Quantum optics of two-level atoms in a dielectric: comparison of macroscopic and microscopic quantizations of the dielectric

Abstract We obtain Langevin–Bloch equations of motion for optically resonant atoms embedded in a dielectric host using both the conventional macroscopic quantization of the field in a dielectric and the microscopic quantization of the Lorentz model of enumerated oscillators embedded in the vacuum. The two sets of equations of motion exhibit substantial differences in their dependence on the index of refraction of the host dielectric medium. We compare and contrast the essential conceptual features of the macroscopic and microscopic theories, relating the inconsistency of the results to differences in the underlying Maxwellian and Lorentzian descriptions of the interaction of the radiation with the vacuum and matter. We invoke the correspondence principle to discriminate between the two results and demonstrate that quantization of the macroscopic Maxwell equations leads to incorrect equations of motion for embedded two-level atoms while the microscopic result is consistent with the correspondence principle.

[1]  Albert Einstein,et al.  Ideas and Opinions , 1954 .

[2]  M. Schuurmans,et al.  Superfluorescence: Quantum-mechanical derivation of Maxwell-Bloch description with fluctuating field source , 1979 .

[3]  Effects of local fields on spontaneous emission in dielectric media , 2000, Physical review letters.

[4]  Bowden,et al.  Intrinsic optical bistability in collections of spatially distributed two-level atoms. , 1986, Physical review. A, General physics.

[5]  D. Marcuse,et al.  Principles of quantum electronics , 1980 .

[6]  S. Ho,et al.  Quantum optics in a dielectric: macroscopic electromagnetic-field and medium operators for a linear dispersive lossy medium-a microscopic derivation of the operators and their commutation relations , 1993 .

[7]  Lorentz local-field effects on spontaneous emission in dielectric media , 2000 .

[8]  M. Fleischhauer Spontaneous emission and level shifts in absorbing disordered dielectrics and dense atomic gases: A Green’s-function approach , 1999, quant-ph/9902076.

[9]  W. Louisell Quantum Statistical Properties of Radiation , 1973 .

[10]  Benedict,et al.  Reflection and transmission of ultrashort light pulses through a thin resonant medium: Local-field effects. , 1991, Physical review. A, Atomic, molecular, and optical physics.

[11]  S. Scheel,et al.  Spontaneous decay of an excited atom in an absorbing dielectric , 1999, Technical Digest. CLEO/Pacific Rim '99. Pacific Rim Conference on Lasers and Electro-Optics (Cat. No.99TH8464).

[12]  Stephen M. Barnett,et al.  Decay of excited atoms in absorbing dielectrics , 1996 .

[13]  Richard H. Pantell,et al.  Fundamentals of quantum electronics , 1969 .

[14]  S. Barnett,et al.  Quantum local-field corrections and spontaneous decay , 1999 .

[15]  J. Eberly,et al.  Optical resonance and two-level atoms , 1975 .

[16]  S. Mukamel,et al.  Intermolecular forces, spontaneous emission, and superradiance in a dielectric medium: Polariton-mediated interactions. , 1989, Physical review. A, General physics.

[17]  P. L. Knight,et al.  Retardation in the resonant interaction of two identical atoms , 1974 .

[18]  Peter W. Milonni,et al.  Field Quantization and Radiative Processes in Dispersive Dielectric Media , 1995 .

[19]  Barnett,et al.  Spontaneous emission in absorbing dielectric media. , 1992, Physical review letters.

[20]  Bowden,et al.  Local-field effects in a dense collection of two-level atoms embedded in a dielectric medium: Intrinsic optical bistability enhancement and local cooperative effects. , 1996, Physical review. A, Atomic, molecular, and optical physics.