Structure of boroaluminosilicate glasses: Impact of [Al2O3]/[SiO2] ratio on the structural role of sodium

Q. J. Zheng,1,2 R. E. Youngman,2,* C. L. Hogue,2 J. C. Mauro,2 M. Potuzak,2 M. M. Smedskjaer,2 and Y. Z. Yue1,3 1Section of Chemistry, Aalborg University, DK-9000 Aalborg, Denmark 2Science & Technology Division, Corning Incorporated, Corning, New York 14831, USA 3Shandong Key Laboratory of Glass and Ceramics, Shandong Polytechnic University, 250353 Jinan, China (Received 28 March 2012; published 22 August 2012)

[1]  P. J. Bray,et al.  Nuclear magnetic resonance studies of the glasses in the system Na2OB2O3SiO2 , 1978 .

[2]  J. Stebbins Effects of temperature and composition on silicate glass structure and dynamics: SI-29 NMR results , 1988 .

[3]  D. Neuville,et al.  Al environment in tectosilicate and peraluminous glasses: A 27Al MQ-MAS NMR, Raman, and XANES investigation , 2004 .

[4]  R. Youngman,et al.  Network Modification in Potassium Borate Glasses: Structural Studies with NMR and Raman Spectroscopies , 1996 .

[5]  Steuernagel,et al.  Z Filtering in MQMAS NMR , 1996, Journal of magnetic resonance. Series A.

[6]  R. Araujo Statistical mechanical model of boron coordination , 1980 .

[7]  Luming Peng,et al.  Sodium germanate glasses and crystals: NMR constraints on variation in structure with composition , 2007 .

[8]  H. Yamashita,et al.  Nuclear magnetic resonance studies of alkaline earth phosphosilicate and aluminoborosilicate glasses , 2000 .

[9]  R. Araujo Statistical mechanics of chemical disorder: application to alkali borate glasses , 1983 .

[10]  D. Neuville,et al.  Advances in understanding the structure of borosilicate glasses: A Raman spectroscopy study , 2009 .

[11]  É. Lippmaa,et al.  Solid-state high-resolution silicon-29 chemical shifts in silicates , 1984 .

[12]  J. Stebbins,et al.  Effects of cation field strength on the structure of aluminoborosilicate glasses: High-resolution 11B, 27Al and 23Na MAS NMR , 2009 .

[13]  T. Charpentier,et al.  Boron Speciation in Soda-Lime Borosilicate Glasses Containing Zirconium , 2010 .

[14]  I. Avramov,et al.  Effect of chemical composition on viscosity of oxide glasses , 2003 .

[15]  S. Sen,et al.  Temperature dependent structural changes in borate, borosilicate and boroaluminate liquids: high-resolution 11B, 29Si and 27Al NMR studies , 1998 .

[16]  T. Rouxel,et al.  Correlation between structure and physical properties of chalcogenide glasses in the AsxSe1-x system , 2010 .

[17]  L. Du,et al.  Network connectivity in aluminoborosilicate glasses: A high-resolution 11B, 27Al and 17O NMR study , 2005 .

[18]  R. Araujo Theoretical prediction of the effect of silica on the formation of BO4 tetrahedra , 1986 .

[19]  J. Stebbins,et al.  Al–O–Al and Si–O–Si sites in framework aluminosilicate glasses with Si/Al=1: quantification of framework disorder , 2000 .

[20]  J. Stebbins,et al.  The distribution of sodium ions in aluminosilicate glasses: A high-field Na-23 MAS and 3Q MAS NMR study , 2003 .

[21]  J. Stebbins,et al.  Quench rate and temperature effects on boron coordination in aluminoborosilicate melts , 2009 .

[22]  J. Stebbins,et al.  NMR evidence for excess non-bridging oxygen in an aluminosilicate glass , 1997, Nature.

[23]  Morten Mattrup Smedskjær,et al.  Composition–structure–property relationships in boroaluminosilicate glasses , 2012 .

[24]  R. E. Youngman,et al.  Multiple boron sites in borate glass detected with dynamic angle spinning nuclear magnetic resonance , 1994 .

