The relative stability of two-dimensional soft quasicrystals in systems with two length scales is examined using a recently developed projection method, which provides a unified numerical framework to compute the free energy of periodic crystal and quasicrystals. Accurate free energies of numerous ordered phases, including dodecagonal, decagonal, and octagonal quasicrystals, are obtained for a simple model, i.e., the Lifshitz-Petrich free-energy functional, of soft quasicrystals with two length scales. The availability of the free energy allows us to construct phase diagrams of the system, demonstrating that, for the Lifshitz-Petrich model, the dodecagonal and decagonal quasicrystals can become stable phases, whereas the octagonal quasicrystal stays as a metastable phase.
[1]
P. Paufler,et al.
Quasicrystals and Geometry
,
1997
.
[2]
C. Janot,et al.
Quasicrystals: A Primer
,
1992
.
[3]
T. Lubensky,et al.
Principles of condensed matter physics
,
1995
.
[4]
T. Janssen,et al.
Aperiodic Crystals: From Modulated Phases to Quasicrystals
,
2007
.
[5]
W. Steurer,et al.
Crystallography of Quasicrystals: Concepts, Methods and Structures
,
2009
.