Generation of hard x rays by ultrafast terawatt lasers

A compact, tabletop terawatt Ti:sapphire laser drive, ultrafast hard x-ray source for time-resolved x-ray diffraction studies is described. With a copper target the energy conversion efficiency from laser photons (800 nm) to copper K x-ray radiation (1.54 A) is 0.008%. The optimal laser intensity for generating these x rays is 1018 W cm−2, lower than the highest laser intensity available (5×1018 W cm−2) from the laser system. These results are consistent with a theoretical model proposed on the basis that the x rays are produced as a result of laser driven electron ionization of core level electrons of Cu atoms near room temperature. This source also provides features such as ultrashort pulse duration, extremely small source size, variable wavelengths, high peak spectral brightness, and the potential for multiple beam line experiments. X-ray diffraction patterns from GaAs single crystals and amorphous Ni films recorded with this source are presented.

[1]  A. Cavalleri,et al.  Picosecond–milliångström lattice dynamics measured by ultrafast X-ray diffraction , 1999, Nature.

[2]  Glover,et al.  Generation of femtosecond pulses of synchrotron radiation , 2000, Science.

[3]  Christopher P. P. Barty,et al.  Picosecond-milliangstrom resolution dynamics by ultrafast x-ray diffraction , 1997, Optics & Photonics.

[4]  K R Wilson,et al.  Generation of 18-fs, multiterawatt pulses by regenerative pulse shaping and chirped-pulse amplification. , 1996, Optics letters.

[5]  L. Alexander,et al.  X-Ray diffraction procedures for polycrystalline and amorphous materials , 1974 .

[6]  G. Mourou,et al.  Terawatt to Petawatt Subpicosecond Lasers , 1994, Science.

[7]  Miriam Rossi,et al.  Crystal Structure Analysis for Chemists and Biologists , 1994 .

[8]  I. Tomov,et al.  High repetition rate picosecond laser system at 1983 nm , 1992 .

[9]  Gauthier,et al.  Efficient K alpha x-ray source from femtosecond laser-produced plasmas. , 1994, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics.

[10]  K R Wilson,et al.  Detection of nonthermal melting by ultrafast X-ray diffraction. , 1999, Science.

[11]  J. Squier,et al.  X-ray Diffraction Study of Laser-Material Interactions with an Ultrafast Table-Top X-ray Source , 1997 .

[12]  Patrick Audebert,et al.  Femtosecond time-resolved X-ray diffraction from laser-heated organic films , 1997, Nature.

[13]  P M Bell,et al.  Time-gated imaging with an ultrashort-pulse, laser-produced-plasma x-ray source. , 1995, Optics letters.

[14]  Gerard Mourou,et al.  Ultrafast x‐ray sources* , 1993 .

[15]  G. M. Davis,et al.  Plasma x-ray source for lithography generated by a ≃30 J, 30 ns KrF laser , 1988 .

[16]  J. Gauthier,et al.  X-ray emission produced by hot electrons from fs-laser produced plasma— diagnostic and application , 1999 .

[17]  Kwanpyo Kim,et al.  Femtosecond X-ray Pulses at 0.4 Å Generated by 90° Thomson Scattering: A Tool for Probing the Structural Dynamics of Materials , 1996, Science.

[18]  Teubner,et al.  Angle-dependent x-ray emission and resonance absorption in a laser-produced plasma generated by a high intensity ultrashort pulse. , 1993, Physical review letters.

[19]  Falcone,et al.  Murnane, Kapteyn, and Falcone reply. , 1989, Physical review letters.

[20]  Perry,et al.  Strong x-ray emission from high-temperature plasmas produced by intense irradiation of clusters. , 1995, Physical review letters.

[21]  W. Leemans,et al.  Ultrafast Structural Dynamics in InSb Probed by Time-Resolved X-Ray Diffraction , 1999 .

[22]  M. Rosen,et al.  Ultrafast X-ray Pulses from Laser-Produced Plasmas , 1991, Science.