[25]  M. Hanaya,et al.  OPTIMIZATION OF TWO-DIMENSIONAL MULTIPLE-QUANTUM MAS NMR EXPERIMENTS FOR I= 3/2 NUCLEI ON A MODERATE-FIELD SPECTROMETER , 1997 .

[26]  A. Pines,et al.  Speciation and local structure in alkali and alkaline earth silicate glasses: Constraints from 29Si NMR spectroscopy , 1987 .

[27]  Karl T. Mueller,et al.  Detection and identification of corrosion products of sodium aluminoborosilicate glasses by 23Na MQMAS and 1H → 23Na CPMAS NMR , 2000 .

[28]  A. P. Taglialavore,et al.  Solid‐state NMR Evidence of 4‐, 5, and 6‐Fold Aluminum Sites in Roller‐Quenched SiO2‐A12O3 Glasses , 1987 .

[29]  S. Sen,et al.  Atomic-scale understanding of structural relaxation in simple and complex borosilicate glasses , 2007 .

[30]  P. J. Bray,et al.  11B NMR studies and structural modeling of Na2O-B2O3-SiO2 glasses of high soda content , 1983 .

[31]  J. Stebbins,et al.  The Structure of Aluminosilicate Glasses: High-Resolution 17O and 27Al MAS and 3QMAS NMR Study , 2000 .

[32]  Y. Yue,et al.  Evidence of Intermediate-Range Order Heterogeneity in Calcium Aluminosilicate Glasses , 2010 .

[33]  G. N. Greaves,et al.  EXAFS and the structure of glass , 1985 .

[34]  S. Gin,et al.  17O 3Q-MAS NMR characterization of a sodium aluminoborosilicate glass and its alteration gel , 2001 .

[35]  John C. Mauro,et al.  Viscosity of glass-forming liquids , 2009, Proceedings of the National Academy of Sciences.

[36]  P. J. Bray,et al.  Change in boron coordination in alkali borate glasses, and mixed alkali effects, as elucidated by NMR , 1989 .

[37]  Yuanzheng Yue,et al.  Topological principles of borosilicate glass chemistry. , 2011, The journal of physical chemistry. B.

[38]  H. Yamashita,et al.  Nuclear magnetic resonance studies of 0.139MO (or M′2O) · 0.673SiO2 · (0.188−x)Al2O3 · xB2O3 (M=Mg, Ca, Sr and Ba, M′=Na and K) glasses , 2003 .

[39]  T. Charpentier,et al.  Effect of temperature and thermal history on borosilicate glass structure , 2012 .

[40]  B. Boizot,et al.  A structural approach by MAS NMR spectroscopy of mechanisms occurring under β-irradiation in mixed alkali aluminoborosilicate glasses , 2004 .

[41]  S. Sen,et al.  High-Resolution Multinuclear NMR Structural Study of Binary Aluminosilicate and Other Related Glasses , 2004 .

[42]  G. Cody,et al.  The effect of Na/Si on the structure of sodium silicate and aluminosilicate glasses quenched from melts at high pressure : A multi-nuclear (Al-27, Na-23, O-17) 1D and 2D solid-state NMR study , 2006 .

[43]  John C. Mauro,et al.  Quantitative Design of Glassy Materials Using Temperature-Dependent Constraint Theory , 2010 .

[44]  R. Youngman,et al.  ON THE FORMATION OF TETRACOORDINATE BORON IN RUBIDIUM BORATE GLASSES , 1995 .

[45]  G. Hoatson,et al.  Modelling one‐ and two‐dimensional solid‐state NMR spectra , 2002 .

[46]  Angular rigidity in tetrahedral network glasses with changing composition , 2011 .

[47]  J. Stebbins Cation sites in mixed-alkali oxide glasses: correlations of NMR chemical shift data with site size and bond distance , 1998 .

[48]  E. Kamitsos,et al.  Molecular dynamics investigation of mixed-alkali borate glasses: Short-range order structure and alkali-ion environments , 2009 .

[49]  L. Du,et al.  Solid-state NMR study of metastable immiscibility in alkali borosilicate glasses , 2001 .

[50]  Y. Yue Characteristic temperatures of enthalpy relaxation in glass , 2008 .

[51]  É. Lippmaa,et al.  Structural studies of silicates by solid-state high-resolution silicon-29 NMR , 1980 .