierls transition in TTF–AuS4C4(CF3)4 , 1982 .

[5]  A. Kotani,et al.  Commensurate and Incommensurate States of a Spin-Peierls System in a Magnetic Field , 1982 .

[6]  J. Northby,et al.  Field-Dependent Differential Susceptibility Studies on Tetrathiafulvalene-AuS4C4(CF3)4: Universal Aspects of the Spin-Peierls Phase Diagram , 1982 .

[7]  H. Fukuyama,et al.  Dimerization and Solitons in One-Dimensional XY-Z Antiferromagnets , 1981 .

[8]  H. Fukuyama,et al.  Solitons in Spin-Peierls Systems and Applications to Polyacetylene , 1980 .

[9]  T. Klaassen,et al.  Spin dynamics of an antiferromagnetic Heisenberg chain at low temperatures , 1979 .

[10]  J. Fabre,et al.  Electron-proton couplings and local susceptibilities in TTF and TCNQ salts , 1979 .

[11]  M. Cross,et al.  A new theory of the spin-Peierls transition with special relevance to the experiments on TTFCuBDT , 1979 .

[12]  E. Ehrenfreund,et al.  Nuclear-spin-lattice relaxation process in spin-Peierls systems , 1977 .

[13]  A. Heeger,et al.  Nuclear relaxation studies of the spin-Peierls transition☆ , 1976 .

[14]  J. M. Luttinger An Exactly Soluble Model of a Many‐Fermion System , 1963 .