Development of a land use regression model for daily NO2 and NOx concentrations in the Brisbane metropolitan area, Australia

Abstract Land use regression models are an established method for estimating spatial variability in gaseous pollutant levels across urban areas. Existing LUR models have been developed to predict annual average concentrations of airborne pollutants. None of those models have been developed to predict daily average concentrations, which are useful in health studies focused on the acute impacts of air pollution. In this study, we developed LUR models to predict daily NO 2 and NO x concentrations during 2009–2012 in the Brisbane Metropolitan Area (BMA), Australia's third-largest city. The final models explained 64% and 70% of spatial variability in NO 2 and NO x , respectively, with leave-one-out-cross-validation R 2 of 3–49% and 2–51%. Distance to major road and industrial area were the common predictor variables for both NO 2 and NO x , suggesting an important role for road traffic and industrial emissions. The novel modeling approach adopted here can be applied in other urban locations in epidemiological studies.

[1]  Lidia Morawska,et al.  Characteristics of ultrafine particle sources and deposition rates in primary school classrooms , 2014 .

[2]  R. Tibshirani,et al.  Least angle regression , 2004, math/0406456.

[3]  J. Gulliver,et al.  A review of land-use regression models to assess spatial variation of outdoor air pollution , 2008 .

[4]  Giorgio Cattani,et al.  Development of nitrogen dioxide and volatile organic compounds land use regression models to estimate air pollution exposure near an Italian airport , 2016 .

[5]  Michael Brauer,et al.  Application of land use regression to estimate long-term concentrations of traffic-related nitrogen oxides and fine particulate matter. , 2007, Environmental science & technology.

[6]  Kees de Hoogh,et al.  Western European land use regression incorporating satellite- and ground-based measurements of NO2 and PM10. , 2013, Environmental science & technology.

[7]  John S. Gulliver,et al.  Development and transferability of a nitrogen dioxide land use regression model within the Veneto region of Italy , 2015 .

[8]  Bert Brunekreef,et al.  Comparison of land-use regression models for predicting spatial NOx contrasts over a three year period in Oslo, Norway , 2011 .

[9]  Bert Brunekreef,et al.  Modeling the intra-urban variability of outdoor traffic pollution in Oslo, Norway—A GA2LEN project , 2007 .

[10]  Adam Szpiro,et al.  Improving spatial concentration estimates for nitrogen oxides using a hybrid meteorological dispersion/land use regression model in Los Angeles, CA and Seattle, WA. , 2010, The Science of the total environment.

[11]  Marcela Rivera,et al.  Effect of the number of measurement sites on land use regression models in estimating local air pollution , 2012 .

[12]  Giovanna Capizzi,et al.  A Least Angle Regression Control Chart for Multidimensional Data , 2011, Technometrics.

[13]  Johan Lindström,et al.  Comparing universal kriging and land-use regression for predicting concentrations of gaseous oxides of nitrogen (NOx) for the Multi-Ethnic Study of Atherosclerosis and Air Pollution (MESA Air). , 2011, Atmospheric environment.

[14]  H. Akaike A new look at the statistical model identification , 1974 .

[15]  Shaofei Kong,et al.  A land use regression for predicting NO2 and PM10 concentrations in different seasons in Tianjin region, China. , 2010, Journal of environmental sciences.

[16]  Yan Zhang,et al.  A land use regression model for estimating the NO2 concentration in Shanghai, China. , 2015, Environmental research.

[17]  Paul H. C. Eilers,et al.  Flexible smoothing with B-splines and penalties , 1996 .

[18]  Jean-Michel Guldmann,et al.  Land-use regression panel models of NO2 concentrations in Seoul, Korea , 2015 .

[19]  Bert Brunekreef,et al.  Spatial variability of fine particle concentrations in three European areas , 2002 .

[20]  B. Brunekreef,et al.  Systematic evaluation of land use regression models for NO₂. , 2012, Environmental science & technology.

[21]  Julian D Marshall,et al.  A national satellite-based land-use regression model for air pollution exposure assessment in Australia. , 2014, Environmental research.

[22]  Lidia Morawska,et al.  Spatial variation of particle number concentration in school microscale environments and its impact on exposure assessment. , 2013, Environmental science & technology.

[23]  Lianfa Li,et al.  Use of generalized additive models and cokriging of spatial residuals to improve land-use regression estimates of nitrogen oxides in Southern California. , 2012, Atmospheric environment.

[24]  J. Neter,et al.  Applied Linear Regression Models , 1983 .

[25]  Bert Brunekreef,et al.  Land use regression models for estimating individual NOx and NO₂ exposures in a metropolis with a high density of traffic roads and population. , 2014, The Science of the total environment.

[26]  Bert Brunekreef,et al.  Development of NO2 and NOx land use regression models for estimating air pollution exposure in 36 study areas in Europe - The ESCAPE project , 2013 .

[27]  Michael Brauer,et al.  The transferability of NO and NO2 land use regression models between cities and pollutants , 2011 .

[28]  B. Brunekreef,et al.  Estimation of outdoor NO(x), NO(2), and BTEX exposure in a cohort of pregnant women using land use regression modeling. , 2008, Environmental science & technology.

[29]  Nectarios Rose,et al.  Validation of a spatiotemporal land use regression model incorporating fixed site monitors. , 2011, Environmental science & technology.

[30]  David Blake,et al.  Development of Land Use Regression models for predicting exposure to NO2 and NOx in Metropolitan Perth, Western Australia , 2015, Environ. Model. Softw..

[31]  Daniela Fecht,et al.  Back-extrapolated and year-specific NO2 land use regression models for Great Britain - Do they yield different exposure assessment? , 2016, Environment international.

[32]  Vlad Isakov,et al.  Evaluation of land-use regression models used to predict air quality concentrations in an urban area , 2010 .