A hybrid in situ bioremediation/pulsed pumping strategy has been developed to cost effectively remediate a carbon tetrachloride plume in Schoolcraft, Michigan. The pulsed pumping system uses a line of alternating injection and extraction wells perpendicular to the direction of natural groundwater flow. The wells pump periodically to clean the recirculation zone between adjacent wells. During the pump-off phase, natural groundwater flow brings new contaminant into the recirculation zone. The wells are pumped again prior to breakthrough of contaminant from the recirculation zone. A computationally efficient reactor model has been developed, which conceptually divides the aquifer into injection, extraction, and recirculation zones, which are represented by a network of chemical reactors. Solute concentration histories from three-dimensional finite difference simulations and from field data confirm the reactor model predictions. The reactor model is used to investigate the optimal well configuration, pumping rate, and pumping schedule for achieving maximum pollutant degradation.
[1]
H. S. Fogler,et al.
Elements of Chemical Reaction Engineering
,
1986
.
[2]
M J Dybas,et al.
Localization and Characterization of the Carbon Tetrachloride Transformation Activity of Pseudomonas sp. Strain KC
,
1995,
Applied and environmental microbiology.
[3]
James M. Tiedje,et al.
Pilot-Scale Evaluation of Bioaugmentation for In-Situ Remediation of a Carbon Tetrachloride-Contaminated Aquifer
,
1998
.
[4]
James M. Tiedje,et al.
Hydraulic Characterization and Design of a Full‐Scale Biocurtain
,
2000
.
[5]
O. Levenspiel.
Chemical Reaction Engineering
,
1972
.
[6]
Mark Bakker,et al.
Capture Zone Delineation in Two-Dimensional Groundwater Flow Models
,
1996
.
[7]
C. Criddle,et al.
Development, operation, and long-term performance of a full-scale biocurtain utilizing bioaugmentation.
,
2002,
Environmental science & technology.