[23]  Freeman,et al.  Resistivity of a simple metal from room temperature to 106 K. , 1988, Physical review letters.

[24]  S. Wilks,et al.  Absorption of ultrashort, ultra-intense laser light by solids and overdense plasmas , 1997 .

[25]  K Yamakawa,et al.  A 50 EW/cm;2 Ti:sapphire laser system for studying relativistic light-matter interactions. , 1999, Optics express.

[26]  S. Svanberg,et al.  X-ray generation for medical applications from a laser-produced plasma , 1996 .

[27]  C. E. Dick,et al.  Large‐angle L x‐ray production by electrons , 1973 .

[28]  L. Alexander,et al.  X-ray diffraction procedures , 1954 .

[29]  Chen,et al.  Hot-electron characterization from K alpha measurements in high-contrast, p-polarized, picosecond laser-plasma interactions. , 1993, Physical review letters.

[30]  A. Moffat Opening the Door to More Membrane Protein Structures , 1997, Science.

[31]  Howard A. Padmore,et al.  Ultrafast structural changes measured by time-resolved X-ray diffraction , 1998 .

[32]  P. Albouy,et al.  Subpicosecond X-ray diffraction study of laser-induced disorder dynamics above the damage threshold of organic solids , 1999 .

[33]  J. Squier,et al.  Hybrid vacuum-atmosphere compressors for ultrafast, high-peak power chirped-pulse amplification , 1998 .

[34]  Y. Fujimoto,et al.  ENHANCEMENT OF HARD X-RAY EMISSION FROM A COPPER TARGET BY MULTIPLE SHOTS OF FEMTOSECOND LASER PULSES , 1999 .

[35]  Hans M. Hertz,et al.  Ultraviolet prepulse for enhanced x‐ray emission and brightness from droplet‐target laser plasmas , 1996 .

[36]  Miquel,et al.  Experimental Confirmation of Ponderomotive-Force Electrons Produced by an Ultrarelativistic Laser Pulse on a Solid Target. , 1996, Physical review letters.

[37]  Graeme Morrison,et al.  X-Ray Microscopy III , 1992 .

[38]  Jeffrey Dellert Kmetec,et al.  Ultrafast laser generation of hard X-rays , 1992 .

[39]  Harris,et al.  MeV x-ray generation with a femtosecond laser. , 1992, Physical review letters.

[40]  P. Lee,et al.  Experimental widths of K and L x-ray lines , 1976 .

[41]  O. Peyrusse,et al.  Picosecond dynamics of a hot solid-density plasma , 1996 .

[42]  Yasushi Fujimoto,et al.  Generation of picosecond hard x rays by tera watt laser focusing on a copper target , 1998 .

[43]  J. Wark Time-resolved X-ray diffraction , 1996 .

[44]  B. Cullity,et al.  Elements of X-ray diffraction , 1957 .

[45]  Boris N. Chichkov,et al.  Short-pulse laser ablation of solid targets , 1996 .

[46]  Y. Fujimoto,et al.  Picosecond Pulsed X-Ray Diffraction from a Pulsed Laser Heated Si(111) , 1999 .

[47]  T. Nishikawa,et al.  Effects of an ultrashort prepulse on soft X-ray generation from an aluminium plasma produced by femtosecond Ti:Sapphire laser pulses , 1996 .

[48]  D. Leitner,et al.  Anharmonic lattice dynamics in germanium measured with ultrafast x-ray diffraction. , 2000, Physical review letters.

[49]  P. Nickles,et al.  Energetic electrons and x-ray photons from multiterawatt Ti:sapphire lasers , 1999 .

[50]  J. J. Macklin,et al.  0.5-TW, 125-fs Ti:sapphire laser. , 1991, Optics letters.

[51]  Yasushi Fujimoto,et al.  Spectroscopy of Hard X-Rays (2–15 keV) Generated by Focusing Femtosecond Laser on Metal Targets , 1999 .